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Two-dimensional (2D) crystals of semiconducting transition metal dichalcogenides (TMD) absorb a large fraction of incident photons in the visible frequencies despite being atomically thin. It has been suggested that the strong absorption is…

The perturbation of a semiconductor from the thermodynamic equilibrium often leads to the display of nonlinear dynamics and formation of spatiotemporal patterns due to the spontaneous generation of competing processes. Here, we describe the…

Materials Science · Physics 2019-09-16 Ebrahim Najafi , Amir Jafari , Bolin Liao , Ahmed Zewail

We report results from ultrafast two-color optical pump-probe spectroscopy on bulk $\beta$-Ga$_2$O$_3$. A two-photon absorption scheme is used to photoexcite carriers with the pump pulse and free-carrier absorption of the probe pulse is…

Materials Science · Physics 2019-01-30 Okan Koksal , Nicholas Tanen , Debdeep Jena , Huili Xing , Farhan Rana

Monolayers of transition metal dichalcogenides (TMDCs) exhibit an exceptionally strong Coulomb interaction between charge carriers due to the two-dimensional carrier confinement in connection with weak dielectric screening. High densities…

Mesoscale and Nanoscale Physics · Physics 2018-08-08 D. Erben , A. Steinhoff , G. Schönhoff , T. O. Wehling , C. Gies , F. Jahnke

Results of experimental pump-probe spectroscopy of a quantum dash optical amplifier biased at transparency are presented. Using strong pump pulses we observe a competition between free carrier absorption and two-photon induced stimulated…

Mesoscale and Nanoscale Physics · Physics 2015-06-03 Per Lunnemann , Sara Ek , Kresten Yvind , Rozenn Piron , Jesper Mørk

Many of the fundamental optical and electronic properties of atomically thin transition metal dichalcogenides are dominated by strong Coulomb interactions between electrons and holes, forming tightly bound atom-like excitons. Here, we…

Understanding defect effect on carrier dynamics is essential for both fundamental physics and potential applications of transition metal dichalcogenides. Here, the phenomenon of oxygen impurities trapping photo-excited carriers has been…

In transition metal dichalcogenides layers of atomic scale thickness, the electron-hole Coulomb interaction potential is strongly influenced by the sharp discontinuity of the dielectric function across the layer plane. This feature results…

Understanding the fundamental mechanisms ruling laser-induced coherent charge transfer in hybrid organic/inorganic interfaces is of paramount importance to exploit these systems in next-generation opto-electronic applications. In a…

Materials Science · Physics 2022-05-12 Matheus Jacobs , Jannis Krumland , Caterina Cocchi

The optical and electronic properties of 2D semiconductors are intrinsically linked via the strong interactions between optically excited bound species and free carriers. Here we use near-field scanning microwave microscopy (SMM) to image…

Optoelectronic excitations in monolayer MoS2 manifest from a hierarchy of electrically tunable, Coulombic free-carrier and excitonic many-body phenomena. Investigating the fundamental interactions underpinning these phenomena - critical to…

In this letter, we present non-degenerate ultrafast optical pump-probe studies of the carrier recombination dynamics in MoS$_{2}$ monolayers. By tuning the probe to wavelengths much longer than the exciton line, we make the probe…

Mesoscale and Nanoscale Physics · Physics 2015-06-22 Haining Wang , Changjian Zhang , Farhan Rana

Optical limiting (OL), a crucial mechanism for protecting human eyes and sensitive sensors from intense radiation, relies on understanding the optical nonlinearities acting on the systems. Assessing and disentangling the effects at play is…

Optics · Physics 2025-07-30 Mustapha Driouech , Michele Guerrini , Caterina Cocchi

Harnessing short-lived photoexcited electron-hole pairs in metal nanostructures has the potential to define a new phase of optoelectronics, enabling control of athermal mechanisms for light harvesting, photodetection and photocatalysis. To…

We analyze the optical pump-probe reflection and transmission coefficients when the photoinduced response depends nonlinearly on the incident pump intensity. Under these conditions, we expect the photoconductivity depth profile to change…

Strongly Correlated Electrons · Physics 2024-10-30 Leya Lopez , Derek G. Sahota , J. Steven Dodge

We study carrier interaction induced many-body effects on the excitonic optical properties of highly photoexcited one-dimensional semiconductor quantum wire systems by solving the dynamically screened Bethe-Salpeter equation using realistic…

Strongly Correlated Electrons · Physics 2009-11-07 D. W. Wang , S. Das Sarma

Prototypes for hot-carrier solar cells based on type-II InAs/AlAsSb multiple quantum wells are examined for AC photoconductivity as a function of lattice temperature and photoexcitation energy to determine the photoexcited charge carrier…

Mesoscale and Nanoscale Physics · Physics 2022-04-12 H. P. Piyathilaka , R. Sooriyagoda , V. R. Whiteside , T. D. Mishima , M. B. Santos , I. R. Sellers , A. D. Bristow

We experimentally demonstrate a novel nonlinear effect in optical fibers: upconversion luminescence generation excited by multiphoton absorption of femtosecond infrared pulses. We directly estimate the average number of photons involved in…

Optics · Physics 2020-09-29 F. Mangini , M. Ferraro , M. Zitelli , A. Niang , A. Tonello , V. Couderc , S. Wabnitz

Optically generated electron-hole pairs can probe strongly correlated electronic matter, or, by forming exciton-polaritons within an optical cavity, give rise to photonic nonlinearities. The present paper theoretically studies the…

Strongly Correlated Electrons · Physics 2020-04-29 Tobias Graß , Ovidiu Cotlet , Atac İmamoğlu , Mohammad Hafezi

We study nonequilibrium carriers (electrons and holes) in an intrinsic graphene at low temperatures under far- and mid-infrared (IR) radiation in a wide range of its intensities. The energy distributions of carriers are calculated using a…

Materials Science · Physics 2010-06-29 A. Satou , F. T. Vasko , V. Ryzhii
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