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Frustrated magnetism in the pyrochlore lattice magnet has proven to be a most fruitful setting for the experimental and theoretical search for spin liquids. Besides the canonical case of spin ice, recent works have identified a variety of…

Strongly Correlated Electrons · Physics 2025-04-03 Daniel Lozano-Gómez , Owen Benton , Michel J. P. Gingras , Han Yan

The centred pyrochlore lattice is a novel geometrically frustrated lattice, realized in the metal-organic framework Mn(ta)$_2$ (arXiv:2203.08780) where the basic unit of spins is a five site centred tetrahedron. Here, we present an in-depth…

Strongly Correlated Electrons · Physics 2023-07-26 Rajah P. Nutakki , Ludovic D. C. Jaubert , Lode Pollet

Synthesis and crystal structures are described for the compounds Ln2(Ti2-xLnx)O7-x/2, where Ln = Tb, Dy, Ho, Er, Tm, Yb, Lu, and x ranges from 0 to 0.67. Rietveld refinements on X-ray powder diffraction data indicate that in Tb and Dy…

Strongly Correlated Electrons · Physics 2009-08-11 G. C. Lau , B. D. Muegge , T. M. McQueen , E. L. Duncan , R. J. Cava

We report the growth of large high quality crystals of the frustrated magnet, Pr2Zr2O7 by the floating zone technique. Several crystals have been produced starting with varying levels of excess of Pr6O11 to compensate for the loss of Pr2O3…

Materials Science · Physics 2016-11-09 M. Ciomaga Hatnean , C. Decorse , M. R. Lees , O. A. Petrenko , D. S. Keeble , G. Balakrishnan

When magnetic moments (spins) are regularly arranged in a geometry of a triangular motif, the spins may not satisfy simultaneously their interactions with their neighbors. This phenomenon, called frustration, leads to numerous energetically…

Statistical Mechanics · Physics 2015-06-17 I. Klich , S. -H. Lee , K. Iida

Frustrated magnets are one class of fascinating materials that host many intriguing phases such as spin ice, spin liquid and complex long-range magnetic orderings at low temperatures. In this work we use first-principles calculations to…

Materials Science · Physics 2019-08-07 Yue-Wen Fang , Ruihan Yang , Hanghui Chen

The recent synthesis of the chromium selenide compound LiCrSe$_2$ constitutes a valuable addition to the ensemble of two-dimensional triangular lattice antiferromagnets (2D-TLA). In this work we present the very first comprehensive study of…

We report a comprehensive study on the magnetic and structural properties of the spinel sulfides LiInCr4S8, LiGaCr4S8, and CuInCr4S8, where Li+/Cu+ and Ga3+/In3+ ions form a zinc-blende-type order. On the basis of synchrotron X-ray…

In recent years, solid state magnetic cooling based on magnetocaloric effect (MCE) have drawn attention worldwide as a promising alternative potential candidate to the conventional gas compression-expansion cooling technique. In this…

Materials Science · Physics 2024-10-23 Vinod Kumar Dwivedi

We have successfully synthesized single crystals, solved the crystal structure, and studied the magnetic properties of a new family of copper halides (C$_4$H$_{14}$N$_2$)Cu$_2X_6$ ($X$= Cl, Br). These compounds crystallize in an…

Materials Science · Physics 2023-06-28 P. Biswal , S. Guchhait , S. Ghosh , S. N. Sarangi , D. Samal , Diptikant Swain , Manoranjan Kumar , R. Nath

We have performed magnetic susceptibility, heat capacity, muon spin relaxation, and neutron scattering measurements on three members of the family Ba3MRu2O9, where M = In, Y and Lu. These systems consist of mixed-valence Ru dimers on a…

Strongly Correlated Electrons · Physics 2017-05-31 D. Ziat , A. A. Aczel , R. Sinclair , Q. Chen , H. D. Zhou , T. J. Williams , M. B. Stone , A. Verrier , J. A. Quilliam

Structural and magnetic properties of a two-dimensional spin-$\frac{5}{2}$ frustrated triangular lattice antiferromagnet NH$_{4}$Fe(PO$_{3}$F)$_2$ are explored via x-ray diffraction, magnetic susceptibility, high-field magnetization, heat…

Materials Science · Physics 2025-02-11 S. Mohanty , K. M. Ranjith , C. S. Saramgi , Y. Skourski , B. Büchner , H. -J. Grafe , R. Nath

We have experimentally identified a new magnetic ground state for the kagome lattice, in the perfectly hexagonal Fe2+ (3d6, S = 2) compound Fe4Si2Sn7O16. Representational symmetry analysis of neutron diffraction data shows that below T_N =…

Strongly Correlated Electrons · Physics 2017-11-22 C. D. Ling , M. C. Allison , S. Schmid , M. Adveev , J. S. Gardner , C. -W. Wang , D. H. Ryan , M. Zbiri , T. Soehnel

We study the influence of the spin lattice distortion on the properties of frustrated magnetic systems and consider the applicability of the spin-1/2 frustrated square lattice model to materials lacking tetragonal symmetry. We focus on the…

Strongly Correlated Electrons · Physics 2009-06-16 Alexander A. Tsirlin , Helge Rosner

The Yb based triangular lattice delafossites $A$Yb$X_2$ ($A$ = alkali metal, $X$ = O, S, Se) have recently been studied as quantum spin liquid candidates. We report the synthesis of powders and single crystals of CuYbSe$_2$ with a perfect…

Strongly Correlated Electrons · Physics 2025-09-23 Barkha Khattar , Anzar Ali , Masahiko Isobe , Yogesh Singh

The gadolinium pyrochlores, Gd$_2B_2$O$_7$, are amongst the best realizations of antiferromagnetically coupled Heisenberg spins on a pyrochlore lattice. We present a magnetic characterization of Gd$_2$Pt$_2$O$_7$, a unique member of this…

Strongly Correlated Electrons · Physics 2016-10-18 A. M. Hallas , A. Z. Sharma , Y. Cai , T. J. Munsie , M. N. Wilson , M. Tachibana , C. R. Wiebe , G. M. Luke

Quantum-disordered magnetic ground states are challenging to identify in three-dimensional (3D) oxides, where strong exchange pathways typically favour long-range magnetic order or spin freezing. The quadruple perovskite…

Strongly Correlated Electrons · Physics 2026-05-11 J. Ming , Abhisek Bandyopadhyay , G. B. G. Stenning , M. T. F. Telling , N. N. Wang , G. Wang , J. -G. Cheng , D. T. Adroja

Magnetic frustration in two-dimensional spin lattices with triangular motifs underpins a series of exotic states, ranging from multi-Q configurations to disordered spin-glasses. The antiferromagnetic kagome lattice, characterized by its…

The (three-dimensional) pyrochlore lattice antiferromagnet with Heisenberg spins of large spin length $S$ is a highly frustrated model with an macroscopic degeneracy of classical ground states. The zero-point energy of (harmonic order) spin…

Strongly Correlated Electrons · Physics 2009-11-11 Christopher L. Henley

Spin-1/2 antiferromagnetic triangular lattice models are paradigms of geometrical frustration, revealing very different ground states and quantum effects depending on the nature of anisotropies in the model. Due to strong spin orbit…