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Most of the performances of electrochemical devices are governed by molecular processes taking place at the solution-electrode interfaces and molecular simulation are the main way to study these processes. Aqueous electrochemical systems…

Chemical Physics · Physics 2019-12-12 Guillaume Jeanmairet , Benjamin Rotenberg , Daniel Borgis , Mathieu Salanne

The study of alloys using computational methods has been a difficult task due to the usually unknown stoichiometry and local atomic ordering of the different structures experimentally. In order to combat this, first-principles methods have…

Materials Science · Physics 2021-12-08 Daniel Wines , Kayahan Saritas , Can Ataca

Based on recent advancements in using machine learning for classical density functional theory for systems with one-dimensional, planar inhomogeneities, we propose a machine learning model for application in two dimensions (2D) akin to…

Statistical Mechanics · Physics 2025-05-22 Felix Glitsch , Jens Weimar , Martin Oettel

By partitioning the electron density into subsystem contributions, the Frozen Density Embedding (FDE) formulation of subsystem DFT has recently emerged as a powerful tool for reducing the computational scaling of Kohn--Sham DFT. To date,…

Materials Science · Physics 2015-06-22 Alessandro Genova , Davide Ceresoli , Michele Pavanello

Density Functional Theory (DFT) has become the quasi-standard for ab-initio simulations for a wide range of applications. While the intrinsic cubic scaling of DFT was for a long time limiting the accessible system size to some hundred…

Materials Science · Physics 2018-02-23 Stephan Mohr , Marc Eixarch , Maximilian Amsler , Mervi J. Mantsinen , Luigi Genovese

Machine learning approaches have the potential to approximate Density Functional Theory (DFT) for atomistic simulations in a computationally efficient manner, which could dramatically increase the impact of computational simulations on…

Computational Physics · Physics 2022-07-05 Joseph Musielewicz , Xiaoxiao Wang , Tian Tian , Zachary Ulissi

The fractional quantum Hall effect remains a captivating area in condensed matter physics, characterized by strongly correlated topological order, which manifests as fractionalized excitations and anyonic statistics. Numerical simulations,…

Strongly Correlated Electrons · Physics 2025-10-27 Yi Yang , Yayun Hu , Zi-Xiang Hu

Specialized Deep Learning (DL) acceleration stacks, designed for a specific set of frameworks, model architectures, operators, and data types, offer the allure of high performance while sacrificing flexibility. Changes in algorithms,…

FFT-based solvers introduced in the 1990s for the numerical homogenization of heterogeneous elastic materials have been extended to a wide range of physical properties. In parallel, alternative algorithms and modified discrete Green…

Materials Science · Physics 2015-05-20 Lionel Gélébart , Franck Ouaki

The simulation of fracture using continuum ductile damage models attains a pathological discretization dependence caused by strain localization, after loss of ellipticity of the problem, in regions whose size is connected to the spatial…

Computational Engineering, Finance, and Science · Computer Science 2021-04-21 M. Magri , S. Lucarini , G. Lemoine , L. Adam , J. Segurado

Density functional theory (DFT) has become a standard tool for the study of point defects in materials. However, finding the most stable defective structures remains a very challenging task as it involves the solution of a multimodal…

Materials Science · Physics 2020-11-16 Marco Arrigoni , Georg K. H. Madsen

There is ample experimental evidence on the existence of several crystalline phases of C4F8, although they still have been not clearly identified. In this paper we perform a series of molecular dynamics (MD) simulations using a partially…

Soft Condensed Matter · Physics 2009-10-31 Z. Gamba , B. M. Powell

Mixed-dimensional mathematical models for flow in fractured media have been prevalent in the modeling community for almost two decades, utilizing the explicit representation of fractures by lower-dimensional manifolds embedded in the…

In modern engineering designs, advanced materials (e.g., fiber/particle-reinforced polymers, metallic alloys, laminar composites, etc.) are widely used, where microscale heterogeneities such as grains, inclusions, voids, micro-cracks, and…

Computational Engineering, Finance, and Science · Computer Science 2022-10-24 Haoyan Wei , Dandan Lyu , Wei Hu , C. T. Wu

Gaussian Mixture Models (GMMs) are a standard tool in data analysis. However, they face problems when applied to high-dimensional data (e.g., images) due to the size of the required full covariance matrices (CMs), whereas the use of…

Machine Learning · Computer Science 2023-08-29 Alexander Gepperth

Mathematical models and computer algorithms are developed to calculate dynamic stress concentration and fracture wave propagation in a reinforced composite sheet. The composite consists of a regular system alternating extensible fibers and…

Computational Physics · Physics 2012-03-09 M. Ayzenberg-Stepanenko , Z. Yanovitsky , G. Osharovich

We benchmark the ground state energies and the density profiles of atomic repulsive Fermi gases in optical lattices computed via Density Functional Theory (DFT) against the results of diffusion Monte Carlo (DMC) simulations. The main focus…

Quantum Gases · Physics 2018-06-12 S. Pilati , I. Zintchenko , M. Troyer , F. Ancilotto

Soft porous crystals present a challenge to molecular dynamics simulations with flexible size and shape of the simulation cell (i.e., in the NPT ensemble), since their framework responds very sensitively to small external stimuli. Hence,…

We extend the FE-DMN method to fully coupled thermomechanical two-scale simulations of composite materials. In particular, every Gauss point of the macroscopic finite element model is equipped with a deep material network (DMN). Such a DMN…

Computational Engineering, Finance, and Science · Computer Science 2021-11-30 Sebastian Gajek , Matti Schneider , Thomas Böhlke

Selecting excitations in localized orbitals to calculate long-range correlation contributions to range-separated density-functional theory can reduce the overall computational effort significantly. Beyond simple selection schemes of excited…

Chemical Physics · Physics 2016-02-29 E Chermak , Peter Reinhardt , Bastien Mussard , Janos Angyan