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Using density matrix equations of motion and a tight-binding band calculation, we predict all-optical switching between four metastable magnetic states of (III,Mn)As ferromagnets. This switching is initiated non-thermally within 100fs,…

Optics · Physics 2015-05-30 M. D. Kapetanakis , P. C. Lingos , C. Piermarocchi , J. Wang , I. E. Perakis

The tremendous interest in the technology and underlying physics of all-optical switching of magnetization brings up the question of how fast the switching can occur and how high the frequency of writing the data with ultrafast laser pulses…

Single femtosecond pulse toggle switching of ferrimagnetic alloys is an essential building block for ultrafast spintronics. Very different element-specific demagnetization dynamics is believed to be a hard limit for switching in…

Materials Science · Physics 2022-05-11 F. Jakobs , U. Atxitia

Energy-efficient control of magnetization without the help of a magnetic field is a key goal of spintronics. Purely heat-induced single-pulse all-optical toggle switching has been demonstrated, but so far only in Gd based amorphous…

Materials Science · Physics 2020-11-10 C. Banerjee , N. Teichert , K. Siewierska , Z. Gercsi , G. Atcheson , P. Stamenov , K. Rode , J. M. D. Coey , J. Besbas

Faster magnetic recording technology is indispensable to massive data storage and big data sciences. {All-optical spin switching offers a possible solution}, but at present it is limited to a handful of expensive and complex rare-earth…

Materials Science · Physics 2016-11-03 G. P. Zhang , Y. H. Bai , T. F. George

Interest in all-optical spin switching (AOS) is growing rapidly. The recent discovery of AOS in Mn$_2$RuGa provides a much needed clean case of crystalline ferrimagnets for theoretical simulations. Here, we attempt to simulate it using the…

Materials Science · Physics 2020-11-05 G. P. Zhang , Robert Meadows , Antonio Tamayo , Y. H. Bai , Thomas F. George

We resolve a significant controversy about how to understand and engineer single-shot all-optical switching of magnetization in ferrimagnets using femto- or picosecond-long heat pulses. By realistically modelling a generic ferrimagnet as…

Mesoscale and Nanoscale Physics · Physics 2020-03-04 C. S. Davies , T. Janssen , J. H. Mentink , A. Tsukamoto , A. V. Kimel , A. F. G. van der Meer , A. Stupakiewicz , A. Kirilyuk

We study the demagnetization dynamics of the fully compensated half-metallic ferrimagnet Mn$_2$Ru$_x$Ga. While the two antiferromagnetically coupled sublattices are both composed of manganese, they exhibit different temperature dependencies…

Materials Science · Physics 2021-01-18 G. Bonfiglio , K. Rode , G. Y. P. Atcheson , P. Stamenov , J. M. D. Coey , A. V. Kimel , Th. Rasing , A. Kirilyuk

All-optical spin switching (AOS) represents a new frontier in magnetic storage technology -- spin manipulation without a magnetic field, -- but its underlying working principle is not well understood. Many AOS ferrimagnets such as GdFeCo…

Materials Science · Physics 2022-07-22 G. P. Zhang , Y. H. Bai , M. S. Si , Thomas F. George

All-optical spin switching (AOS) is a new phenomenon found in a small group of magnetic media, where a single laser pulse can switch spins from one direction to another, without assistance of a magnetic field, on a time scale much shorter…

Materials Science · Physics 2024-06-18 G. P. Zhang , Y. Q. Liu , M. S. Si , Nicholas Allbritton , Y. H. Bai , Wolfgang Hübner , Thomas F. George

Picosecond switching of the staggered antiferromagnetic order is shown to be realizable through spin-transfer torques from a short current pulse. The coupled dynamics of sublattice magnetization is mapped onto a classical pendulum subject…

Mesoscale and Nanoscale Physics · Physics 2015-03-03 Ran Cheng , Matthew W. Daniels , Jian-Gang Zhu , Di Xiao

We bridge an essential knowledge gap on the understanding of all-optical ultrafast switching in ferrimagnets; namely, the connection between atomistic spin dynamics methods and macroscopic phenomenological models. All-optical switching of…

Materials Science · Physics 2022-06-29 Florian Jakobs , Unai Atxitia

Although all-optical magnetization switching with fs laser pulses has garnered much technological interest, the ultimate data rates achievable have scarcely been investigated. Recently it has been shown that after a switching event in a…

Mesoscale and Nanoscale Physics · Physics 2022-07-06 Youri L. W. van Hees , Bert Koopmans , Reinoud Lavrijsen

Single-pulse switching has been experimentally demonstrated in ferrimagnetic GdFeCo and Mn$_2$Ru$_x$Ga alloys. Complete understanding of single-pulse switching is missing due to the lack of an established theory accurately describing the…

Materials Science · Physics 2022-07-27 Florian Jakobs , Unai Atxitia

$FeCr_2S_4$ is a ferrimagnet with two oppositely ordered spin sublattices (Fe and Cr), connected via superexchange interaction, giving a non-zero net magnetic moment. We show, using time-resolved measurements of the magneto-optic Kerr…

The Slater-Pauling rule states that L21 Heusler compounds with 24 valence electrons do never exhibit a total spin magnetic moment. In case of strongly localized magnetic moments at one of the atoms (here Mn) they will exhibit a fully…

In this work, we investigate single-shot all-optical switching (AOS) in Tb/Co/Gd/Co/Tb multilayers in an attempt to establish AOS in synthetic ferrimagnets with high perpendicular magnetic anisotropy. In particular, we study the effect of…

Ultrashort optical pulses are a cornerstone for manipulating electronic and magnetic states in materials on a femtosecond timescale. Conventional models assume that optical excitation primarily modifies the occupation of the electron energy…

Materials Science · Physics 2025-05-12 Sergii Parchenko , Peter M. Oppeneer , Andreas Scherz

Experimentally observed ultrafast all-optical magnetization reversal in ferrimagnetic metals and heterostructures based on antiferromagnetically coupled ferromagnetic $d-$ and $f-$metallic layers relies on intricate energy and angular…

Strongly Correlated Electrons · Physics 2016-03-02 Alexandra Kalashnikova , Veniamin Kozub

Ultrafast control of magnetization on the nanometer length scale, in particular all-optical switching, is key to putting ultrafast magnetism on the path towards future technological application in data storage technology. However,…

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