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The optical properties of transition metal dichalcogenide monolayers such as the two-dimensional semiconductors MoS$_2$ and WSe$_2$ are dominated by excitons, Coulomb bound electron-hole pairs. The light emission yield depends on whether…

Materials Science · Physics 2016-03-23 J. P. Echeverry , B. Urbaszek , T. Amand , X. Marie , I. C. Gerber

In transition metal dichalcogenides layers of atomic scale thickness, the electron-hole Coulomb interaction potential is strongly influenced by the sharp discontinuity of the dielectric function across the layer plane. This feature results…

The optical responses of semiconducting transition metal dichalcogenides are dominated by excitons. Being able to strongly interact with light and other materials excitations, excitons in semiconductors are prototypes for investigating…

Mesoscale and Nanoscale Physics · Physics 2021-01-28 Xuke Jiang , Masoud Taleb , Florian Diekmann , Kai Rossnagel , Nahid Talebi

Optical spectroscopy of ultimately thin materials has significantly enhanced our understanding of collective excitations in low-dimensional semiconductors. This is particularly reflected by the rich physics of excitons in atomically thin…

We study carrier interaction induced many-body effects on the excitonic optical properties of highly photoexcited one-dimensional semiconductor quantum wire systems by solving the dynamically screened Bethe-Salpeter equation using realistic…

Strongly Correlated Electrons · Physics 2009-11-07 D. W. Wang , S. Das Sarma

Single-layer WS$_2$ is a direct-gap semiconductor showing strong excitonic photoluminescence features in the visible spectral range. Here, we present temperature-dependent photoluminescence measurements on mechanically exfoliated…

Mesoscale and Nanoscale Physics · Physics 2015-09-08 Gerd Plechinger , Philipp Nagler , Julia Kraus , Nicola Paradiso , Christoph Strunk , Christian Schüller , Tobias Korn

Calculations combining first-principles electron-phonon ($e$-ph) interactions with the Boltzmann equation enable studies of ultrafast carrier and phonon dynamics. However, in materials with weak Coulomb screening, electrons and holes form…

Materials Science · Physics 2022-10-13 Hsiao-Yi Chen , Marco Bernardi

Excitons are key quasiparticles determining the optical properties of solids. As such, they can be utilized to coherently control the electronic structure of materials using optical femtosecond pulses. Identifying the decoherence mechanism…

Strong Coulomb interaction in atomically-thin transition metal dichalcogenides makes these systems particularly promising for studies of excitonic physics. Of special interest are the manifestations of the charged excitons, also known as…

Mesoscale and Nanoscale Physics · Physics 2020-08-26 M. M. Glazov

Excitons -- elementary excitations formed by bound electron-hole pairs -- govern the optical properties and excited-state dynamics of materials. In two-dimensions (2D), excitons are theoretically predicted to have a linear energy-momentum…

Materials Science · Physics 2025-03-14 Luna Y. Liu , Steffi Y. Woo , Jinyuan Wu , Bowen Hou , Cong Su , Diana Y. Qiu

Spatially structured light fields applied to semiconductor quantum dots yield fundamentally different absorption spectra than homogeneous beams. In this paper, we theoretically discuss the resulting spectra for different light beams using a…

Mesoscale and Nanoscale Physics · Physics 2020-11-04 M. Holtkemper , G. F. Quinteiro , D. E. Reiter , T. Kuhn

Applying the novel exact-exchange (EXX) Kohn-Sham method within time-dependent density-functional theory, we obtained the optical absorption spectrum of bulk silicon in good agreement with experiments including excitonic features. Analysis…

Materials Science · Physics 2016-01-01 Yong-Hoon Kim , Andreas Goerling

The exciton binding energy ($E_b$) is a key parameter that governs the physics of many optoelectronic devices. At their best, trustworthy and precise measurements of $E_b$ challenge theoreticians to refine models, are a driving force in…

Materials Science · Physics 2023-06-27 Kameron R. Hansen , John S. Colton , Luisa Whittaker-Brooks

Low-dimensional materials differ from their bulk counterpart in many respects. In particular, the screening of the Coulomb interaction is strongly reduced, which can have important consequences such as the significant increase of exciton…

We simulate the time-dependent coherent dynamics of a spatially indirect exciton (an electron-hole pair with the two particles confined in different layers) in a GaAs coupled quantum well system. We use a unitary wave-packet propagation…

Mesoscale and Nanoscale Physics · Physics 2016-05-25 Federico Grasselli , Andrea Bertoni , Guido Goldoni

Resonant optical excitation of few-level quantum systems enables coherent quantum control, resonance fluorescence, and direct characterization of dephasing mechanisms. Experimental demonstrations have been achieved in a variety of atomic…

Mesoscale and Nanoscale Physics · Physics 2016-04-20 S. Kumar , M. Brotons-Gisbert , R. Al-Khuzheyri , A. Branny , G. Ballesteros-Garcia , J. F. Sanchez-Royo , B. D. Gerardot

Atomically thin two-dimensional crystals have revolutionized materials science. In particular, monolayer transition metal dichalcogenides promise novel optoelectronic applications, due to their direct energy gaps in the optical range. Their…

In semiconductor physics, many essential optoelectronic material parameters can be experimentally revealed via optical spectroscopy in sufficiently large magnetic fields. For monolayer transition-metal dichalcogenide semiconductors, this…

Mesoscale and Nanoscale Physics · Physics 2020-08-20 M. Goryca , J. Li , A. V. Stier , T. Taniguchi , K. Watanabe , E. Courtade , S. Shree , C. Robert , B. Urbaszek , X. Marie , S. A. Crooker

The negatively charged quasi-two-dimensional exciton ($X^-$) is studied numerically in the presence of a uniform B-field and various in-plane confinements. The corresponding photoluminescence (PL) spectra, including shakeup processes, are…

Condensed Matter · Physics 2009-10-30 J. R. Chapman , N. F. Johnson , V. N. Nicopoulos

Excitons and their correlated complexes underpin the rich photophysics of quantum-confined semiconductors. Among these, biexcitons -- bound states of two electrons and two holes -- provide a sensitive probe of Coulomb correlations,…

Materials Science · Physics 2026-01-23 Katherine A. Koch , Carlos Silva-Acuña , Ajay Ram Srimath Kandada