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The routine atomic-resolution structure determination of single particles is expected to have profound implications for probing the structure-function relationship in systems ranging from energy materials to biological molecules.…

Structure determination is a key application of XFELs and 4th generation synchrotron sources, particularly using the coherent and pulsed X-ray radiation from X-ray free-electron lasers (XFEL). Scientific interest focuses on understanding…

Instrumentation and Detectors · Physics 2025-03-07 Markus Kuster , Robert Hartmann , Steffen Hauf , Peter Holl , Tonn Rüter , Lothar Strüder

Convergent beam electron diffraction is routinely applied for studying deformation and local strain in thick crystals by matching the crystal structure to the observed intensity distributions. Recently, it has been demonstrated that CBED…

Mesoscale and Nanoscale Physics · Physics 2020-03-31 Tatiana Latychevskaia , Colin Robert Woods , Yi Bo Wang , Matthew Holwill , Eric Prestat , Sarah J. Haigh , Kostya S. Novoselov

In this study we elaborate on the recent concept of metagratings proposed in Ra'di et al. [Phys. Rev. Lett. 119, 067404 (2017)] for efficient manipulation of reflected waves. Basically, a metagrating is a set of 1D arrays of polarization…

Applied Physics · Physics 2018-08-01 V. Popov , F. Boust , S. N. Burokur

It is critical to characterize the carrier and instantaneous frequency distribution variation in ultrafast processes, all of which are determined by the optical phase. Nevertheless, there is no method that can single-shot record the…

Optics · Physics 2021-06-18 Wenchao Wang , Tianhao Xian , Li Zhan

Incoherent Diffraction Imaging - IDI - is a diffraction-based imaging technique that has been recently proposed to exploit the partial coherence of incoherently scattered light to retrieve structural information from the scattering centers.…

Coherent X-ray photons with energies higher than 50 keV offer new possibilities for imaging nanoscale lattice distortions in bulk crystalline materials using Bragg peak phase retrieval methods. However, the compression of reciprocal space…

Signal Processing · Electrical Eng. & Systems 2018-08-14 Siddharth Maddali , Irene Calvo-Almazan , Jonathan Almer , Peter Kenesei , Jun-Sang Park , Ross Harder , Youssef Nashed , Stephan Hruszkewycz

Recent interest in structure solution and refinement using electron diffraction (ED) has been fuelled by its inherent advantages when applied to crystals of sub-micron size, as well as a better sensitivity to light elements. Currently, data…

Computational Physics · Physics 2022-08-23 Anton Cleverley , Richard Beanland

In ultrafast electron diffraction (UED) experiments, accurate retrieval of time-resolved structural parameters, such as atomic coordinates and thermal displacement parameters, requires an accurate scattering model. Unfortunately,…

Materials Science · Physics 2023-01-03 Daniel B. Durham , Colin Ophus , Khalid M. Siddiqui , Andrew M. Minor , Daniele Filippetto

Phase-sensitive coherent imaging exploits changes in the phases of backscattered light to observe tiny alterations of scattering structures or variations of the refractive index. But moving scatterers or a fluctuating refractive index…

Two-color X-ray imaging with Free Electron Laser pulses offers a powerful approach for probing ultrafast structural dynamics in nanoscale systems, combining (near-)atomic spatial resolution with femtosecond temporal precision. The first…

Direct imaging of exoplanets requires very high contrast levels, which are obtained using coronagraphs. But residual quasi-static aberrations create speckles in the focal plane downstream of the coronagraph which mask the planet. This…

Instrumentation and Methods for Astrophysics · Physics 2015-06-16 J. Mazoyer , P. Baudoz , R. Galicher , M. Mas , G. Rousset

Single-shot coherent diffractive imaging (CDI) with intense short-wavelength light pulses enables the structural characterization of individual nanoparticles in free flight with high spatial and temporal resolution. Conventional CDI assumes…

Coherent diffractive imaging is unique as the only route for achieving diffraction-limited spatial resolution in the extreme ultraviolet and X-ray regions, limited only by the wavelength of the light. Recently, advances in coherent short…

We report the fabrication and performance evaluation of single crystal diamond refractive x-ray lenses with a paraboloid of rotation form factor for focusing x-rays in two dimensions simultaneously. The lenses were manufactured using a…

Instrumentation and Detectors · Physics 2015-07-13 S. Antipov , S. V. Baryshev , J. E. Butler , O. Antipova , Z. Liu , S. Stoupin

X-ray diffraction studies of nanoporous gold face the poorly understood diffraction scenario where large coherent crystals are riddled with nanoscale holes. Theoretical considerations derived in this study show that the ligament size of the…

Materials Science · Physics 2017-12-27 Matthias Graf , Bao-Nam Dinh Ngô , Jörg Weissmüller , Jürgen Markmann

Electronic screening renormalizes the linear bands of graphene and in the vicinity of the Dirac point, creates a diamond shaped structure in the quasiparticle spectral density. This is a result of electron-plasmon scattering processes which…

Mesoscale and Nanoscale Physics · Physics 2013-05-09 J. P. F. LeBlanc , J. P. Carbotte

Diffraction microtomography in coherent light is foreseen as a promising technique to image transparent living samples in three dimensions without staining. Contrary to conventional microscopy with incoherent light, which gives…

Optics · Physics 2009-11-13 Stanislas Vertu , Jean-Jacques Delaunay , Olivier Haeberle

Bragg coherent x-ray diffractive imaging is a powerful technique for investigating dynamic nanoscale processes in nanoparticles immersed in reactive, realistic environments. Its temporal resolution is limited, however, by the oversampling…

Materials Science · Physics 2016-05-25 A. Ulvestad , A. Tripathi , S. O. Hruszkewycz , W. Cha , S. M. Wild , G. B. Stephenson , P. H. Fuoss

We present results of a coherent x-ray diffractive imaging experiment performed on a single colloidal crystal grain. The full three-dimensional (3D) reciprocal space map measured by an azimuthal rotational scan contained several orders of…