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Thin film growth of iron chalcogenides by pulsed laser deposition (PLD) is still a delicate issue in terms of simultaneous control of stoichiometry, texture, substrate/film interface properties, and superconducting properties. The high…

In this study, we fabricate 5-30-nm-thick films of FeSe/STO using pulsed laser deposition (PLD). The grown films exhibit superconductivity with an onset $T_{\mathrm{c}}$ that is much higher than that of bulk FeSe under ambient pressure. The…

Superconductivity · Physics 2022-06-16 T. Kobayashi , H. Ogawa , F. Nabeshima , A. Maeda

The interest in Fe-chalcogenide unconventional superconductors is intense after the critical temperature of FeSe was reported enhanced by more than one order of magnitude in the monolayer limit at the interface to an insulating oxide…

FeSe$_{1-x}$Te$_{x}$ thin films with PbO-type structure are successfully grown on MgO(100) and LaSrAlO$_{4}$(001) substrates from FeSe$_{1-x}$Te$_{x+d}$ polycrystalline targets by pulsed-laser deposition. The film deposited on the MgO…

Superconductivity · Physics 2009-08-11 Yoshinori Imai , Ryo Tanaka , Takanori Akiike , Masafumi Hanawa , Ichiro Tsukada , Atsutaka Maeda

Superconducting films emerge from the complex interplay of multiple growth parameters, making their optimization challenging. In iron-based superconductors, compressive strain is known to enhance the transition temperature (Tc) of FeSe…

Superconductivity · Physics 2026-04-22 Ya-Xun He , Xing-Jian Liu , Qun Wang , Ting Chen , Hassan Ali , Jia-Ying Zhang , Bao-Juan Kang , Zheng Zhang , Jun-Yi Ge

We have investigated the crystal structures and superconducting properties of thin films of FeSe$_{0.5}$Te$_{0.5}$ grown on eight different substrates. Superconductivity is not correlated with the lattice mismatch; rather it is correlated…

There is an ongoing debate about the relative importance of structural change versus doping charge carriers on the mechanism of superconductivity in Fe-based materials. Elucidating this issue is a major challenge since it would require a…

We have investigated the correlation between structural and transport properties in sputtered $\beta$-FeSe films grown onto SrTiO$_3$ (100). The growth parameters, such as substrate temperature and thickness, have been varied in order to…

Superconductivity · Physics 2019-10-23 M. V. Ale Crivillero , M. L. Amigó , N. Haberkorn , G. Nieva , J. Guimpel

The layered nature and simple structure of FeSe reveal this iron-based superconductor as a unique building block for the design of artificial heterostructure materials. While superconductivity develops in ultrathin films of FeSe on SrTiO3…

Superconductivity · Physics 2024-11-19 Yongsong Wang , Haojie Guo , Ane Etxebarria , Sandra Sajan , Sara Barja , Miguel M. Ugeda

We report the successful growth of epitaxial thin films of FeSe$_{1-x}$S$_x$ with $x \leq 0.43$ via pulsed laser deposition. As S content increases, the nematic transition temperature, $T_{\mathrm s}$, decreases systematically and the…

Superconductivity · Physics 2018-07-04 Fuyuki Nabeshima , Tomoya Ishikawa , Ken-ichi Oyanagi , Masataka Kawai , Atsutaka Maeda

Superconductivity was recently found in the simple tetragonal FeSe structure. Recent studies suggest that FeSe is unconventional, with the symmetry of the superconducting pairing state still under debate. To tackle these problems, clean…

Superconductivity · Physics 2015-05-13 M. J. Wang , J. Y. Luo , T. W. Huang , H. H. Chang , T. K. Chen , F. C. Hsu , C. T Wu , P. M. Wu , A. M. Chang , M. K. Wu

In this study, we demonstrate the successful fabrication of TiO2/FeSe/STO and TiO2/FeSe/LaAlO3 heterostructures using PLD. When the growth rates were sufficiently low, anatase TiO2, which has been reported to induce superconductivity in…

Superconductivity · Physics 2025-09-30 Tomoki Kobayashi , Hiroki Nakagawa , Ryo Ogawa , Atsutaka Maeda

Stabilized FeSe thin films in ambient pressure with tunable superconductivity would be a promising candidate for superconducting electronic devices yet its superconducting transition temperature (Tc) is below 10 K in bulk materials. By…

The presumably unconventional superconductor Beta-FeSe was deposited by radio frequency sputtering and molecular beam epitaxy (MBE) from two elementary sources. Superconducting thin films were grown in (001)-orientation on MgO(100) and…

Superconductivity · Physics 2015-05-12 Eike Venzmer , Alexander Kronenberg , Janek Maletz , Martin Jourdan

Pulsed laser deposition, a non-equilibrium thin-film growth technique, was used to stabilize metastable tetragonal iron sulfide (FeS), the bulk state of which is known as a superconductor with a critical temperature of 4 K. Comprehensive…

Materials Science · Physics 2019-03-22 Kota Hanzawa , Masato Sasase , Hidenori Hiramatsu , Hideo Hosono

We have studied the effect of tensile strain on the superconductivity in FeSe films. 50 nm, 100 nm, and 200 nm FeSe films were grown on MgO, SrTiO$_3$, and LaAlO$_3$ substrates by using a pulsed laser deposition technique. X-ray diffraction…

Superconductivity · Physics 2009-09-25 Y. F. Nie , E. Brahimi , J. I. Budnick , W. A. Hines , M. Jain , B. O. Wells

We report comprehensive angle-resolved photoemission investigations on the electronic structure of single crystal multiple-layer FeSe films grown on CaF2 substrate by pulsed laser deposition (PLD) method. Measurements on FeSe/CaF2 samples…

Superconductivity · Physics 2017-06-20 Bing Shen , Zhongpei Feng , Jianwei Huang , Yong Hu , Qiang Gao , Cong Li , Yu Xu , Guodong Liu , Li Yu , Lin Zhao , Kui Jin , X. J. Zhou

Superconducting epitaxial FeSe0.5Te0.5 thin films were prepared on SrTiO3 (001) substrates by pulsed laser deposition. The high purity of the phase, the quality of the growth and the epitaxy were studied with different experimental…

In contrast to its bulk crystals, the FeSe film or layer exhibits better superconductivity performance, which attract much interest in its fundamental research as well as potential application. In present work, transition from insulator to…

Superconductivity · Physics 2017-03-27 Wenbin Qiu , Zongqing Ma , Yongchang Liu , Xiaolin Wang , Shi Xue Dou

The discovery of high-temperature superconductivity in FeSe/SrTiO3 has sparked significant interests in exploring new superconducting systems with engineered interfaces. Here, using molecular beam epitaxy growth, we successfully fabricate…

Superconductivity · Physics 2025-02-20 Yunkai Guo , Xuanyu Long , Jingming Yan , Zheng Liu , Qi-Kun Xue , Wei Li
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