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In this paper we study magnetoelectric effects in two-dimensional magnetic bilayers and introduce the notion of a layer dipole magnetoelectric polarizability. This magnetoelectric polarizability describes the magnetization response to an…

Strongly Correlated Electrons · Physics 2025-12-08 H. Radhakrishnan , C. Ortix , J. W. F. Venderbos

We show that the surface of a centrosymmetric, collinear, compensated antiferromagnet, which hosts bulk ferroically ordered magnetic octupoles, exhibits a linear magnetoelectric effect, a net magnetization, and a net electric dipole moment.…

Materials Science · Physics 2025-06-10 Sayantika Bhowal , Andrea Urru , Sophie F. Weber , Nicola A. Spaldin

We uncover a new pathway towards multiferroicity, showing how magnetism can drive ferroelectricity without relying on inversion symmetry breaking of the magnetic ordering. Our free-energy analysis demonstrates that any commensurate…

Materials Science · Physics 2009-11-11 Joseph J. Betouras , Gianluca Giovannetti , Jeroen van den Brink

Perovskite manganites with small A-site ions, as the first and canonical branch of type-II multiferroics, are ideal systems to exhibit magnetism-induced ferroelectricity. Despite their established magnetoelectric phase diagrams under low…

Materials Science · Physics 2026-01-15 Ming Yang , Jun Chen , Junfeng Wang , Chao Dong , Chengliang Lu , Gang Xu , Jinguang Cheng , Jianshi Zhou , Shuai Dong

We show that anisotropic energy of a 2D antiferromagnet is greatly enhanced via stacking on a magnetic substrate layer, arising from the sublattice-dependent interlayer magnetic interaction that defines an effective anisotropic energy.…

Mesoscale and Nanoscale Physics · Physics 2022-08-16 Feiping Xiao , Qingjun Tong

The discovery of atomically thin van der Waals ferroelectric and magnetic materials encourages the exploration of 2D multiferroics, which holds the promise to understand fascinating magnetoelectric interactions and fabricate advanced…

Materials Science · Physics 2023-07-21 Shuang Wu , Xinyu Chen , Canyu Hong , Xiaofei Hou , Zhanshan Wang , Zhiyuan Sheng , Zeyuan Sun , Yanfeng Guo , Shiwei Wu

Skyrmions and antiskyrmions are topologically protected spin structures with opposite topological charge. Particularly in coexisting phases, these two types of magnetic quasi-particles may show fascinating physics and potential for…

Using neutron diffraction, we have studied the magnetic field effect on charge structures in the charge-ordered multiferroic material LuFe$_2$O$_4$. An external magnetic field is able to change the magnitude and correlation lengths of the…

Strongly Correlated Electrons · Physics 2009-04-10 Jinsheng Wen , Guangyong Xu , Genda Gu , S. M. Shapiro Brookhaven National Laboratory

Two-dimensional multiferroic materials are highly sought after due to their huge potential for applications in nanoelectronic and spintronic devices. Here, we predict, based on first-principle calculations, a single phase {\it triferroic}…

Materials Science · Physics 2022-11-07 Srishti Bhardwaj , T. Maitra

Electric field control of magnetism in solids, i.e. the converse magnetoelectricity, is highly desired for applications of scalable energy-efficient logic devices. However, it is not only a technical challenge but also a scientific paradox,…

Materials Science · Physics 2024-08-16 Ying Zhou , Haoshen Ye , Junting Zhang , Shuai Dong

The realization of multiferroics in nanostructures, combined with a large electric dipole and ferromagnetic ordering, could lead to new applications, such as high-density multi-state data storage. Although multiferroics have been broadly…

Materials Science · Physics 2018-04-18 Chengxi Huang , Yongping Du , Haiping Wu , Hongjun Xiang , Kaiming Deng , Erjun Kan

Ferroelectric control of altermagnetism in momentum space has been studied widely, while the control of magnetism in real space of altermagnets are still rare. We present a design rule to identify multiferroicity in n=2 Ruddlesden-Popper…

Materials Science · Physics 2025-08-20 Ying Zhou , Hui-Min Zhang , Cheng-Ao Ji , Hongjun Xiang , Shuai Dong , James M. Rondinelli , Xue-Zeng Lu

The concepts of topology have a profound impact on physics research spanning the fields of condensed matter, photonics and acoustics and predicting topological states that provide unprecedented versatility in routing and control of waves of…

Ferroics, characterized by a broken symmetry state with nonzero elastic, polar, or magnetic order parameters $\vec{u}$, are recognized platforms for staging and manipulating topologically-protected structures as well as for detecting…

Materials Science · Physics 2018-10-31 Antonio B. Mei , Ramamoorthy Ramesh , Darrell G. Schlom

An appealing mechanism for inducing multiferroicity in materials is the generation of electric polarization by a spatially varying magnetization that is coupled to the lattice through the spin-orbit interaction. Here we describe the…

Two-dimensional (2D) multiferroics exhibit cross-control capacity between magnetic and electric responses in reduced spatial domain, making them well suited for next-generation nanoscale devices; however, progress has been slow in…

Materials Science · Physics 2020-05-15 Jing Shang , Chun Li , Aijun Du , Ting Liao , Yuantong Gu , Yandong Ma , Liangzhi Kou , Changfeng Chen

Multiferroics, materials where spontaneous long-range magnetic and dipolar orders coexist, represent an attractive class of compounds, which combine rich and fascinating fundamental physics with a technologically appealing potential for…

Materials Science · Physics 2015-05-13 Silvia Picozzi , Claude Ederer

The structural, electronic and lattice dielectric properties of multiferroic TbMn$_2$O$_5$ are investigated using density functional theory within the generalized gradient approximation (GGA). We use collinear spin approximations and ignore…

Materials Science · Physics 2009-11-13 Chenjie Wang , Guang-Can Guo , Lixin He

We present a theoretical study of the onset of electric polarization close to a surface in magnetic materials and in thin films and multilayers. We consider two different paths that lead to the onset of multiferroic behavior at the boundary…

Materials Science · Physics 2021-05-12 Ahmed R. Tarkhany , Marco Discacciati , Joseph J. Betouras

Density-functional calculations are carried out to investigate incommensurate magnetic structures and ferroelectric polarization in newly discovered multiferroic material MnI$_2$. The exchange interactions among local moments on Mn are…

Strongly Correlated Electrons · Physics 2013-05-30 Xianxin Wu , Yingxiang Cai , Qing Xie , Hongming Weng , Heng Fan , Jiangping Hu