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Electrochemical devices often consist of multicomponent electrolyte solutions. Two processes influence the overall dynamics of these devices: the formation of electrical double layers and chemical conversion due to redox reactions. However,…

Chemical Physics · Physics 2022-06-20 Nathan Jarvey , Filipe Henrique , Ankur Gupta

We solve the nonlinear Poisson-Boltzmann equation for two parallel and likely charged plates both inside a symmetric elecrolyte, and inside a 2 : 1 asymmetric electrolyte, in terms of Weierstrass elliptic functions. From these solutions we…

Classical Physics · Physics 2013-05-29 Xiangjun Xing

We perform a linearization of the Poisson-Boltzmann (PB) density functional for spherical Wigner-Seitz cells that yields Debye-H\"uckel-like equations agreeing asymptotically with the PB results in the weak-coupling (high-temperature)…

Soft Condensed Matter · Physics 2009-11-07 M. N. Tamashiro , H. Schiessel

Exceptional points (EPs) are special spectral degeneracies of non-Hermitian operators: at the EP, the complex eigenvalues coalesce, i.e., they become degenerate in both their real and imaginary parts. In two-dimensional (2D) photonic…

Optics · Physics 2025-06-17 Luigi Frau , Simone Zanotti , Lydie Ferrier , Dario Gerace , Hai Son Nguyen

A major challenge in the molecular simulation of electric double layer capacitors (EDLCs) is the choice of an appropriate model for the electrode. Typically, in such simulations the electrode surface is modeled using a uniform fixed charge…

Computational Physics · Physics 2015-06-22 Zhenxing Wang , Yang Yang , David L. Olmsted , Mark Asta , Brian B. Laird

We present a series of three-dimensional discrete Boltzmann (DB) models for compressible flows in and out of equilibrium. The key formulating technique is the construction of discrete equilibrium distribution function through inversely…

Fluid Dynamics · Physics 2018-03-06 Yanbiao Gan , Aiguo Xu , Guangcai Zhang , Huilin Lai

The radiolysis of water is an important study in microdosimetry, one of the resulting and important molecules in this study is the $OH^-$. Theoretical quantum mechanics calculations are used to obtain the differential cross section for the…

Chemical Physics · Physics 2023-09-28 C. H. Zepeda Fernández , U. Reyes Ortega , F. Magaña Ibañez , E. Moreno Barbosa

Polymeric ionic liquids are emerging polyelectrolyte materials for modern electrochemical applications. In this paper, we propose a self-consistent field theory of the polymeric ionic liquid on a charged conductive electrode. Taking into…

Soft Condensed Matter · Physics 2022-02-02 Yury A. Budkov , Nikolai N. Kalikin , Andrei L. Kolesnikov

We present the open source distributed software package Poisson-Boltzmann Analytical Method (PB-AM), a fully analytical solution to the linearized Poisson Boltzmann equation, for molecules represented as non-overlapping spherical cavities.…

Biomolecules · Quantitative Biology 2016-09-27 Lisa E. Feldberg , David H. Brookes , Eng-Hui Yap , Elizabeth Jurrus , Nathan Baker , Teresa Head-Gordon

Particle-vortex duality is a powerful theoretical tool that has been used to study bosonic systems. Here we propose an analogous duality for Dirac fermions in 2+1 dimensions. The physics of a single Dirac cone is proposed to be described by…

Strongly Correlated Electrons · Physics 2016-07-06 Max A. Metlitski , Ashvin Vishwanath

Large-scale relativistic calculations are performed for the transition energy and line strength of the $ 1s^{2} 2s 2p$ $^1P_{1} \,-\ 1s^{2} 2s^{2}$ $^1S_{0} $ transition in Be-like carbon. Based on the multiconfiguration…

A general relation is derived between the linear and second-order nonlinear ac conductivities of an electron system in the hydrodynamic regime of frequencies below the interparticle scattering rate. The magnitude and tensorial structure of…

Other Condensed Matter · Physics 2018-03-20 Zhiyuan Sun , D. N. Basov , M. M. Fogler

This paper provides a para-differential calculus toolbox on compact Lie groups and homogeneous spaces. It helps to understand non-local, nonlinear partial differential operators with low regularity on manifolds with high symmetry. In…

Analysis of PDEs · Mathematics 2023-10-11 Chengyang Shao

The magnetic-dipole transition probabilities between the fine-structure levels (1s^2 2s^2 2p) ^2P_1/2 - ^2P_3/2 for B-like ions and (1s^2 2s 2p) ^3P_1 - ^3P_2 for Be-like ions are calculated. The configuration-interaction method in the…

There have been discussions in the recent literature regarding the accuracy of the available electron impact excitation rates (equivalently effective collision strengths $\Upsilon$) for transitions in Be-like ions. In the present paper we…

Atomic Physics · Physics 2016-09-07 K. M. Aggarwal , F. P. Keenan , K. D. Lawson

The Buckley-Leverett equation for two phase flow in a porous medium is modified by including a dependence of capillary pressure on the rate of change of saturation. This model, due to Gray and Hassanizadeh, results in a nonlinear…

Analysis of PDEs · Mathematics 2011-09-06 K. Spayd , M. Shearer

Temperature gradients drive asymmetric ion distributions via thermodiffusion (the Soret effect), leading to deviations from the classical Debye--H\"uckel potential.We introduce the Eastman entropy of transfer, $\hat{S}_\pm = \alpha_\pm…

Soft Condensed Matter · Physics 2026-03-24 Kazuhiko Seki

The Linearized Poisson--Boltzmann (LPB) equation is a popular and widely accepted model for accounting solvent effects in computational (bio-) chemistry. In the present article we derive the analytical forces of the…

Numerical Analysis · Mathematics 2023-09-14 Abhinav Jha , Michele Nottoli , Aleksandr Mikhalev , Chaoyu Quan , Benjamin Stamm

In this paper we present a full discretization of the layer potentials and boundary integral operators for the elastic wave equation on a parametrizable smooth closed curve in the plane. The method can be understood as a non-conforming…

Numerical Analysis · Mathematics 2025-07-08 Victor Dominguez , Tonatiuh Sanchez-Vizuet , Francisco-Javier Sayas

Understanding ion relaxation dynamics in overlapping electric double layers (EDLs) is critical for the development of efficient nanotechnology based electrochemical energy storage, electrochemomechanical energy conversion and…

Chemical Physics · Physics 2014-11-04 Vaibhav Thakore , James J. Hickman