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We describe an ab initio and non-perturbative $R$-matrix with time-dependence theory for ultrafast atomic processes in light fields of arbitrary polarization. The theory is applicable to complex, multielectron atoms and atomic ions subject…

Atomic Physics · Physics 2018-12-04 D. D. A. Clarke , G. S. J. Armstrong , A. C. Brown , H. W. van der Hart

We investigate the orientation dependence of Enhanced Ionization (EI) during strong-field-driven nuclear motion in acetylene (C$_2$H$_2$). Here, we both initiate and probe molecular dynamics in acetylene with intense 6-fs cross-polarized…

Atomic Physics · Physics 2024-11-08 S. A. Mohideen , A. J. Howard , C. Cheng , I. Gabalski , A. M. Ghrist , E. Weckwerth , P. H. Bucksbaum

We report on tunnel ionization of Xe by 2-cycle, intense, infrared laser pulses and its dependence on carrier-envelope-phase (CEP). At low values of optical field ($E$), the ionization yield is maximum for cos-like pulses with the…

In a previous publication, procedures were proposed for unambiguously extracting amplitudes for single and double ionization from a time-dependent wavepacket by effectively propagating for an infinite time following a radiation pulse. Here…

Atomic Physics · Physics 2009-11-13 A. Palacios , T. N. Rescigno , C. W. McCurdy

It has long been observed that the number of weak lines from many-electron atoms follows a power law distribution of intensity. While computer simulations have reproduced this dependence, its origin has not yet been clarified. Here we…

Atomic Physics · Physics 2020-05-13 Keisuke Fujii , Julian C. Berengut

We review the main aspects of multiple photoionization processes in atoms exposed to intense, short wavelength radiation. The main focus is the theoretical framework for the description of such processes as well as the conditions under…

Atomic Physics · Physics 2014-01-21 P. Lambropoulos , G. M. Nikolopoulos

It is shown that it is feasible to use ultrashort time delay between two XUV femtosecond pulses in order to control two photon resonant ionization. The proposal is demonstrated on the spectrum of Helium, in terms of nonperturbative…

Atomic Physics · Physics 2019-08-22 Theodoros Mercouris , Yannis Komninos , Cleanthes A. Nicolaides

Photoelectron energy spectra resulting by the interaction of hydrogen with two short pulses having carrier frequencies, respectively, in the range of the infrared and XUV regions have been calculated. The effects of the pulse duration and…

Other Condensed Matter · Physics 2015-05-18 Saverio Bivona , Giovanni Bonanno , Riccardo Burlon , Claudio Leone

We apply time-dependent R-matrix theory to study inner-shell ionization of C atoms in ultra-short high-frequency light fields with a photon energy between 170 and 245 eV. At an intensity of 10$^{17}$ W/cm$^2$, ionization is dominated by…

Atomic Physics · Physics 2015-08-12 H. F. Rey , H. W. van der Hart

We calculate the electron energy spectrum of ionization by a high energy photon, accompanied by creation of electron-positron pair. The total cross section of the process is also obtained. The asymptotics of the cross section does not…

Quantum Physics · Physics 2015-06-26 E. G. Drukarev , A. I. Mikhailov , I. A. Mikhailov , Kh. Yu. Rakhimov , W. Scheid

We describe new exact results for a model of ionization of a bound state, induced by an oscillating potential. In particular we have obtained exact expressions, in the form of readily computable rapidly convergent sums, for the energy…

Mathematical Physics · Physics 2017-10-17 Ovidiu Costin , Rodica D. Costin , Joel L. Lebowitz

Multiphoton ionization of sodium by laser pulses of 800 nm wavelength and 57 fs duration is studied in the range of laser peak intensities belonging to over-the-barrier ionization regime. Photoelectron momentum distributions (PMD) and the…

Atomic Physics · Physics 2019-03-21 Andrej Bunac , Duška B. Popović , Nenad S. Simonović

The multiphoton ionization rate of molecules depends on the alignment of the molecular axis with respect to the ionizing laser polarization. By studying molecular frame photo-electron angular distributions from N$_2$, O$_2$ and benzene, we…

Chemical Physics · Physics 2015-06-15 C T L Smeenk , L Arissian , A V Sokolov , M Spanner , K F Lee , A Staudte , D M Villeneuve , P B Corkum

A new method for the generation of a train of pulses from a single high-energy, ultra short pulse is presented, suited for Resonant Multi-Pulse Ionization injection. The method is based on different transverse portion of the pulse being…

Accelerator Physics · Physics 2018-12-26 G. Vantaggiato , L. Labate , P. Tomassini , L. A. Gizzi

The electron residual energy originated from the stochastic heating in under-dense field-ionized plasma is here investigated. The optical response of plasma is initially modeled by using the concept of two counter-propagating…

Plasma Physics · Physics 2018-04-26 Elnaz Khalilzadeh , Jam Yazdanpanah , Jafar Jahanpanah , Amir Chakhmachi , Elnaz Yazdani

We explore the interactions between Argon and extreme ultraviolet (XUV) laser pulses across photon energies of 200 eV, 260 eV, and 315 eV, scrutinizing the influence of photon energy on Argon ion yields and unraveling the associated…

Atomic Physics · Physics 2024-04-15 Linhao Xiong

We extend a recently developed three-dimensional semiclassical model [\href{https://journals.aps.org/pra/abstract/10.1103/PhysRevA.109.033106}{Phys. Rev. \textbf{A} 109, 033106 (2024)}] to study multielectron ionization and the formation of…

Atomic Physics · Physics 2026-02-17 Georgios Petros Katsoulis , Agapi Emmanouilidou

We study strong field molecular ionization using few- (four to ten) cycle laser pulses. Employing a supercontinuum light source, we are able to tune the optical laser wavelength (photon energy) over a range of about $\sim$200 nm (500 meV).…

Exchange correlation plays an important role in double-ionization of complex atoms by ultrashort laser pulse. In this work, we investigate two-photon double inner-shell electron ionization of neon induced by an attosecond extreme…

Atomic Physics · Physics 2019-06-05 Jianpeng Liu , Yongqiang Li , Jianmin Yuan

We present a method to measure the kinetic energy of electrons emitted upon ion impact via their time-of-flight. Pulsed beams of H$^{+}$, D$_2^{+}$, He$^{+}$ and Ne$^{+}$ ions with velocities between 0.4 and 3.5 a.u. are transmitted through…

Instrumentation and Detectors · Physics 2020-08-26 Svenja Lohmann , Anna Niggas , Vincent Charnay , Radek Holeňák , Daniel Primetzhofer