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Recent advancements in ultrashort and intense X-ray sources have enabled the utilisation of resonant inelastic X-ray scattering (RIXS) as a probing technique for monitoring photoinduced dynamics in molecular systems. To account for dynamic…

Chemical Physics · Physics 2024-03-19 Antonia Freibert , David Mendive-Tapia , Oriol Vendrell , Nils Huse

Resonant inelastic X-ray scattering (RIXS) detects various types of high- and low-energy elementary excitations in correlated solids, and this tool will play an increasingly important role in investigations of time-dependent phenomena in…

Strongly Correlated Electrons · Physics 2021-12-21 Philipp Werner , Steven Johnston , Martin Eckstein

While new light sources allow for unprecedented resolution in experiments with X-rays, a theoretical understanding of the scattering cross-section is lacking. In the particular case of strongly correlated electron systems, numerical…

Strongly Correlated Electrons · Physics 2023-05-29 Krissia Zawadzki , Alberto Nocera , Adrian E. Feiguin

Time-resolved measurements of materials provide a wealth of information on quasiparticle dynamics, and have been the focus of optical studies for decades. In this paper, we develop a theory for explicitly evaluating time-resolved resonant…

Strongly Correlated Electrons · Physics 2019-03-27 Yuan Chen , Yao Wang , Chunjing Jia , Brian Moritz , Andrij M. Shvaika , James K. Freericks , Thomas P. Devereaux

We present a computational study of $L$-edge resonant inelastic x-ray scattering (RIXS) in correlated 3$d$ transition-metal oxides using an $ab$ $initio$ method based on local density approximation + dynamical mean-field theory (DMFT). The…

Strongly Correlated Electrons · Physics 2020-03-25 Atsushi Hariki , Mathias Winder , Takayuki Uozumi , Jan Kuneš

In the past decade, Resonant Inelastic X-ray Scattering (RIXS) has made remarkable progress as a spectroscopic technique. This is a direct result of the availability of high-brilliance synchrotron X-ray radiation sources and of advanced…

Strongly Correlated Electrons · Physics 2012-12-03 Luuk J. P. Ament , Michel van Veenendaal , Thomas P. Devereaux , John P. Hill , Jeroen van den Brink

Recent experiments show that indirect resonant inelastic X-ray scattering (RIXS) is a new probe of spin dynamics. Here I derive the cross-section for magnetic RIXS and determine the momentum dependent four-spin correlation function that it…

Strongly Correlated Electrons · Physics 2015-06-25 Jeroen van den Brink

Resonant inelastic x-ray scattering (RIXS) is an extremely valuable tool for the study of elementary, including magnetic, excitations in matter. Latest developments of this technique mostly aimed at improving the energy resolution and…

We develop a formalism for calculating resonant inelastic x-ray scattering (RIXS) spectra in systems of itinerant electrons with arbitrary band structures, accounting for the effect of the positively-charged core hole exactly. We apply this…

Superconductivity · Physics 2013-12-24 David Benjamin , Israel Klich , Eugene Demler

We calculate the resonant inelastic X-ray scattering (RIXS) response in a Mott insulator which is described by the Falicov-Kimball model. The model can be solved exactly within the single site dynamical mean-field theory (DMFT)…

Strongly Correlated Electrons · Physics 2015-03-31 Nandan Pakhira , J. K. Freericks , A. M. Shvaika

Resonant inelastic X-ray scattering (RIXS) spectra of model copper- and nickel-based transition metal oxides are measured over a wide range of energies near the M-edge (h$\nu$=60-80eV) to better understand the properties of resonant…

Strongly Correlated Electrons · Physics 2012-11-20 L. Andrew Wray , Wanli Yang , Hiroshi Eisaki , Zahid Hussain , Yi-De Chuang

The capability to probe the dispersion of elementary spin, charge, orbital, and lattice excitations has positioned resonant inelastic x-ray scattering (RIXS) at the forefront of photon science. Here we develop the scattering theory for RIXS…

Superconductivity · Physics 2015-04-10 Pasquale Marra , Steffen Sykora , Krzysztof Wohlfeld , Jeroen van den Brink

Resonant Inelastic X-ray Scattering (RIXS) in the soft x-ray range is an element-specific energy-loss spectroscopy used to probe the electronic and magnetic excitations in strongly correlated solids. In the recent years, RIXS has been…

We present an ab initio theory of core- and valence resonant inelastic x-ray scattering (RIXS) based on a real-space multiple scattering Green's function formalism and a quasi-boson model Hamiltonian. Simplifying assumptions are made which…

Materials Science · Physics 2011-01-25 J. J. Kas , J. J. Rehr , J. A. Soininen , P. Glatzel

Resonant inelastic x-ray scattering (RIXS) is a well-established tool for studying electronic, nuclear and collective dynamics of excited atoms, molecules and solids. An extension of this powerful method to a time-resolved probe technique…

Chemical Physics · Physics 2015-11-03 Victor Kimberg , Nina Rohringer

We develop a formalism to study the Resonant Inelastic X-ray Scattering (RIXS) response in metals based on the diagrammatic expansion for its cross section. The standard approach to the solution of the RIXS problem relies on two key…

Strongly Correlated Electrons · Physics 2019-11-20 A. M. Tsvelik , R. M. Konik , N. V. Prokof'ev , I. S. Tupitsyn

Resonant inelastic x-ray scattering (RIXS) is a widely used spectroscopic technique, providing access to the electronic structure and dynamics of atoms, molecules, and solids. However, RIXS requires a narrow bandwidth x-ray probe to achieve…

We investigate resonant inelastic X-ray scattering (RIXS) at the O $K$-edge in insulating cuprates by means of three methods: cluster perturbation theory (CPT), Hartree--Fock approximation (HFA) and exact diagonalization (ED) method. We…

Strongly Correlated Electrons · Physics 2023-02-22 Yukihiro Matsubayashi , Sumio Ishihara

Resonant Inelastic X-ray scattering (RIXS) is a synchrotron-based spectroscopy that has seen growing interest across a range of scientific disciplines beyond fundamental physics. The interpretation of experimental RIXS data requires…

Quasi-one-dimensional systems exhibit many-body effects elusive in higher dimensions. A prime example is spin-orbital separation, which has been measured by resonant inelastic X-ray scattering (RIXS) in Sr$_2$CuO$_3$. Here, we theoretically…

Strongly Correlated Electrons · Physics 2022-10-03 Aaron Müller , Francesco Grandi , Martin Eckstein
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