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Laser radiation incident on a ferromagnetic sample produces excited electrons and currents whose spin polarization must not be aligned with the magnetization -- an effect due to spin-orbit coupling that is ubiquitous in spin- and…

Materials Science · Physics 2023-11-03 Oliver Busch , Franziska Ziolkowski , Ingrid Mertig , Jürgen Henk

While the understanding of altermagnetism is still at a very early stage, it is expected to play a role in various fields of condensed matter research, for example spintronics, caloritronics and superconductivity. In the field of optical…

Mesoscale and Nanoscale Physics · Physics 2024-09-04 T. Adamantopoulos , M. Merte , F. Freimuth , D. Go , M. Ležaić , W. Feng , Y. Yao , J. Sinova , L. Šmejkal , S. Blügel , Y. Mokrousov

We theoretically study the dynamic time evolution following laser pulse pumping in an antiferromagnetic insulator Cr$_{2}$O$_{3}$. From the photoexcited high-spin quartet states to the long-lived low-spin doublet states, the ultrafast…

Strongly Correlated Electrons · Physics 2017-06-29 Feng Guo , Na Zhang , Wei Jin , Jun Chang

In the context of spin electronics, the two spin-channel model assumes that the spin carriers are composed of two distinct populations: the conduction electrons of spin up, and the conduction electrons of spin down. In order to distinguish…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 J. -E. Wegrowe , H. -J. Drouhin

We report on {\it ab-initio} simulations of the quantum dynamics of electronic charge and spin when subjected to intense laser pulses. By performing separate calculations for a Ni thin film and bulk Ni, we conclude that surface effects have…

Materials Science · Physics 2017-05-24 K. Krieger , P. Elliott , T. Müller , N. Singh , J. K. Dewhurst , E. K. U. Gross , S. Sharma

The total angular momentum of a close system is a conserved quantity, which should remain constant in time for any excitation experiment once the pumping signal has extinguished. Such conservation, however, is never satisfied in practice in…

Mesoscale and Nanoscale Physics · Physics 2022-04-13 Jacopo Simoni , Stefano Sanvito

It is of great interest to develop methods to rapidly and effectively control the magnetic configurations in artificial spin ices, which are arrangements of dipolar coupled nanomagnets that have a variety of fascinating collective magnetic…

Mesoscale and Nanoscale Physics · Physics 2026-02-10 D. Pecchio , S. Sahoo , O. Chubykalo-Fesenko , S. Koraltan , G. M. Macauley , T. Thomson , D. Suess , V. Scagnoli , L. J. Heyderman

The magnetization dynamics of a synthetic antiferromagnet subject to a short magnetic field pulse, has been studied by using a combination of first-principles and atomistic spin dynamics simulations. We observe switching phenomena on the…

Despite spin (SAM) and orbital (OAM) angular momentum dynamics are well-studied in demagnetization processes, their components receive less focus. Here, we utilize the non-collinear spin version of real-time time-dependent density…

Mesoscale and Nanoscale Physics · Physics 2024-02-28 Junjie He , Shuo Li , Thomas Fruenheim

Current induced magnetization manipulation is a key issue for spintronic application. Therefore, deterministic switching of the magnetization at the picoseconds timescale with a single electronic pulse represents a major step towards the…

Materials Science · Physics 2017-04-13 Y. Xu , M. Deb , G. Malinowski , M. Hehn , W. Zhao , S. Mangin

Irradiating solids with ultrashort laser pulses is known to initiate femtosecond timescale magnetization dynamics. However, sub-femtosecond spin dynamics have not yet been observed or predicted. Here, we explore ultrafast light-driven spin…

Mesoscale and Nanoscale Physics · Physics 2023-03-28 Ofer Neufeld , Nicolas Tancogne-Dejean , Umberto De Giovannini , Hannes Hübener , Angel Rubio

The ultrafast response to an optical pulse excitation of the spin-spin exchange interaction in transition metal anti-ferromagnets is studied within the framework of the time-dependent spin-density functional theory. We propose a formulation…

Mesoscale and Nanoscale Physics · Physics 2017-08-16 Jacopo Simoni , Maria Stamenova , Stefano Sanvito

We analyze theoretically the novel pathway of ultrafast spin dynamics for ferromagnets with high enough single-ion anisotropy (non-Heisenberg ferromagnets). This longitudinal spin dynamics includes the coupled oscillations of the modulus of…

Strongly Correlated Electrons · Physics 2013-10-28 E. G. Galkina , V. I. Butrim , Yu. A. Fridman , B. A. Ivanov , F. Nori

Magneto-optical techniques have become essential tools in spintronics, enabling the investigation of spin dynamics in the ultrafast regime. A key challenge in this field has been to accurately isolate the contributions to magneto-optical…

Picosecond switching of the staggered antiferromagnetic order is shown to be realizable through spin-transfer torques from a short current pulse. The coupled dynamics of sublattice magnetization is mapped onto a classical pendulum subject…

Mesoscale and Nanoscale Physics · Physics 2015-03-03 Ran Cheng , Matthew W. Daniels , Jian-Gang Zhu , Di Xiao

The ultra-fast demagnetization of small iron clusters initiated by an intense optical excitation is studied with time-dependent spin density functional theory (TDSDFT). In particular we investigate the effect of the spin-orbit interaction…

Mesoscale and Nanoscale Physics · Physics 2016-07-27 Maria Stamenova , Jacopo Simoni , Stefano Sanvito

We analyze theoretically the demagnetization dynamics in a ferromagnetic model system due to the interplay of spin-orbit coupling and electron-electron Coulomb scattering. We compute the $k$-resolved electronic reduced spin-density matrix…

Materials Science · Physics 2022-08-05 Svenja Vollmar , Kai Leckron , Hans Christian Schneider

We report about the dephasing of the spins states in a Garnet film excited by femtosecond laser pulses. It is shown that magneto-optical four-wave-mixing signals are efficiently generated and controlled with an external static magnetic…

Mesoscale and Nanoscale Physics · Physics 2013-11-05 M. Barthelemy , M. Vomir , M. Sanches Piaia , H. Vonesch , P. Molho , B. Barbara , J. -Y. Bigot

The ultra-fast magnetisation relaxation rates during the laser-induced magnetisation process are analyzed in terms of the Landau-Lifshitz-Bloch (LLB) equation for different values of spin $S$. The LLB equation is equivalent in the limit $S…

Materials Science · Physics 2015-05-20 U. Atxitia , O. Chubykalo-Fesenko

At the ultrafast limit of optical spin manipulation is the theoretically predicted phenomena of optical intersite spin transfer (OISTR), in which laser induced charge transfer between the sites of a multi-component material leads to control…

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