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The Haldane spin-chain compound, Tb2BaNiO5, with two antiferromagnetic transitions, one at T1=63K, and the other at T2=25K, has been recently shown by us to be an exotic multiferroic below T2. Here, we report the results of our…

Strongly Correlated Electrons · Physics 2019-09-04 Sanjay K Upadhyay , E. V. Sampathkumaran

The Haldane-spin chain compound, Tb2BaNiO5, has been known to be an exotic multiferroic system, exhibiting antiferromagnetic anomalies at T_N1= 63 K and T_N2= 25 K, with ferroelectricity appearing below T_N2 only. Previous reports in…

Strongly Correlated Electrons · Physics 2023-05-24 Ram Kumar , S. Rayaprol , A. Hoser , E. V. Sampathkumaran

We report an unusual canted magnetism due to 3d and 4f electrons, occupying two different crystallographic sites, with its consequence to electric dipole order. This is based on neutron powder diffraction measurements on Tb2BaNiO5…

The Haldane spin-chain compound, Tb2BaNiO5, has been known to order antiferromagnetically below (T_N= ) 63 K. The present magnetic studies on the polycrystals bring out that there is another magnetic transition at a lower temperature (T_2=…

Strongly Correlated Electrons · Physics 2019-02-22 Sanjay Kumar Upadhyay , P. L. Paulose , E. V. Sampathkumaran

We have studied the influence of external pressure up to 1 GPa on the magnetic transitions of the orthorhombic Haldane-spin chain compound Tb2BaNiO5 an exotic multiferroic material. This parent compound is known to undergo N\'eel ordering…

Strongly Correlated Electrons · Physics 2021-07-28 K. K. Iyer , Ram Kumar , S. Rayaprol , K. Maiti , E. V. Sampathkumaran

We report the observation of electric polarization in the magnetically ordered state of the Haldane chain compound, Gd$_2$BaNiO$_5$, with strongly correlated magnetic and dielectric properties. The results of dc magnetic susceptibility and…

Materials Science · Physics 2015-06-22 S. Chowki , Tathamay Basu , K. Singh , N. Mohapatra , E. V. Sampathkumaran

We have recently reported that the Haldane spin-chain system, Er2BaNiO5, undergoing antiferromagnetic order below 32 K, is characterized by the onset of ferroelectricity near 60K due to magnetoelectric coupling induced by short-range…

Strongly Correlated Electrons · Physics 2015-06-22 Tathamay Basu , Kiran Singh , N. Mohapatra , E. V. Sampathkumaran

We report the magnetic, heat-capacity, dielectric and magnetodielectric (MDE) behaviour of a Haldane spin-chain compound containing light rare-earth ion, Nd2BaNiO5, in detail, as a function of temperature (T) and magnetic field (H) down to…

Materials Science · Physics 2015-03-12 Tathamay Basu , Niharika Mohapatra , Kiran Singh , E. V. Sampathkumaran

The Haldane spin-chain (S=1) insulating compound, Sm2BaNiO5, which has been proposed to order antiferromagnetically around (T_N=) 55 K, was investigated for its complex dielectric permittivity, magnetodielectric and pyrocurrent behavior as…

Strongly Correlated Electrons · Physics 2017-08-30 Sanjay Kumar Upadhyay , Kartik K Iyer , E. V. Sampathkumaran

We report the results of detailed investigations of magnetization, heat-capacity, dielectric, pyrocurrent, and magneto(di)electric measurements on Tb2BaCoO5, belonging to a hither-to-unexplored spin-chain cobaltates family, R2BaCoO5 (R=…

Strongly Correlated Electrons · Physics 2018-08-01 Sanjay K Upadhyay , E. V. Sampathkumaran

DyMn$_2$O$_5$ is an intriguing multiferroic material showing multiple magnetic, electric and structural transitions. We present here the systematic study on the effect of Sr doping at the Dy site of DyMn$_2$O$_5$ through magnetic and…

Strongly Correlated Electrons · Physics 2020-04-22 P. Dutta , M. Das , S. Mukherjee , S. Chatterjee , S. Giri , S. Majumdar

We report that the spin-chain compound Dy2BaNiO5 recently proven to exhibit magnetoelectric coupling below its Neel temperature (T_N) of 58 K, exhibits strong frequency-dependent behavior in ac magnetic susceptibility and complex dielectric…

Strongly Correlated Electrons · Physics 2014-03-18 Tathamay Basu , P. L. Paulose , Kartik K Iyer , Kiran Singh , N. Mohapatra , S. Chowki , Babu Gonde , E. V. Sampathkumaran

We report the results of various measurements, namely magnetization, complex dielectric permittivity and electric polarization (P) on Dy2BaNiO5 as a function of temperature (T) and magnetic-field (H), apart from heat-capacity (C), with the…

Materials Science · Physics 2015-06-15 Kiran Singh , Tathamay Basu , S. Chowki , N. Mahapotra , K. Iyer , P. L. Paulose , E. V. Sampathkumaran

Superconductivity with a remarkably high $T_c$ has recently been found in Sr-doped NdNiO$_2$ thin films. While this system bears strong similarities to the cuprates, some differences, such as a weaker antiferromagnetic exchange coupling and…

Strongly Correlated Electrons · Physics 2020-01-15 Philipp Werner , Shintaro Hoshino

Observation of ferroelectricity among non-d0 systems, which was believed for a long time an unrealistic concept, led to various proposals for the mechanisms to explain the same (i.e. magnetically induced ferroelectricity) during last…

The effect of electron doping by trivalent charge state rare-earth ion (RE = La, Ce, Pr, and Nd) substitutions on the superconductivity in BaFe2As2 was examined using epitaxial films. Each of the RE substitutions suppressed the resistivity…

Superconductivity · Physics 2013-07-10 Takayoshi Katase , Hidenori Hiramatsu , Toshio Kamiya , Hideo Hosono

In this work, we report the growth and functional characterizations of multiferroic TbMnO3 thin films grown on Nb-doped SrTiO3 (001) substrates using pulsed laser deposition. By performing detailed magnetic and ferroelectric properties…

Materials Science · Physics 2015-12-16 Ni Hu , Chengliang Lu , Zhengcai Xia , Rui Xiong , Pengfei Fang , Jing Shi , Jun-Ming Liu

BaFe2As2 is the parent compound of the '122' iron arsenide superconductors and crystallizes with the tetragonal ThCr2Si2 type structure, space group I4/mmm. A spin density wave transition at 140 K is accompanied by a symmetry reduction to…

Superconductivity · Physics 2015-05-13 Dirk Johrendt , Rainer Poettgen

We report a neutron diffraction study of the multiferroic mechanism in (ND4)2FeCl5D2O, a molecular compound that exhibits magnetically induced ferroelectricity. This material exhibits two successive magnetic transitions on cooling: a…

We report NdCrTiO5 to be an unusual multiferroic material with large magnetic field dependent electric polarization. While magneto-electric coupling in this two magnetic sub-lattice oxide is well established, the purpose of this study is to…

Materials Science · Physics 2015-06-17 J. Saha , G. Sharma , S. Patnaik
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