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The structure of exotic nuclei provides valuable tests for state-of-the-art nuclear theory. In particular electromagnetic transition rates are more sensitive to aspects of nuclear forces and many-body physics than excitation energies alone.…

We investigate the structure and features of an ultralong-range triatomic Rydberg molecule formed by a Rb Rydberg atom and a KRb diatomic molecule. In our numerical description, we perform a realistic treatment of the internal rotational…

Basics of the Born-Oppenheimer (B-O) approximation are reviewed. Assuming the domain of applicability of B-O approximation is limited to 4 significant digits (s.d.) in energy spectrum, where mass, relativistic and QED corrections do NOT…

Atomic Physics · Physics 2025-04-10 Horacio Olivares-Pilon , Alexander V Turbiner

The calcium monohydroxide radical (CaOH) is an important astrophysical molecule relevant to cool stars and rocky exoplanets, amongst other astronomical environments. Here, we present a consistent set of highly accurate rovibronic…

Chemical Physics · Physics 2020-06-01 Y. Wang , A. Owens , J. Tennyson , S. N. Yurchenko

This is the first in a series of articles in which we study the rotating Morse potential model for diatomic molecules in the tridiagonal J-matrix representation. Here, we compute the bound states energy spectrum by diagonalizing the finite…

Chemical Physics · Physics 2011-11-10 I. Nasser , M. S. Abdelmonem , H. Bahlouli , A. D. Alhaidari

YbOH molecule is one of the most sensitive systems for the electron electric dipole moment ($e$EDM) searches. The $e$EDM-induced energy shift is proportional to polarization ($P$) of the molecule. In Ref. [A. Petrov and A. Zakharova, Phys.…

Atomic Physics · Physics 2024-02-14 Alexander Petrov

We investigate the nonrelativistic magnetic effect on the energy spectra, expectation values of some quantum mechanical observables and diamagnetic susceptibility for some diatomic molecules bounded by the Isotropic oscillator plus inverse…

We show the existence of ultra-long-range giant dipole molecules formed by a neutral alkali ground state atom that is bound to the decentered electronic wave function of a giant dipole atom. The adiabatic potential surfaces emerging from…

Atomic Physics · Physics 2012-03-14 Markus Kurz , Michael Mayle , Peter Schmelcher

We present a new theoretical method to treat the atom diatom radiative association within a time independent approach. This method is an adaptation of the driven equations method developed for photodissociation. The bound states energies…

Chemical Physics · Physics 2017-09-13 T. Stoecklin , F. Lique , M. Hochlaf

The LiFr diatomic represents a promising candidate for indirect laser cooling that has not yet been investigated not theoretically or experimentally. The potential energy curves of the ground and low_lying excited states of the LiFr…

Atomic Physics · Physics 2023-12-29 Maksim Shundalau , Patrizia Lamberti

Diatomic molecules with an energetically low-lying $^3 \Delta_1$ state are attractive platforms to detect new physics beyond the Standard Model, such as parity- and time-reversal violating phenomena. One of the advantages of using a $^3…

Atomic Physics · Physics 2026-02-19 Ayaki Sunaga , Timo Fleig

Vibrational energies and wave functions of the triplet state of the H3+ ion have been determined. In the calculations, the ground and first excited triplet electronic states are included as well as the non-Born-Oppenheimer coupling between…

Chemical Physics · Physics 2016-05-25 Alexander Alijah , Viatcheslav Kokoouline

Using the effective rotational Hamiltonian method, we have conducted an analysis of the D218O ground and the first excited vibration state rotational energy levels. The analysis was based on the effective Hamiltonians represented in several…

Chemical Physics · Physics 2021-01-18 I. A. Vasilenko , O. V. Naumenko , E. R. Polovtseva , A. D. Bykov

Using the ground potential energy surface[M. Ayouz \textit{et\, al}. J. Chem Phys \textbf{132} 194309 (2010)] of the H$_3^-$ molecule, we have determined the energies and widths of the complex resonant levels of H$_3^-$ located up to 4000…

Atomic Physics · Physics 2015-06-15 M. Ayouz , Olivier Dulieu , J. Robert

The vibrational branching ratios of SrOH for radiative decay to the ground electronic state, $X^{2}\Sigma^{+}$, from the first two electronically excited states, $A^{2}\Pi$ and $B^{2}\Sigma^{+}$, are determined experimentally at the…

Atomic Physics · Physics 2022-08-17 Zack Lasner , Annika Lunstad , Chaoqun Zhang , Lan Cheng , John M. Doyle

Searches for violations of the fundamental symmetries of parity P and time reversal T in atomic and molecular systems provide a powerful tool for precise measurements of the physics of and beyond the standard model. In this work, we…

Atomic Physics · Physics 2024-12-12 Sebastian Lahs , Daniel Comparat

We report optical trapping of a polyatomic molecule, calcium monohydroxide (CaOH). CaOH molecules from a magneto-optical trap are sub-Doppler laser cooled to $20(3)~\mu\text{K}$ in free space and loaded into an optical dipole trap. We…

Interatomic potentials approximate the potential energy of atoms as a function of their coordinates. Their main application is the effective simulation of many-atom systems. Here, we review empirical interatomic potentials designed to…

Materials Science · Physics 2022-11-11 Martin H. Muser , Sergey V. Sukhomlinov , Lars Pastewka

Full control of molecular interactions, including reactive losses, would open new frontiers in quantum science. Here, we demonstrate extreme tunability of chemical reaction rates by using an external electric field to shift excited…

Doppler and Sisyphus cooling of $^{174}$YbOH are achieved and studied. This polyatomic molecule has high sensitivity to physics beyond the Standard Model and represents a new class of species for future high-precision probes of new…