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It is now well established that a few femtosecond laser pulse will induce an ultrafast loss of moment in a magnetic material. Here we show that the opposite effect can also occur: an ultrafast increase in moment. Employing both…

Ultrafast magnetization dynamics are governed by energy flow between electronic, magnetic, and lattice degrees of freedom. A quantitative understanding of these dynamics must be based on a model that agrees with experimental results for all…

Femtosecond laser light can transfer spin angular momentum between magnetic subspecies that exhibit hybridized valence bands within an alloy or compound, and represents the fastest route for manipulating the magnetization of a material. To…

We propose a semi-classical model for femtosecond-laser induced demagnetization due to spin-polarized excited electron diffusion in the super-diffusive regime. Our approach treats the finite elapsed time and transport in space between…

Materials Science · Physics 2011-06-14 Marco Battiato , Karel Carva , Peter M. Oppeneer

A joint theoretical and experimental investigation is performed to understand the underlying physics of laser-induced demagnetization in Ni and Co films. Experimentally dynamics of spins is studied by determining the time-dependent…

Disentangling orbital (OAM) and spin (SAM) angular momenta in the ultrafast spin dynamics of two-dimensional (2D) ferromagnets on subfemtoseconds is a challenge in the field of ultrafast magnetism. Herein, we employed non-collinear spin…

Materials Science · Physics 2024-01-09 Shuo Li , Ran Wang , Thomas Frauenheim , Junjie He

The ultimate control of magnetic states of matter at femtosecond (or even faster) timescales defines one of the most pursued paradigm shifts for future information technology. In this context, ultrafast laser pulses developed into extremely…

Mesoscale and Nanoscale Physics · Physics 2022-03-15 Hanan Hamamera , Filipe Souza Mendes Guimarães , Manuel dos Santos Dias , Samir Lounis

The orbital angular momenta (OAM) of electrons play an increasingly important role in ultrafast electron and magnetization dynamics. In this theoretical study, we investigate the electron dynamics induced by femtosecond laser pulses in a…

Materials Science · Physics 2023-10-13 Oliver Busch , Franziska Ziolkowski , Ingrid Mertig , Jürgen Henk

Reducing energy dissipation while increasing speed in computation and memory is a long-standing challenge for spintronics research. In the last 20 years, femtosecond lasers have emerged as a tool to control the magnetization in specific…

Ultrafast demagnetization of magnetic layers pumped by a femtosecond laser pulse is accompanied by a nonthermal spin-polarized current of hot electrons. These spin currents are studied here theoretically in a spin valve with noncollinear…

Mesoscale and Nanoscale Physics · Physics 2018-02-26 Pavel Baláž , Martin Žonda , Karel Carva , Pablo Maldonado , Peter M. Oppeneer

Irradiation with an ultrashort laser pulse can completely destroy the magnetic order of ferromagnetic thin films on the femtosecond timescale. This phenomenon holds great potential for ultrafast spintronics and information processing and is…

Optics · Physics 2022-06-16 Eva Prinz , Benjamin Stadtmüller , Martin Aeschlimann

The dynamics of single laser-driven electrons and many particle systems with spin are investigated on the basis of a classical theory. We demonstrate that the spin forces can alter the electron dynamics in an ultra-relativistic laser field…

Plasma Physics · Physics 2014-06-17 Meng Wen , Heiko Bauke , Christoph H. Keitel

Femtosecond laser pulses can be used to induce ultrafast changes of the magnetization in magnetic materials. Several microscopic mechanisms have been proposed to explain the observations, including the transport of ultrashort spin-polarized…

By comparing femtosecond laser pulse induced ferro- and antiferromagnetic dynamics in one and the same material - metallic dysprosium - we show both to behave fundamentally different. Antiferromagnetic order is considerably faster and much…

Femtosecond laser pulses can induce ultrafast demagnetization as well as generate bursts of hot electron spin currents. In trilayer spin valves consisting of two metallic ferromagnetic layers separated by a nonmagnetic one, hot electron…

Materials Science · Physics 2020-05-27 Ulrike Ritzmann , Pavel Baláž , Pablo Maldonado , Karel Carva , Peter M. Oppeneer

Most laser-induced femtosecond magnetism investigations are done in magnetic thin films. Nanostructured magnetic dots, with their reduced dimensionality, present new opportunities for spin manipulation. Here we predict that if a magnetic…

Materials Science · Physics 2015-05-27 G. P. Zhang , M. S. Si , T. F. George

Exact calculated time evolutions in the framework of a many-electron model of itinerant magnetism provide new insights into the laser-induced ultrafast demagnetization observed in ferromagnetic (FM) transition metal thin films. The…

Strongly Correlated Electrons · Physics 2015-11-25 W. Töws , G. M. Pastor

Spin and orbital angular momenta are two intrinsic properties of an electron and are responsible for the physics of a solid. How the spin and orbital evolve with respect to each other on several hundred femtoseconds is largely unknown, but…

Materials Science · Physics 2021-06-25 G. P. Zhang , Mingqiang Gu , Y. H. Bai , T. L. Jenkins , Thomas F. George

Experimental observations of the ultrafast (less than 50 fs) demagnetization of Ni have so far defied theoretical explanations particularly since its spin-flipping time is much less than that resulting from spin-orbit and electron-lattice…

Strongly Correlated Electrons · Physics 2020-07-08 Shree Ram Acharya , Volodymyr Turkowski , Guo-ping Zhang Talat S. Rahman

We demonstrate optical control of magnons using femtosecond laser pulses by performing ab-initio real-time time-dependent density functional theory (TDDFT) simulations. We predict that the spin-wave dynamics in Fe$_{50}$Ni$_{50}$ can be…

Materials Science · Physics 2021-04-07 N. Singh , P. Elliott , J. K. Dewhurst , S. Sharma