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The temperature-dependent optical response of excitons in semiconductors is controlled by the exciton-phonon interaction. When the exciton-lattice coupling is weak, the excitonic line has a Lorentzian profile resulting from motional…

Materials Science · Physics 2017-05-31 T. Q. P. Vuong , G. Cassabois , P. Valvin , S. Liu , J. H. Edgar , B. Gil

Reflectance and magneto-reflectance experiments together with theoretical modelling based on the $\mathbf{k\cdot p}$ approach have been employed to study the evolution of direct bandgap excitons in MoS$_2$ layers with a thickness ranging…

Mesoscale and Nanoscale Physics · Physics 2019-03-01 A. O. Slobodeniuk , Ł. Bala , M. Koperski , M. R. Molas , P. Kossacki , K. Nogajewski , M. Bartos , K. Watanabe , T. Taniguchi , C. Faugeras , M. Potemski

The coupling between lattice vibration quanta and valence electrons can induce charge density modulations and decisively influence the transport properties of materials, e.g. leading to conventional superconductivity. In high critical…

Two-dimensional (2D) semiconductors are promising candidates for optoelectronic application and quantum information processes due to their inherent out-of-plane 2D confinement. In addition, they offer the possibility of achieving…

Optical excitation of chiral phonons plays a vital role in studying the phonon-driven magnetic phenomena in solids. Transition metal dichalcogenides host chiral phonons at high symmetry points of the Brillouin zone, providing an ideal…

We present a transient absorption setup combining broadband detection over the visible-UV range with high temporal resolution ($\sim$20fs) which is ideally suited to trigger and detect vibrational coherences in different classes of…

The temperature-dependent linewidths of excitons in ZnO quantum wells were studied by measuring absorption spectra from 5 K to room temperature. We deduced experimentally the exciton-longitudinal-optical (LO) phonon coupling strength, which…

Materials Science · Physics 2015-06-25 T. Makino , Y. Segawa , M. Kawasaki

We study the neutral exciton energy spectrum fine structure and its spin dephasing in transition metal dichalcogenides such as MoS$_2$. The interaction of the mechanical exciton with its macroscopic longitudinal electric field is taken into…

Mesoscale and Nanoscale Physics · Physics 2014-05-15 M. M. Glazov , T. Amand , X. Marie , D. Lagarde , L. Bouet , B. Urbaszek

Single-walled carbon nanotubes (SWCNTs) are quasi-one-dimensional systems with poor Coulomb screening and enhanced electron-phonon interaction, and are good candidates for excitons and exciton-phonon couplings in metallic state. Here we…

Materials Science · Physics 2009-04-20 Hualing Zeng , Hongbo Zhao , Fu-Chun Zhang , Xiaodong Cui

Polariton-based devices require materials where light-matter coupling under ambient conditions exceeds losses, but our current selection of such materials is limited. Here we measured the dispersion of polaritons formed by the $A$ and $B$…

Materials Science · Physics 2021-06-16 Patryk Kusch , Niclas S. Mueller , Martin T. Hartmann , Stephanie Reich

Despite the weak, van-der-Waals interlayer coupling, photoinduced charge transfer vertically across atomically thin interfaces can occur within surprisingly fast, sub-50fs timescales. Early theoretical understanding of the charge transfer…

We find that the optical properties of carbon nanotubes reflect remarkably strong effects of exciton-phonon coupling. Tight-binding calculations show that a significant fraction of the spectral weight of the absorption peak is transferred…

Materials Science · Physics 2009-11-10 Vasili Perebeinos , J. Tersoff , Phaedon Avouris

Due to a strong Coulomb interaction, excitons dominate the excitation kinetics in 2D materials. While Coulomb-scattering between electrons has been well studied, the interaction of excitons is more challenging and remains to be explored. As…

Materials Science · Physics 2021-01-27 Daniel Erkensten , Samuel Brem , Ermin Malic

In this letter we report measurements of the coupling between Dirac fermion quasiparticles (DFQs) and phonons on the (001) surface of the strong topological insulator Bi2Se3. While most contemporary investigations of this coupling have…

Materials Science · Physics 2012-05-07 Xuetao Zhu , Luiz Santos , Colin Howard , R. Sankar , Fangcheng Chou , Claudio Chamon , Michael El-Batanouny

The coupling between spin, charge, and lattice degrees of freedom plays an important role in a wide range of fundamental phenomena. Monolayer semiconducting transitional metal dichalcogenides have emerged as an outstanding platform for…

We present the micro-photoluminescence ($\mu$PL) and micro-reflectance contrast spectroscopy studies on thin films of MoSe2 with layer thicknesses ranging from a monolayer (1L) up to 5L. The thickness dependent evolution of the ground and…

Mesoscale and Nanoscale Physics · Physics 2016-01-20 Ashish Arora , Karol Nogajewski , Maciej R. Molas , Maciej Koperski , Marek Potemski

We examine a mechanism by which excitons are generated via the LO (longitudinal optical) phonon-assisted scattering process after optical excitation of monolayer transition metal dichalcogenides. The exciton formation time is computed as a…

Materials Science · Physics 2016-10-12 A. Thilagam

Monolayer transition metal dichalcogenides, known for exhibiting strong excitonic resonances, constitute a very interesting and versatile platform for investigation of light-matter interactions. In this work we report on a strong coupling…

Mesoscale and Nanoscale Physics · Physics 2019-05-20 M. Król , K. Lekenta , R. Mirek , K. Łempicka , D. Stephan , K. Nogajewski , M. R. Molas , A. Babiński , M. Potemski , J. Szczytko , B. Piętka

The concept of \textit{optical} exciton - a photo-excited bound electron-hole pair within a crystal - is routinely used to interpret and model a wealth of excited-state phenomena in semiconductors. Beside originating sub-band gap signatures…

Materials Science · Physics 2022-09-21 Fulvio Paleari , Andrea Marini

Group-VI monochalcogenides are attracting a great deal of attention due to their peculiar anisotropic properties. Very recently, it has been suggested that GeS could act as a promissory absorbing material with high input-output ratios,…

Materials Science · Physics 2017-04-20 Cesar E. P. Villegas , A. R. Rocha , A. Marini
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