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We present a method for the reconstruction of ion kinetic energy distributions from ion time-of-flight mass spectra through ion trajectory simulations. In particular, this method is applicable to complicated spectrometer geometries with…

Atomic and Molecular Clusters · Physics 2024-05-22 Aaron Ngai , Katrin Dulitz , Sebastian Hartweg , Janine Franz , Marcel Mudrich , Frank Stienkemeier

For the description of an H2 molecule an effective one-electron model potential is proposed which is fully determined by the exact ionization potential of the H2 molecule. In order to test the model potential and examine its properties it…

Chemical Physics · Physics 2009-11-13 Armin Lühr , Yulian V. Vanne , Alejandro Saenz

We introduce a machine learning model to predict atomization energies of a diverse set of organic molecules, based on nuclear charges and atomic positions only. The problem of solving the molecular Schr\"odinger equation is mapped onto a…

Photoelectron momentum distributions (PMDs) from atoms and molecules undergo qualitative changes as laser parameters are varied. We present a model to interpret the shape of the PMDs. The electron's motion is guided by a fictitious particle…

Chaotic Dynamics · Physics 2018-09-19 Jonathan Dubois , Simon Berman , Cristel Chandre , Turgay Uzer

Strong field ionization provides a unique mean to address complex dynamics of an electron in competing Coulomb and laser fields. Recent streak camera experiment (K\"ubel, et al., Phys. Rev. Lett. 119, 183201) analyzed asymmetries in the…

We propose a pseudopotential for the electron-electron Coulomb interaction to improve the efficiency of many-body electronic structure calculations. The pseudopotential accurately replicates the scattering properties of the Coulomb…

Strongly Correlated Electrons · Physics 2015-09-02 J. H. Lloyd-Williams , R. J. Needs , G. J. Conduit

We investigate the physical processes in which an electron, upon return to its parent ion, promotes a second electron to an excited state, from which it subsequently tunnels. Employing the strong-field approximation and saddle-point…

Atomic Physics · Physics 2015-05-13 T. Shaaran , C. Figueira de Morisson Faria

We give a procedure for reconstructing a magnetic field and electric potential from boundary measurements related to the magnetic Schroedinger operator in three and higher dimensions.

Analysis of PDEs · Mathematics 2007-05-23 Mikko Salo

At the future electron-positron TeV linear collider, the reachable physics will be strongly dependent on the detector capability to reconstruct high energy jets in multi-jet environment. At LEP, SLD experiments, a technique combining…

Instrumentation and Detectors · Physics 2017-08-23 Jean-Claude Brient

We experimentally demonstrate that a non-classical state prepared in an atomic memory can be efficiently transferred to a single mode of free-propagating light. By retrieving on demand a single excitation from a cold atomic gas, we realize…

We demonstrate that the angular distribution of photoelectrons from a strongly polarizable target exposed to a laser field can deviate noticeably from the prediction of conventional theory. Even within the dipole-photon approximation the…

Atomic and Molecular Clusters · Physics 2009-11-13 A. V. Korol , A. V. Solov'yov

We present a procedure to reconstruct objects from holograms recorded in in-line holography settings. Working with one beam of polarized light, the topological derivatives and energies of functionals quantifying hologram deviations yield…

Optics · Physics 2018-04-09 A. Carpio , T. G. Dimiduk , V. Selgas , P. Vidal

We have probed the fragmentation dynamics in a bent triatomic molecule, water, a non-planar molecule, methanol, and a planar ring-structured molecule, benzene, using 100 fs duration pulses of linearly and circularly polarized, infrared,…

Atomic Physics · Physics 2009-11-10 F A Rajgara , M Krishnamurthy , D Mathur

Recently, in a strong Coulomb field regime of tunneling ionization an unexpected large enhancement of photoelectron spectra due to the Coulomb field of the atomic core has been identified by numerical solution of time-dependent…

Atomic Physics · Physics 2018-12-05 Pei-Lun He , Michael Klaiber , Karen Z. Hatsagortsyan , Christoph H. Keitel

An iterative method is derived for image reconstruction. Among other attributes, this method allows constraints unrelated to the radiation measurements to be incorporated into the reconstructed image. A comparison is made with the widely…

Computational Physics · Physics 2011-01-06 Clinton DeW. Van Siclen

Strong-field ionization can induce electron motion in both the continuum and the valence shell of the parent ion. Here, we explore their interplay by studying laser-induced electron diffraction (LIED) patterns arising from interaction with…

Multiphoton ionization of helium is investigated in the superintense field regime, with particular emphasis on the role of the electron-electron interaction in the ionization and stabilization dynamics. To accomplish this, we solve ab…

Quantum Physics · Physics 2015-05-27 S. A. Sørngård , S. Askeland , R. Nepstad , M. Førre

We explore the mathematical and numerical aspects of reconstructing a potential energy profile of a molecular bond from its rupture time distribution. While reliable reconstruction of gross attributes, such as the height and the width of an…

Statistical Mechanics · Physics 2015-05-18 Pak-Wing Fok , Tom Chou

Quantifying material mass and electron density from computed tomography (CT) reconstructions can be highly valuable in certain medical practices, such as radiation therapy planning. However, uniquely parameterising the X-ray attenuation in…

Medical Physics · Physics 2019-04-30 Jonathan H. Mason , Alessandro Perelli , William H. Nailon , Mike E. Davies

A method for characterising the wave-function of freely-propagating particles would provide a useful tool for developing quantum-information technologies with single electronic excitations. Previous continuous-variable quantum tomography…

Mesoscale and Nanoscale Physics · Physics 2020-01-22 J. D. Fletcher , N. Johnson , E. Locane , P. See , J. P. Griffiths , I. Farrer , D. A. Ritchie , P. W. Brouwer , V. Kashcheyevs , M. Kataoka
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