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Comparative molecular dynamics simulations of a hexamer cluster of the protic ionic liquid ethylammonium nitrate are performed using density functional theory (DFT) and density functional-based tight binding (DFTB) methods. The focus is on…

Chemical Physics · Physics 2017-03-24 Tobias Zentel , Oliver Kühn

We present a state-of-the-art density functional theory (DFT) study which models crucial features of the partially disordered orbital order stacking in the prototypical layered transition metal dichalcogenide 1T-TaS2 . Our results not only…

Strongly Correlated Electrons · Physics 2018-12-05 Tobias Ritschel , Helmuth Berger , Jochen Geck

The IrTe2 transition metal dichalcogenide undergoes a series of structural and electronic phase transitions when doped with Pt. The nature of each phase and the mechanism of the phase transitions have attracted much attention. In this…

Superconductivity · Physics 2015-04-22 Wei Ruan , Peizhe Tang , Aifang Fang , Peng Cai , Cun Ye , Xintong Li , Wenhui Duan , Nanling Wang , Yayu Wang

We studied dielectric properties of a polar nematic phase (NF) sandwiched between two gold or ITO electrodes, serving as a cell surfaces. In bulk, NF is expected to exhibit a Goldstone mode (phason), because polarization can uniformly…

The family of molecular conductors TMTTF/TMTSF-X demonstrates almost all known electronic phases in parallel with a set of weak structural modifications of anion ordering and mysterious structureless transitions. Only in early 2000's their…

Strongly Correlated Electrons · Physics 2007-05-23 Serguei Brazovskii

We study the dopant-induced inhomogeneity effect on the electronic properties of heavy fermionCeCoIn5using a combined approach of density functional theory (DFT) and dynamical mean-field theory (DMFT). The inhomogeneity of the hybridization…

Strongly Correlated Electrons · Physics 2022-04-06 Hong Chul Choi , Eric D. Bauer , Filip Ronning , Jian-Xin Zhu

Transition metal dichalcogenides offer unprecedented versatility to engineer 2D materials with tailored properties to explore novel structural and electronic phase transitions. In this work, we present the atomic-scale evolution of the…

Materials Science · Physics 2022-03-16 Wen Wan , Darshana Wickramaratne , Paul Dreher , Rishav Harsh , I. I. Mazin , Miguel M. Ugeda

The recent discovery of high-$T_c$ superconductivity in Ruddlesden-Popper (RP) nickelates has motivated extensive efforts to explore higher $T_c$ superconductors. Here, we systematically investigate Nd-doped La$_3$Ni$_2$O$_7$ using density…

Superconductivity · Physics 2026-01-06 Cui-Qun Chen , Wenyuan Qiu , Zhihui Luo , Meng Wang , Dao-Xin Yao

We explore the possibility and potential benefit of rolling a Si2BN sheet into single-walled nanotubes (NTs). Using density functional theory (DFT), we consider both structural stability and the impact on the nature of chemical bonding and…

Mesoscale and Nanoscale Physics · Physics 2022-03-16 Deobrat Singh , Vivekanand Shukla , Nabil Khossossi , Per Hyldgaard , Rajeev Ahuja

The metal-insulator transition (MIT) of VO2 is discussed with particular emphasis on the structural instability of the rutile compounds toward dimerization. Ti substitution experiments reveal that the MIT is robust up to 20% Ti…

Strongly Correlated Electrons · Physics 2022-02-01 Zenji Hiroi

Freeze Fracture Transmission Electron Microscopy (FFTEM) study of the nanoscale structure of the so-called "twist-bend" nematic (NX) phase of the cyanobiphenyl (CB) dimer molecule CB(CH2)7CB reveals a stripe texture of fluid layers…

The extended Frank elastic energy density is used to investigate the existence of a stable periodically modulate structure that appears as a ground state exhibiting a twist-bend molecular arrangement. For an unbounded sample, we show that…

Soft Condensed Matter · Physics 2017-06-01 M. P. Rosseto , R. R. Ribeiro de Almeida , R. S. Zola , G. Barbero , I. Lelidis , L. R. Evangelista

The role of layer disorder is important in establishing the topological phases of MoTe${_2}$. A rich tapestry of atomic ordering influences the structural phase transitions (SPTs), but there is little understanding of the mechanistic…

Materials Science · Physics 2023-12-07 Sumit Khadka , Leighanne C. Gallington , Byron Freelon

Depositing monolayer graphene on a transition metal dichalcogenide (TMD) semiconductor substrate has been shown to change the dynamics of the electronic states in graphene, inducing spin orbit coupling (SOC) and staggered potential effects.…

Mesoscale and Nanoscale Physics · Physics 2018-12-05 Abdulrhman M. Alsharari , Mahmoud M. Asmar , Sergio E. Ulloa

Spin-polarized DFT has been used to perform a comprehensive study of the geometric structures and electronic properties for isolated M4X4 nano-clusters between their two stable isomers - a planar rhombus-like 2D structure and a cubane-like…

Mesoscale and Nanoscale Physics · Physics 2015-12-29 Soumendu Datta , Badiur Rahaman

We present an ab initio analysis for the ground-state properties of a correlated organic compound $\kappa$-(BEDT-TTF)2Cu(NCS)2. First, we derive an effective two-dimensional low-energy model from first principles, having short-ranged…

Strongly Correlated Electrons · Physics 2012-03-09 Hiroshi Shinaoka , Takahiro Misawa , Kazuma Nakamura , Masatoshi Imada

The dipole moment is a crucial molecular property linked to a molecular system's bond polarity and overall electronic structure. To that end, the electronic dipole moment, which results from the electron density of a system, is often used…

Within the nuclear DFT approach, we determined the magnetic dipole and electric quadrupole moments for paired nuclear states corresponding to the proton (neutron) quasiparticles blocked in the p11/2- (n13/2+) intruder configurations. We…

Nuclear Theory · Physics 2023-08-22 J. Bonnard , J. Dobaczewski , G. Danneaux , M. Kortelainen

During the last half-decade, a new class of ferroic-fluid, ferroelectric nematic liquid crystals (NFLCs), creates a noise owing to its exceptional properties such as a colossal polarization, high electro-optic activity plus high fluidity.…

The Rietveld refinement of the polycrystalline powders of 1% Fe and Mn-doped (Na0.5Bi0.5)0.94Ba0.06Ti0.98V0.02O3 at the Ti-site confirmed a single rhombohedral (R3c) phase. The bandgap, (Eg) was affected by the anti-phase octahedral tilt…

Materials Science · Physics 2021-10-11 Koyal Suman Samantaray , Ruhul Amin , E. G Rini , Indranil Bhaumik , A. Mekki , K. Harrabi , Somaditya Sen