Related papers: Slow Spin Relaxation in Single Endohedral Fulleren…
Spins confined in quantum dots are a leading candidate for solid-state quantum bits that can be coherently controlled by optical pulses. There are, however, many challenges to developing a scalable multibit information processing device…
We determine experimentally the spin structure of half-metallic Co2FeAl0.4Si0.6 Heusler alloy elements using magnetic microscopy. Following magnetic saturation, the dominant magnetic states consist of quasi-uniform configurations, where a…
Magnetic relaxation in coordination compounds is largely dominated by the interaction of the spin with phonons. Large zero-field splitting and exchange coupling values have been empirically found to strongly suppress spin relaxation and…
We review the problem of spin decoherence of magnetic atoms deposited on a surface. Recent breakthroughs in scanning tunnelling microscopy (STM) make it possible to probe the spin dynamics of individual atoms, either isolated or integrated…
Spin dynamics of assemblies of magnetic nanomolecules and nanoclusters can be made coherent by inserting the sample into a coil of a resonant electric circuit. Coherence is organized through the arising feedback magnetic field of the coil.…
Recent theory and experiment in crystals of molecular magnets suggest that fundamental tests of the decoherence mechanisms of macroscopic quantum phenomena may be feasible in these systems (which are almost ideal quantum spin glasses). We…
Polar polyatomic molecules provide an ideal but largely unexplored platform to encode qubits in rotational states. Here, we trap cold (100-600 mK) formaldehyde (H$_2$CO) inside an electric box and perform a Ramsey-type experiment to observe…
We investigate the performance of dynamical decoupling methods at suppressing electron spin decoherence from a low-temperature nuclear spin reservoir in a quantum dot. The controlled dynamics is studied through exact numerical simulation,…
Single-molecule magnets are among the most promising platforms for achieving molecular-scale data storage and processing. Their magnetisation dynamics are determined by the interplay between electronic and vibrational degrees of freedom,…
This study investigates spin squeezed states in nuclear magnetic resonance (NMR) quadrupolar systems with spins $I=3/2$ and $I=7/2$ at room temperature, taking into account the effects of relaxation on the dynamics. The origin of spin…
The spin dynamics in [TbPc$_{2}$]$^{0}$ and [DyPc$_{2}$]$^{0}$ single molecule magnets have been investigated by means of muon and nuclear spin-lattice relaxation rate measurements. The correlation time for the spin fluctuations was found…
Micron-sized magnetic platelets in the flux closed vortex state are characterized by an in-plane curling magnetization and a nanometer-sized perpendicularly magnetized vortex core. Having the simplest non-trivial configuration, these…
We investigate the magnetocaloric properties of certain antiferromagnetic spin systems that have already been or very likely can be synthesized as magnetic molecules. It turns out that the special geometric frustration which is present in…
Entanglement in a many-particle system can enable measurement sensitivities beyond that achievable by only classical correlations. For an ensemble of spins, all-to-all interactions are known to reshape the quantum projection noise, leading…
Below 360 mK, Fe magnetic molecular clusters are in the pure quantum relaxation regime and we show that the predicted square-root time relaxation is obeyed, allowing us to develop a new method for watching the evolution of the distribution…
Given the effectiveness of semiconductor devices for classical computation one is naturally led to consider semiconductor systems for solid state quantum information processing. Semiconductors are particularly suitable where local control…
We explore how to encode more than a qubit in vanadyl porphyrin molecules hosting a electronic spin 1/2 coupled to a nuclear spin 7/2. The spin Hamiltonian and its parameters, as well as the spin dynamics, have been determined via a…
Strongly interacting spins underlie many intriguing phenomena and applications ranging from magnetism to quantum information processing. Interacting spins combined with motion display exotic spin transport phenomena, such as superfluidity…
We investigated the spin coherence of high-mobility two-dimensional electron gases confined in multilayer GaAs quantum wells. The dynamics of the spin polarization was optically studied using pump-probe techniques: time-resolved Kerr…
We report specific heat, magnetic, and muon spin relaxation measurements performed on a polycrystalline sample of the normal spinel CdHo2S4. The rare-earth ions sit on a lattice of corner-sharing regular tetrahedra as in pyrochlore…