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Paired electrolysis at industrial current densities offers an energy-efficient and sustainable alternative to thermocatalytic chemical synthesis by leveraging anodic and cathodic valorization. However, its industrial feasibility remains…

Electrochemical CO2 reduction (CO2R) offers a promising approach to decarbonize chemical manufacturing through production of carbon-neutral fuels. However, insufficient performance and instability of membrane electrode assembly (MEA)…

The conversion of waste carbon dioxide (CO2) gas into valuable products and fuels through an electrocatalytic CO2 reduction reaction (CO2RR) is a promising approach. The sluggish kinetics of the CO2RR require the development of novel…

Materials Science · Physics 2024-04-16 Lokesh Yadav , Srimanta Pakhira

The catalytic activities of high-spin small Fe(III) oxides have been investigated for efficient hydrogen production through ammonia decomposition, using the Artificial Force Induced Reaction (AFIR) method within the framework of density…

Atomic and Molecular Clusters · Physics 2024-10-01 Sapajan Ibragimov , Andrey Lyalin , Sonu Kumar , Yuriko Ono , Tetsuya Taketsugu , Maciej Bobrowski

The search for earth abundant, efficient and stable electrocatalysts that can enable the chemical reduction of CO2 to value-added chemicals and fuels at an industrially relevant scale, is a high priority for the development of a global…

We have used a combination of density functional theory (DFT) and kinetic Monte Carlo (KMC) simulations to calculate the reaction rates for the selective oxidation of ammonia on RuO2(110). We find that the overall energy barrier for NH3 + O…

Mesoscale and Nanoscale Physics · Physics 2010-07-15 Sampyo Hong , Altaf Karim , Talat S. Rahman , Karl Jacobi , Gerhard Ertl

Recent advances in Neural Radiance Fields (NeRF) have demonstrated significant potential for representing 3D scene appearances as implicit neural networks, enabling the synthesis of high-fidelity novel views. However, the lengthy training…

Computer Vision and Pattern Recognition · Computer Science 2023-10-04 Tong Wang , Shuichi Kurabayashi

The development of high-activity and low-price cathodic catalysts to facilitate the electrochemical sluggish O$_2$ reduction reaction (ORR) is very important to achieve the commercial application of fuel cells. Here, we have investigated…

Materials Science · Physics 2023-07-14 Ashok Singh , Srimanta Pakhira

The oxygen reduction reaction (ORR) plays a pivotal role in clean energy generation and sustainable chemical production, particularly in the synthesis of hydrogen peroxide (H\textsubscript{2}O\textsubscript{2}). In this study,…

Photocatalytic nitrogen fixation provides a promising route to produce reactive nitrogen compounds at benign conditions. Titania has been reported as an active photocatalyst for reduction of dinitrogen to ammonia; however there is little…

Chemical Physics · Physics 2018-02-01 Benjamin M. Comer , Andrew J. Medford

Electrocatalyst surfaces continuously reorganize on the timescale of catalytic turnover, obscuring the identification of active sites under operando conditions and hindering rational catalyst design. Here, we resolve the operando Cu(111)…

Materials Science · Physics 2025-11-14 Xue-Chun Jiang , Jia-Lan Chen , Wei-Xue Li , Jin-Xun Liu

We construct a fast, transferable, general purpose, machine-learning interatomic potential suitable for large-scale simulations of $N_2$. The potential is trained only on high quality quantum chemical molecule-molecule interactions, no…

Computational Physics · Physics 2024-05-10 Marcin Kirsz , Ciprian G. Pruteanu , Peter I. C. Cooke , Graeme J. Ackland

Altermagnets can replace ferromagnets in tunnel junctions, yielding large tunneling magnetoresistance, ultrafast switching, and low-power functionality. While most studies explore the linear-response regime, interesting features emerge at…

Mesoscale and Nanoscale Physics · Physics 2026-05-14 Sajjan Sheoran , Luke Keenan , Declan Nell , Stefano Sanvito

Background: The nuclear interaction potential and hence the fusion barrier formed between the interacting nuclei are the keys to understanding the complex fusion process dynamics. Purpose: This work intends to explore the fusion barrier…

Nuclear Theory · Physics 2022-05-31 Shilpa Rana , Mrutunjaya Bhuyan , Raj Kumar

Photoelectrocatalytic (PEC) reduction of N2 to ammonia (NH3) is emerging as the potential alternative to overcome the standard Haber-Bosch approach. In this communication, solar N2 reduction was demonstrated with molybdenum carbide (Mo2C)…

Relativistic corrections have been made in the non-relativistic antisymmetrized molecular dynamics (AMD) simulations to apply to the high energy neutron production in the $^{12}$C+$^{12}$C and $^{16}$O+$^{12}$C collisions at incident…

Nuclear Theory · Physics 2023-10-13 Q. Hu , G. Y. Tian , R. Wada , X. Q. Liu , W. P. Lin , H. Zheng , Y. P. Zhang , Z. Q. Chen , R. Han , M. R. Huang

Significant efforts have been committed to understanding the fundamental combustion chemistry of ammonia at high-pressure and low-temperature conditions with or without blending with other fuels, as these are promising to improve ammonia…

Chemical Physics · Physics 2024-10-03 Mingrui Wang , Ruoyue Tang , Xinrui Ren , Hongqing Wu , Yuxin Dong , Ting Zhang , Song Cheng

Here we develop a class off face centred cubic structure of metallic silver nanocrystals, to enable high ORR activity process. Silver nanoparticles deposited within different carbon supports: carboxylated-graphene, SiO2-doted reduced-…

The electrocatalytic CO2 reduction reaction (CO2RR) is a complex multi-proton-electron transfer process that generates a vast network of reaction intermediates. Accurate prediction of free energy changes (G) of these intermediates and…

Chemical Physics · Physics 2025-04-23 Xuxin Kang , Wenjing Zhou , Ziyuan Li , Zhaoqin Chu , Hanqin Yin , Shan Gao , Aijun Du , Xiangmei Duan

Developing efficient electrocatalysts for CO$_2$ reduction into value-added products is crucial for the green economy. Inspired by the recent synthesis of Biphenylene (BPH), we have systematically investigated pristine, defective, and…

Materials Science · Physics 2024-10-28 Radha N Somaiya , Muhammad Sajjad , Nirpendra Singh , Aftab Alam