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High-resolution time-of-flight powder neutron diffraction and high-field magnetization were measured to investigate the magnetic structure and existence of a field-induced magnetic phase transition in the distorted kagome antiferromagnet…

The effect of substituting iron and zinc for cobalt in CaBaCo$_4$O$_7$ has been investigated using neutron diffraction and x-ray absorption spectroscopy. The orthorhombic distortion present in the parent compound CaBaCo$_4$O$_7$ decreases…

Materials Science · Physics 2020-09-01 V. Cuartero , J. Blasco , G. Subías , J. García , J. A. Rodríguez-Velamazán , C. Ritter

We determined the spin exchanges between the Cu2+ ions in the kagome layers of volborthite, Cu3V2O7(OH)2x2H2O, by performing the energy-mapping analysis based on DFT+U calculations, to find that the kagom\'e layers of Cu2+ ions are hardly…

Strongly Correlated Electrons · Physics 2022-03-02 Myung-Hwan Whangboa , Hyun-Joo Koo , Eva Brücher , Pascal Puphal , Reinhard K. Kremer

The quantum spin liquid material herbertsmithite is described by an antiferromagnetic Heisenberg model on the kagome lattice with non-negligible Dzyaloshinskii-Moriya interaction~(DMI). A well established phase transition to the $\mathbf…

Strongly Correlated Electrons · Physics 2017-07-04 Laura Messio , Samuel Bieri , Claire Lhuillier , Bernard Bernu

We have carried out neutron powder-diffraction measurements on zinc paratacamite Zn$_x$Cu$_{4-x}$(OH)$_6$Cl$_2$ with $x=1$, and studied the heat capacity in fields of up to 9 T for $0.5 \leq x \leq 1$. The $x=1$ phase has recently been…

Strongly Correlated Electrons · Physics 2009-11-13 M. A. de Vries , K. V. Kamenev , W. A. Kockelmann , J. Sanchez-Benitez , A. Harrison

We perform an exact diagonalization study of the spin-$1/2$ XXZ Heisenberg antiferromagnet on the kagome lattice at finite magnetization $m = \frac{2}{3}$ with an emphasis on the XY point ($J_z = 0$), and in the presence of a small chiral…

Strongly Correlated Electrons · Physics 2016-10-18 Krishna Kumar , Hitesh J. Changlani , Bryan K. Clark , Eduardo Fradkin

The search for Kitaev's quantum spin liquid (KQSL) state in real materials has recently expanded with the prediction that honeycomb lattices of divalent, high-spin cobalt ions could host the dominant bond-dependent exchange interactions…

Disorder induced by chemical inhomogeneity and Jahn-Teller (JT) distortions is often observed in mixed valence perovskite manganites. The main reasons for the evolution of this disorder are connected with the cationic size differences and…

Materials Science · Physics 2021-11-30 Sagar Ghorai , Sergey A. Ivanov , Ridha Skini , Petter Ström , Peter Svedlindh

The nontrivialness of quantum spin liquid (QSL) typically manifests in the non-local observables that signifies their existence, however, this fact actually casts shadow on detecting QSL with experimentally accessible probes. Here, we…

Strongly Correlated Electrons · Physics 2018-08-22 Guang Yu Sun , Yan-Cheng Wang , Chen Fang , Yang Qi , Meng Cheng , Zi Yang Meng

Owing to its unique geometry, the kagome lattice hosts various many-body quantum states including frustrated magnetism, superconductivity, and charge-density waves (CDWs), with intense efforts focused on kagome metals exhibiting $2\times2$…

Strongly Correlated Electrons · Physics 2023-11-28 Saizheng Cao , Chenchao Xu , Hiroshi Fukui , Taishun Manjo , Ming Shi , Yang Liu , Chao Cao , Yu Song

Two kagome compounds, volborthite Cu3V2O7(OH)2-2H2O and herbertsmithite ZnCu3(OH)6Cl2, are compared in order to derive information about the intrinsic properties of the spin-1/2 kagome antiferromagnet. Volborthite shows a broad maximum at T…

Strongly Correlated Electrons · Physics 2009-11-13 Z Hiroi , H Yoshida , Y Okamoto , M Takigawa

We compute the real-space spin correlations and frquency and wave-vector resolved dynamic structure factors $S(\vec q,\omega)$ for the nearest-neighbor Kagome-Lattice Heisenberg Antiferromagnet (KLHM) at finite temperatures using Numerical…

Strongly Correlated Electrons · Physics 2018-01-31 Nicholas E. Sherman , Rajiv R. P. Singh

Frustrated magnets offer a plethora of exotic magnetic ground states, including quantum spin liquids (QSLs), in which enhanced quantum fluctuations prevent a long-range magnetic ordering of the strongly correlated spins down to lowest…

New physics can emerge in magnetic materials where quantum fluctuations are enhanced due to reduced dimensionality and strong frustration. One long sought example is the resonating-valence-bond (RVB) state, where atomic magnetic moments are…

Strongly Correlated Electrons · Physics 2013-07-19 Tian-Heng Han , Joel S. Helton , Shaoyan Chu , Daniel G. Nocera , Jose A. Rodriguez-Rivera , Collin Broholm , Young S. Lee

Geometrical frustration among interacting spins combined with strong quantum fluctuations destabilize long-range magnetic order in favour of more exotic states such as spin liquids. By following this guiding principle, a number of spin…

Motivated by the search for chiral spin liquids (CSL), we consider a simple model defined on the kagome lattice of interacting SU(3) spins (in the fundamental representation) including two-site and three-site permutations between nearest…

Quantum spin liquid (QSL) phases exist in theory, but real candidate QSL materials are often extraordinarily sensitive to structural defects which disrupt the ground state. Here, we investigate candidate triangular QSL material…

Quantum spin liquids (QSLs) have become a key area of research in magnetism due to their remarkable properties, such as long-range entanglement, fractional excitations, pinch-point singularities, and topologically protected phenomena. In…

Strongly Correlated Electrons · Physics 2024-08-23 M. G. Gonzalez , V. Noculak , A. Sharma , V. Favre , J-R. Soh , A. Magrez , R. Bewley , H. O. Jeschke , J. Reuther , H. M. Rønnow , Y. Iqbal , I. Živković

The spin-1/2 kagome antiferromagnets are key prototype materials for studying frustrated magnetism. Three isostructural kagome antiferromagnets LnCu$_3$(OH)$_6$Cl$_3$ (Ln = Gd, Tb, Dy) have been successfully synthesized by the hydrothermal…

Strongly Correlated Electrons · Physics 2021-08-27 Ying Fu , Lianglong Huang , Xuefeng Zhou , Jian Chen , Xinyuan Zhang , Pengyun Chen , Shanmin Wang , Cai Liu , Dapeng Yu , Hai-Feng Li , Le Wang , Jia-Wei Mei

Motivated by the recent discovery of superconductivity in the kagome $A$V$_3$Sb$_5$ ($A$: K, Rb, Cs) metals, we perform a theoretical study of the symmetry-allowed superconducting orders on the two-dimensional kagome lattice with focus on…

Superconductivity · Physics 2023-10-27 Sofie Castro Holbæk , Morten H. Christensen , Andreas Kreisel , Brian M. Andersen