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For a deeply supercooled liquid just above its glass transition temperature, we present a simple thermodynamic model, where the deeply supercooled liquid is assumed to be a mixture of solid-like and liquid-like micro regions. The mole…

Statistical Mechanics · Physics 2012-10-17 Hiroshi Matsuoka

We present here a numerical study of a lattice model of a chiral liquid. The low symmetry of the favoured local structure depresses the freezing point to reveal an exotic liquid-liquid transition characterised by the appearance of an…

Soft Condensed Matter · Physics 2013-08-27 Pierre Ronceray , Peter Harrowell

Below the melting temperature $T_m$ crystals are the stable phase of typical elemental or molecular systems. However, cooling down a liquid below $T_m$, crystallization is anything but inevitable. The liquid can be supercooled, eventually…

Disordered Systems and Neural Networks · Physics 2017-03-07 M. Zanatta , L. Cormier , L. Hennet , C. Petrillo , F. Sacchetti

Pure liquids in thermodynamic equilibrium are structurally homogeneous. In liquid crystals, flow and light pulses are used to create reconfigurable domains with polar order. Moreover, through careful engineering of concerted microfluidic…

Soft Condensed Matter · Physics 2020-01-03 Tadej Emeršič , Rui Zhang , Žiga Kos , Simon Čopar , Natan Osterman , Juan J. de Pablo , Uroš Tkalec

Amorphous solids, or glasses, are distinguished from crystalline solids by their lack of long-range structural order. At the level of two-body structural correlations, glassformers show no qualitative change upon vitrifying from a…

Soft Condensed Matter · Physics 2015-06-11 C. Patrick Royall , Stephen R. Williams

A novel supersolid phase is predicted for an ensemble of Rydberg atoms in the dipole-blockade regime, interacting via a repulsive dipolar potential "softened" at short distances. Using exact numerical techniques, we study the low…

Quantum Gases · Physics 2010-09-23 F. Cinti , P. Jain , M. Boninsegni , A. Micheli , P. Zoller , G. Pupillo

A statistical analysis of the geometries of particle trajectories in the supercooled liquid state is reported. We examine two structurally different fragile glass-forming liquids simulated by molecular dynamics. In both liquids, the…

Soft Condensed Matter · Physics 2008-11-19 Tomas Oppelstrup , Mikhail Dzugutov

Disordered systems like liquids, gels, glasses, or granular materials are not only ubiquitous in daily life and in industrial applications but they are also crucial for the mechanical stability of cells or the transport of chemical and…

Disordered Systems and Neural Networks · Physics 2019-04-30 Zhen Zhang , Walter Kob

We present a review on the study of metastable silicon, primarily focusing mainly on the aspects of liquid-liquid transition, critical point and phase behaviour, structural and dynamic properties of liquid phase as well as crystal…

Materials Science · Physics 2021-09-01 Vishwas V. Vasisht , Srikanth Sastry

The glass transition remains one of the great unsolved mysteries of contemporary condensed matter physics. When crystallization is bypassed by rapid cooling, a supercooled liquid, retaining amorphous particle arrangment, results. The…

Materials Science · Physics 2016-10-12 Nicholas B. Weingartner , Zohar Nussinov

Glasses obtained from vapor deposition on a cold substrate have superior thermodynamic and kinetic stability with respect to ordinary glasses. Here we perform molecular dynamics simulations of vapor deposition of a model glass-former and…

Soft Condensed Matter · Physics 2023-05-24 Fabio Leoni , Fausto Martelli , C. Patrick Royall , John Russo

The atomic structure of the supercooled liquid has often been discussed as a key source of glass formation in metals. The presence of icosahedrally-coordinated clusters and their tendency to form networks have been identified as one…

Materials Science · Physics 2013-10-30 Logan Ward , Dan Miracle , Wolfgang Windl , Oleg Senkov , Katharine Flores

We find that the hierarchical organization of the potential energy landscape in a model supercooled liquid can be related to a change in the spatial distribution of soft normal modes. For groups of nearby minima, between which fast…

Disordered Systems and Neural Networks · Physics 2014-03-17 Majid Mosayebi , Patrick Ilg , Asaph Widmer-Cooper , Emanuela Del Gado

While deeply supercooled liquids exhibit divergent viscosity and increasingly heterogeneous dynamics as the temperature drops, their structure shows only seemingly marginal changes. Understanding the nature of relaxation processes in this…

Materials Science · Physics 2022-11-03 Matthias Lerbinger , Armand Barbot , Damien Vandembroucq , Sylvain Patinet

Crystal growth and crystal coalescence processes in supercooled systems strongly depend on the concentration of crystallization centers. We perform atomistic dynamics simulations of the crystallization process in the ultrathin metallic film…

Materials Science · Physics 2019-09-04 Bulat N. Galimzyanov , Vladimir I. Ladyanov , Anatolii V. Mokshin

Crystal structure and physical properties of the novel BiS2-based layered superconductors are briefly reviewed. Superconductivity in the BiS2-based layered compounds is induced by electron doping into the BiS2 conduction layers. The…

Superconductivity · Physics 2015-04-06 Yoshikazu Mizuguchi

The precipitation of a glass forming solute from solution is modelled using a lattice model previously introduced to study dissolution kinetics of amorphous materials. The model includes the enhancement of kinetics at the surface of a glass…

Soft Condensed Matter · Physics 2019-05-15 Ian Douglass , Peter Harrowell

Temperature-driven polyamorphism has been reported in various supercooled liquids and glasses. The dynamical and structural routes followed by the system during such crossovers are however not universal and appear to be related to intrinsic…

Disordered Systems and Neural Networks · Physics 2018-08-29 S. Hechler , B. Ruta , M. Stolpe , E. Pineda , Z. Evenson , O. Gross , W. Hembree , A. Bernasconi , R. Busch , I. Gallino

We investigate the phase behavior of a single-component system in 3 dimensions with spherically-symmetric, pairwise-additive, soft-core interactions with an attractive well at a long distance, a repulsive soft-core shoulder at an…

Soft Condensed Matter · Physics 2009-11-07 G. Franzese , G. Malescio , A. Skibinsky , S. V. Buldyrev , H. E. Stanley

The formation of chain-folded structures from the melt is observed in molecular dynamics simulations resembling the lamellae of polymer crystals. Crystallization and subsequent melting temperatures are related linearly to the inverse…

Soft Condensed Matter · Physics 2009-10-31 Hendrik Meyer , Florian Mueller-Plathe