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The perovskite oxynitride LaTiO\textsubscript{2}N is a promising material for photocatalytic water splitting under visible light. One of the obstacles towards higher efficiencies of this and similar materials stems from charge-carrier…

Materials Science · Physics 2018-01-31 Nathalie Vonrüti , Ulrich Aschauer

We report the relationship between epitaxial strain and the crystallographic orientation of the in-phase rotation axis and A-site displacements in Pbnm-type perovskite films. Synchrotron diffraction measurements of EuFeO3 films under strain…

Multiferroics are a unique class of materials where magnetic and ferroelectric orders coexist. The research on multiferroics contributes significantly to the fundamental understanding of the strong correlations between different material…

Materials Science · Physics 2021-11-03 A. C. Garcia-Castro , Yanjun Ma , Zachary Romestan , Eric Bousquet , Cheng Cen , Aldo H. Romero

Perovskite oxynitrides are a promising class of material for photocatalytic water-splitting due to their small band gaps and suitably aligned band edges. Recently, epitaxially strained oxynitrides started to attract interest due to the…

Materials Science · Physics 2018-10-17 Nathalie Vonrüti , Ulrich Aschauer

Perovskite oxynitrides have recently attracted attention for their ability to photocatalytically split water. Compared to oxides the arrangement of anions in the material represents a further structural degree of freedom. The bulk…

Materials Science · Physics 2018-10-31 Silviya Ninova , Ulrich Aschauer

B-site ordered thin films of double perovskite Sr$_2$CoIrO$_6$ were epitaxially grown by a metal-organic aerosol deposition technique on various substrates, actuating different strain states. X-ray diffraction, transmission electron…

Strongly Correlated Electrons · Physics 2018-05-23 S. Esser , C. F. Chang , C. -Y. Kuo , S. Merten , V. Roddatis , T. D. Ha , A. Jesche , V. Moshnyaga , H. -J. Lin , A. Tanaka , C. T. Chen , L. H. Tjeng , P. Gegenwart

We have investigated the effect of epitaxial strain on the magnetic properties and $B$-site cation ordering in multiferroic Bi$_2$FeCrO$_6$ (001) thin films using a density-functional theory approach. We find that in thin films with…

Materials Science · Physics 2016-03-30 Paresh Chandra Rout , Aditya Putatunda , Varadharajan Srinivasan

Epitaxial thin films of multiferroic perovskite BiMnO3 were synthesized on SrTiO3 substrates, and orbital ordering and magnetic properties of the thin films were investigated. The ordering of the Mn^{3+} e_g orbitals at a wave vector (1/4…

Materials Science · Physics 2009-11-11 C. -H. Yang , T. Y. Koo , S. -H. Lee , C. Song , K. -B. Lee , Y. H. Jeong

We report the synthesis of SrMnO$_{3-{\delta}}$F$_{{\gamma}}$ perovskite oxyfluoride thin films using a vapor transport method to fluorinate as-grown SrMnO$_{2.5}$ epitaxial thin films. The influence of the fluoropolymer, which acts as a…

Materials Science · Physics 2018-07-25 Jiayi Wang , Yongjin Shin , Elke Arenholz , Benjamin M. Lefler , James M. Rondinelli , Steven J. May

We use first-principles calculations to investigate the stability of bi-axially strained \textit{Pnma} perovskite CaMnO$_3$ towards the formation of oxygen vacancies. Our motivation is provided by promising indications that novel material…

Materials Science · Physics 2013-08-28 Ulrich Aschauer , Reto Pfenninger , Sverre M. Selbach , Tor Grande , Nicola A. Spaldin

Switchable order parameters in ferroic materials are essential for functional electronic devices, yet disruptions of the ordering can take the form of planar boundaries or defects that exhibit distinct properties. Characterizing the…

We demonstrate how shape-induced strain can be used to control antiferromagnetic order in NiO/Pt thin films. For rectangular elements patterned along the easy and hard magnetocrystalline anisotropy axes of our film, we observe different…

We use first principles density functional theory calculations to examine the effect of multiple anions on the Peierls distortion in the rutile oxyfluoride TiOF. By using a structure enumeration approach, we obtain the ground state atomic…

Materials Science · Physics 2024-05-14 Siddhartha S. Nathan , Danilo Puggioni , James M. Rondinelli

We use first-principles calculations based on density functional theory to investigate the interplay between oxygen vacancies, A-site cation size / tolerance factor, epitaxial strain, ferroelectricity and magnetism in the perovskite…

Materials Science · Physics 2021-03-09 Astrid Marthinsen , Carina Faber , Ulrich Aschauer , Nicola A. Spaldin , Sverre M. Selbach

Epitaxial strain plays an important role in determining physical properties of perovskite ferroelectric oxide thin films. However, it is very challenging to directly measure properties such as polarization in ultrathin strained films using…

Perovskites with the generic composition ABO$_3$ exhibit an enormous variety of quantum states such as magnetism, orbital order, ferroelectricity and superconductivity. Their flexible and comparatively simple structure allows for facile…

In the perovskite oxide SrCrO$_{3}$ the interplay between crystal structure, strain and orbital ordering enables a transition from a metallic to an insulating electronic structure under certain conditions. We identified a narrow window of…

We investigate energetically favorable structures of ABO$_2$N oxynitrides as functions of pressure and strain via swarm-intelligence-based structure prediction methods, DFT lattice dynamics and first-principles molecular dynamics. We…

Materials Science · Physics 2021-06-11 Li Zhu , Hiroyuki Takenaka , R. E. Cohen

We attribute the structural phase transition (SPT) in the parent compounds of the iron pnictides to orbital ordering. Due to the anisotropy of the $d_{xz}$ and $d_{yz}$ orbitals in the $xy$ plane, a ferro-orbital ordering makes the…

Strongly Correlated Electrons · Physics 2013-05-29 Weicheng Lv , Jiansheng Wu , Philip Phillips

We report and compare the structural, magnetic, and optical properties of ordered La2NiMnO6 thin films and its disordered LaNi0.5Mn0.5O3 counterpart. An x-ray diffraction study reveals that the B-site Ni/Mn ordering induces additional XRD…

Materials Science · Physics 2015-05-13 M. P. Singh , K. D. Truong , S. Jandl , P. Fournier
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