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Related papers: Towards the complete phase profiling of attosecond…

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Laser-assisted photoemission from a solid is considered within a numerically exactly solvable one-dimensional model of a crystal. The effect of the inelastic scattering and of the finite duration of the pump pulse on the photoelectron…

Materials Science · Physics 2015-06-10 E. E. Krasovskii , C. Friedrich , W. Schattke , P. M. Echenique

We investigate theoretically electron dynamics under a VUV attosecond pulse train which has a controlled phase delay with respect to an additional strong infrared laser field. Using the strong field approximation and the fact that the…

Atomic Physics · Physics 2015-05-13 P. Riviere , O. Uhden , U. Saalmann , J. M. Rost

The present work focuses on the characterisation of the amount of orbital angular momentum (OAM) encoded in the twisted attosecond pulses via energy- and angle-resolved attosecond streaking in pump-probe setup. It is found that the…

Atomic Physics · Physics 2020-06-03 Irfana N. Ansari , Deependra S. Jadoun , Gopal Dixit

We present an analytical model capable of describing two-photon ionization of atoms with attosecond pulses in the presence of intermediate and final isolated autoionizing states. The model is based on the finite-pulse formulation of…

Atomic Physics · Physics 2016-03-02 Álvaro Jiménez Galán , Fernando Martín , Luca Argenti

Natively, atomic and molecular processes develop in a sub-femtosecond time scale. In order to, for instance, track and capture the electron motion in that scale we need suitable `probes'. Attosecond pulses configure the most appropriate…

Shape resonances in physics and chemistry arise from the spatial confinement of a particle by a potential barrier. In molecular photoionization, these barriers prevent the electron from escaping instantaneously, so that nuclei may move and…

Attosecond angular streaking measurements have revealed deep insights into the timing of tunnel ionization processes of atoms in intense laser fields. So far experiments of this type have been performed only with a cold-target recoil-ion…

Atomic Physics · Physics 2013-10-21 Matthias Weger , Jochen Maurer , André Ludwig , Lukas Gallmann , Ursula Keller

Coherent, broadband pulses of extreme ultraviolet (XUV) light provide a new and exciting tool for exploring attosecond electron dynamics. Using photoelectron streaking, interferometric spectrograms can be generated that contain a wealth of…

Atomic Physics · Physics 2020-08-26 Luca Pedrelli , Phillip D. Keathley , Laura Cattaneo , Franz X. Kärtner , Ursula Keller

Attosecond light pulses in the extreme ultraviolet have drawn a great deal of attention due to their ability to interrogate electronic dynamics in real time. Nevertheless, to follow charge dynamics and excitations in materials, element…

Atomic Physics · Physics 2016-06-08 S. M. Teichmann , F. Silva , S. L. Cousin , M. Hemmer , J. Biegert

Coherence among rotational ion channels during photoionization is exploited to control the anisotropy of the resulting photoelectron angular distributions at specific photoelectron energies. The strategy refers to a robust and single…

Chemical Physics · Physics 2019-09-11 R. Chamakhi , M. Telmini , O. Atabek , E. Charron

Characterizing the quantum state of intense light fields on sub-cycle timescales remains beyond the reach of existing methods. Here, we show that attosecond streaking provides direct, phase-sensitive access to the quantum properties of the…

Quantum Physics · Physics 2026-04-16 En-Rui Zhou , Yi-Jia Mao , Pei-Lun He , Feng He

Field-emission of electrons underlies major advances in science and technology, ranging from imaging the atomic-scale structure of matter to signal processing at ever-higher frequencies. The advancement of these applications to their…

Optics · Physics 2023-02-22 H. Y. Kim , M. Garg , S. Mandal , L. Seiffert , T. Fennel , E. Goulielmakis

We study the temporal aspects of laser-assisted extreme ultraviolet (XUV) photoionization using attosecond pulses of harmonic radiation. The aim of this paper is to establish the general form of the phase of the relevant transition…

Time-resolved photoelectron spectra are proposed for the measurement of classical information recorded in the quantum phases of a molecular rotational wave packet. Taking Li2 as a prototypical system, we show that an interference arises…

Quantum Physics · Physics 2007-05-23 Eric Charron , Maurice Raoult

Ultrafast processes in matter, such as the electron emission following light absorption, can now be studied using ultrashort light pulses of attosecond duration ($10^{-18}$s) in the extreme ultraviolet spectral range. The lack of spectral…

We present a combined numerical and theoretical study of atomic photoionization in the time domain. We show how a photoelectron wave packet rapidly changes its shape after being emitted, from a complex multi-peak structure to eventually a…

Atomic Physics · Physics 2018-04-03 Ruihua Xu , Zhaoyan Zhou , Xu Wang

The generation of the shortest isolated attosecond pulses requires both broad spectral bandwidth and control of the spectral phase. Rapid progress has been made in both aspects, leading to the generation of the world-record-shortest 67 as…

Optics · Physics 2013-12-06 Michael Chini , Kun Zhao , Zenghu Chang

Attosecond interferometry in a two-color field is central to attosecond metrology and spectroscopy. In this technique, a photoelectron wave packet is released when a single photon from an extreme ultraviolet comb is absorbed. The wave…

We explore the novel capabilities offered by attosecond extreme ultraviolet and x-ray pulses that can be now generated by free-electron lasers and high-harmonics generation sources for probing photon-induced electron dynamics in molecules.…

Quantum Physics · Physics 2023-02-15 Marvin Reuner , Daria Popova-Gorelova