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Photoelectrochemical (PEC) water splitting offers an elegant approach for solar energy conversion into hydrogen fuel. Large-scale hydrogen production requires stable and efficient photoelectrodes and scalable PEC cells that are fitted for…

The current state of the art in direct water splitting in photo-electrochemical cells (PECs) is presented together with: (i) a case study of water splitting using a simple solar cell with the most efficient water splitting electrodes and…

The splitting of water with sunlight using photoelectrochemical cell (PEC) to produce hydrogen is a promising avenue for sustainable energy production. The greatest virtue of PEC is that it uses sunlight as the only source to split water,…

Chemical Physics · Physics 2013-05-14 Qiang Yu , Chuanbao Cao

Although photoelectrochemical water splitting is likely to be an important and powerful tool to provide environmentally friendly hydrogen, most developments in this field have been conducted on a laboratory scale so far. In order for the…

The majority of photoelectrochemical (PEC) water splitting cells cannot drive the overall water splitting reactions without the assistance of an external power source. To provide added power, the cells are usually connected to photovoltaic…

Applied Physics · Physics 2018-10-31 Gideon Segev , Jeffery Beeman , Ian D. Sharp

Photoelectrochemical (PEC) water splitting to generate hydrogen is one of the most studied methods for converting solar energy into clean fuel because of its simplicity and potentially low cost. Despite over 40 years of intensive research,…

Materials Science · Physics 2019-01-02 Ling-Ju Guo , Jun-Wei Luo , Tao He , Su-Huai Wei , Shu-Shen Li

Photoelectrochemical (PEC) water splitting is a promising method for conversing solar energy into chemical energy stored in the form of hydrogen. Nanostructured hematite ($\alpha$-Fe$_2$O$_3$) is one of the most attractive materials for…

The low conversion rate and efficiency always weaken the performance of thermochemical water-splitting reaction. Herein, we, for the first time, conducted the thermodynamic study of a hydrogen permeable membrane (HPM) in an isothermal…

Materials Science · Physics 2018-08-08 Chenxi Sui , Hongsheng Wang , Xiang Liu , Xuejiao Hu

Hydrogen is considered a promising environmentally friendly energy carrier for replacing traditional fossil fuels. In this context, photoelectrochemical (PEC) cells effectively convert solar energy directly to H2 fuel by water…

Applied Physics · Physics 2019-03-22 Sebastiano Bellani , Maria Rosa Antognazza , Francesco Bonaccorso

Recent rapid progress in efficiencies for solar water splitting by photoelectrochemical devices has enhanced its prospects to enable storable renewable energy. Efficient solar fuel generators all use tandem photoelectrode structures, and…

The photocatalytic splitting of water into molecular hydrogen and molecular oxygen with sunlight is the dream reaction for solar energy conversion. Since decades, transition-metal-oxide semiconductors and supramolecular organometallic…

Chemical Physics · Physics 2018-07-10 Wolfgang Domcke , Johannes Ehrmaier , Andrzej L. Sobolewski

Photocatalytic water splitting offers a viable and sustainable method for hydrogen production. MXenes, a class of 2D transition-metal carbides/nitrides, have emerged as potential photocatalysts and co-catalysts due to their tunable…

Materials Science · Physics 2025-06-17 C. B. Subba , Prasad Mattipally , J. Sivakumar , A. Laref , A. Yvaz , D. P. Rai , Z. Pachuau

Due to the energy supply pressure caused by non-renewable fuels as well as the environment-related issues, the efficient conversion of solar-chemical energy via photo-induced water splitting is one of the promising strategies to address the…

Chemical Physics · Physics 2021-03-23 Zhexu Xi

Photosynthesis is nature's route to convert intermittent solar irradiation into storable energy, while its use for an industrial energy supply is impaired by low efficiency. Artificial photosynthesis provides a promising alternative for…

Materials Science · Physics 2015-09-16 Matthias M. May , Hans-Joachim Lewerenz , David Lackner , Frank Dimroth , Thomas Hannappel

The production of hydrogen from water using only a catalyst and solar energy is one of the most challenging and promising outlets for the generation of clean and renewable energy. Semiconductor photocatalysts for solar hydrogen production…

In this review, we discuss disruptive decoupled water splitting schemes, in which the concurrent production of hydrogen and oxygen in close proximity to each other in conventional electrolysis is replaced by time- or space-separated…

Applied Physics · Physics 2020-07-28 Avigail Landman , Gideon S. Grader , Avner Rothschild

In this work, we present a novel artificial photosynthetic paradigm with square meter (m2) level scalable production by integrating photovoltaic electrolytic water splitting device and solar heating CO2 hydrogenation device, successfully…

Photocatalytic water splitting has greatly stimulated as an ideal technique for producing hydrogen (H$_{2}$) fuel by employing two renewable sources, i.e., water and solar energy. Here, we have adopted a facile hydrothermal approach for the…

Chemical Physics · Physics 2022-01-04 Fahmida Sharmin , Dayal Chandra Roy , M. A. Basith

Energy storage becomes crucial for energy systems with an increasing share of renewable energy sources. Artificial photosynthesis, in particular photovoltaic water splitting, provides both sustainable energy generation and energy storage in…

Materials Science · Physics 2016-04-12 Bugra Turan , Jan-Philipp Becker , Felix Urbain , Friedhelm Finger , Uwe Rau , Stefan Haas

Photoelectrochemical solar water splitting is a promising approach to convert solar energy into sustainable hydrogen fuel using semiconductor electrodes. Due to their visible light absorption properties, oxynitrides have shown to be…

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