Related papers: Coherent optical creation of a single molecule
We investigate the stimulated Raman adiabatic passage in two-color photoassociation for a atom-molecule Bose-Einstein condensate. By applying two time-varying Guassian laser pulses that fulfill generalized two-photon resonance condition, we…
Ultracold polar molecules uniquely combine a rich structure of long-lived internal states with access to controllable long-range, anisotropic dipole-dipole interactions. In particular, the rotational states of polar molecules confined in…
Ultracold polar molecules are promising for quantum information processing and searches for physics beyond the Standard Model. Laser cooling to ultracold temperatures is an established technique for trapped diatomic and triatomic molecules.…
Novel optical phenomena, including electromagnetically induced transparency, slow light, superluminal light propagation, have recently been demonstrated in diverse physical implementations. These phenomena are challenging to realize in…
We report on the creation and characterization of heteronuclear KRb Feshbach molecules in an optical dipole trap. Starting from an ultracold gas mixture of K-40 and Rb-87 atoms, we create as many as 25,000 molecules at 300 nK by rf…
We develop an ultrafast frequency-resolved Raman spectroscopy with entangled photons for polyatomic molecules in condensed phases, to probe the electronic and vibrational coherences. Using quantum correlation between the photons, the signal…
We suggest and analyze a novel technique for efficient and robust creation of dense ultracold molecular ensembles in their ground rovibrational state. In our approach a molecule is brought to the ground state through a series of…
In open-shell atoms and ions, processes such as photoionization, combination (Raman) scattering, electron scattering and recombination, are often mediated by many-electron compound resonances. We show that their interference (neglected in…
We propose and demonstrate a novel technique that combines Raman scattering and optical cycling in molecules with diagonal Franck-Condon factors. This resonance Raman optical cycling manipulates molecules to behave like efficient…
The strong coupling of atoms to optical cavities can improve optical lattice clocks as the cavity enables metrologically useful collective atomic entanglement and high-fidelity measurement. To this end, it is necessary to cool the ensemble…
Single-photon coherent optics represents a fundamental importance for the investigation of quantum light-matter interactions. While most work has considered the interaction in the steady-state regime, here we demonstrate that a…
We perform Raman spectroscopy of optically trapped non interacting \Rb atoms, and observe revivals of the atomic coherence at integer multiples of the trap period. The effect of coherence control methods such as echo and dynamical…
We report generation of cascaded rotational Raman scattering up to 58th orders in coherently excited CO_2 molecules. The high-order Raman scattering, which produces a quasiperiodic frequency comb with more than 600 sidebands, is obtained…
We report measurements of superradiant optical transition radiation in the 550-800 nm range produced by ultrashort relativistic electron bunches at a dielectric boundary. In the measured optical spectra, we observe photon production with…
The motion of chemical bonds within molecules can be observed in real time, in the form of vibrational wavepackets prepared and interrogated through ultrafast nonlinear spectroscopy. Such nonlinear optical measurements are commonly…
Two-photon optical transitions combined with long-range dipole-dipole interactions can be used for the coherent manipulation of collective metastable states composed of different atoms. We show that it is possible to induce optical…
We associate Sr atom pairs on sites of a Mott insulator optically and coherently into weakly-bound ground-state molecules, achieving an efficiency above 80\%. This efficiency is 2.5 times higher than in our previous work [S. Stellmer, B.…
Techniques to control the quantum state of light play a crucial role in a wide range of fields, from quantum information science to precision measurements. While for electrons in solid state materials complex quantum states can be created…
We perform narrowline cooling of single dysprosium atoms trapped in a 1D optical tweezers array, employing the narrow single-photon transition at 741 nm. At the trapping wavelength of 532 nm, the excited state is less trapped than the…
Entanglement between a single photon and a matter qubit is an indispensable resource for quantum repeater and quantum networks. With atomic ensembles, the entanglement creation probability is typically very low to inhibit high-order events.…