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A long sought-after goal for photocathode electron sources has been to improve performance by temporally shaping the incident exitation laser pulse. The narrow bandwidth, short wavelength, and picosecond pulse duration make it challenging…

We investigate the propagation of a coherent probe light pulse through a three-level atomic medium (in the $\Lambda$--configuration) in the presence of a pump laser under the conditions for gain without inversion. When the carrier frequency…

Quantum Physics · Physics 2007-05-23 Filippo Caruso , Ivan Herrera , Saverio Bartalini , Francesco Cataliotti

We present an experimental technique enabling mechanical-noise free, cavity-enhanced frequency measurements of an atomic transition and its hyperfine structure. We employ the 532nm frequency doubled output from a Nd:YAG laser and an iodine…

Optics · Physics 2009-11-10 Glenn de Vine , David E. McClelland , John D. Close , Malcolm B. Gray

Single-beam super-resolution microscopy, also known as superlinear microscopy, exploits the nonlinear response of fluorescent probes in confocal microscopy. The technique requires no complex purpose-built system, light field modulation, or…

The nonlinear oscillator model is useful to basically understand the most important properties of nonlinear optical processes. It has been shown to give the correct asymptotic behaviour and to provide the general feature of harmonic…

Optics · Physics 2009-10-31 Franco Bassani , Valerio Lucarini

We present an experimental study of the effects of temporal modulation of the pump intensity on a random laser. The nanosecond pump pulses exhibit rapid intensity fluctuations which differ from pulse to pulse. Specific temporal profiles of…

Optics · Physics 2019-01-10 Stefan Bittner , Sebastian Knitter , Seng Fatt Liew , Hui Cao

Fundamental to many applications of laser pulses in science and technology is an extended interaction length with matter that significantly exceeds the distance over which the pulse would normally diffract and transversely spread. At low…

Plasma Physics · Physics 2025-12-10 J. E. Shrock , B. Miao , E. Rockafellow , H. M. Milchberg

Diagnostics capable of interrogating dynamics in harsh environments such as plasma have remained essentially unchanged in recent decades. Developments in advanced microscopy techniques will improve our understanding of the physics involved…

We show how to emulate a conventional pump-probe scheme using a single frequency-chirped ultrashort UV pulse to obtain a time-resolved image of molecular ultrafast dynamics. The chirp introduces a spectral phase in time that encodes the…

Chemical Physics · Physics 2017-05-03 Denis Jelovina , Johannes Feist , Fernando Martín , Alicia Palacios

Ultrafast pump-probe technique is a powerful tool to understand and manipulate properties of materials for designing novel quantum devices. An intense, single cycle terahertz pulse can change the intrinsic properties of semiconductor…

Mesoscale and Nanoscale Physics · Physics 2020-07-13 Chen-Yen Lai , D. A. Yarotski , Jian-Xin Zhu

A method is shown for preventing temporal broadening of ultrafast optical pulses in highly dispersive and fluctuating media for arbitrary signal-pulse profiles. Pulse pairs, consisting of a strong-field control-pulse and a weak-field…

Optics · Physics 2021-11-17 Haider Zia

Coherent spin resonance methods, such as nuclear magnetic resonance and electron spin resonance spectroscopy, have led to spectrally highly sensitive, non-invasive quantum imaging techniques. Here, we propose a pump-probe spin resonance…

Quantum Physics · Physics 2024-12-02 Philipp Haslinger , Stefan Nimmrichter , Dennis Rätzel

We consider the theory of the non-linear spectroscopy for a single molecule undergoing stochastic dynamics and interacting with a sequence of two laser pulses. General expressions for photon counting statistics are obtained, and an exact…

Optics · Physics 2008-01-13 F. Shikerman , E. Barkai

The dynamics triggered by the impact of an ion onto a solid surface has been explored mainly by theoretical modeling or computer simulation to date. Results indicate that the microscopic non-equilibrium relaxation processes triggered by the…

Atomic Physics · Physics 2023-03-03 L. Kalkhoff , A. Golombek , M. Schleberger , K. Sokolowski-Tinten , A. Wucher , L. Breuer

We report a simple method to suppress the light shift in optical pumping systems. This method uses only frequency modulation of a radio frequency or microwave source, which is used to excite an atomic resonance, to simultaneously lock the…

Atomic Physics · Physics 2013-02-19 B. H. McGuyer , Y. -Y. Jau , W. Happer

Specific types of atomic coherences between Zeeman sublevels can be generated and detected using a method based on nonlinear magneto-optical rotation with frequency modulated light. Linearly polarized, frequency modulated light is employed…

In this paper we develop a method capable of modeling the space-time focusing of nondiffracting pulses. The new pulses can possess arbitrary peak velocities and, in addition to being resistant to diffraction, can have their peak intensities…

Optics · Physics 2016-10-19 Michel Zamboni-Rached , Ioannis M. Besieris

Dynamic phase-only beam shaping with a liquid crystal spatial light modulator is a powerful technique for tailoring the beam's intensity profile or wave front. While shaping and controlling the light field is a highly researched topic,…

Lensless imaging is an elegant approach to high-resolution microscopy, which is rapidly gaining popularity in applications where imaging optics are problematic. However, current lensless imaging methods require objects to be placed within a…

Mid-infrared photothermal microscopy is a new chemical imaging technology in which a visible beam senses the photothermal effect induced by a pulsed infrared laser. This technology provides infrared spectroscopic information at sub-micron…

Optics · Physics 2021-04-08 Yi Zhang , Haonan Zong , Cheng Zong , Yuying Tan , Meng Zhang , Yuewei Zhan , Ji-Xin Cheng
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