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Spectro-microscopy is an experimental technique which can be used to observe spatial variations in chemical state and changes in chemical state over time or under experimental conditions. As a result it has broad applications across areas…

Medical Physics · Physics 2026-02-05 Maike Meier , Lorenzo Lazzarino , Boris Shustin , Hussam Al Daas , Paul Quinn

Frequency comb spectroscopy has significantly advanced molecular spectroscopy across scientific research and diverse applications. Among its key performance metrics especially for time-resolved studies, sensitivity and measurement speed are…

Joint spectral measurements are a powerful tool for characterising biphoton spectral correlation, which is crucial for quantum information and communication technologies. In these applications, highly pure biphoton states are essential in…

Spectral diffusion is a result of random spectral jumps of a narrow line as a result of a fluctuating environment. It is an important issue in spectroscopy, because the observed spectral broadening prevents access to the intrinsic line…

Long-range active imaging has a variety of applications in remote sensing and target recognition. Single-photon LiDAR (light detection and ranging) offers single-photon sensitivity and picosecond timing resolution, which is desirable for…

Image and Video Processing · Electrical Eng. & Systems 2020-09-07 Zheng-Ping Li , Xin Huang , Yuan Cao , Bin Wang , Yu-Huai Li , Weijie Jin , Chao Yu , Jun Zhang , Qiang Zhang , Cheng-Zhi Peng , Feihu Xu , Jian-Wei Pan

Distinguishing photon-arrival time and position is crucial for advancing quantum technology. However, capturing spatial and temporal information efficiently remains challenging. Here, we present a novel photon-detection technique to achieve…

Quantum Physics · Physics 2024-07-24 Ozora Iso , Kensuke Miyajima , Ryosuke Shimizu

By utilizing the frequency anticorrelation of two-photon states produced via spontaneous parametric down conversion (SPDC), the working principle of a novel remote spectrometer is demonstrated. With the help of a local scanning…

Quantum Physics · Physics 2016-09-08 Giuliano Scarcelli , Alejandra Valencia , Samuel Gompers , Yanhua Shih

Single molecule spectroscopy aims at unveiling often hidden but potentially very important contributions of single entities to a system's ensemble response. Albeit contributing tremendously to our ever growing understanding of molecular…

Chemical Physics · Physics 2017-12-19 Matz Liebel , Costanza Toninelli , Niek F. van Hulst

We demonstrate coherent dual frequency-comb spectroscopy for detecting variations in greenhouse gases. High signal-to-noise spectra are acquired spanning 5990 to 6260 cm^-1 (1600 to 1670 nm) covering ~700 absorption features from CO2, CH4,…

Recent advances in techniques for generating quantum light have stimulated research on novel spectroscopic measurements using quantum entangled photons. One such spectroscopy technique utilizes non-classical correlations among entangled…

Chemical Physics · Physics 2021-07-28 Yuta Fujihashi , Akihito Ishizaki

Exploring the interaction of light and matter at the ultimate limit of single photons and single emitters is of great interest both from a fundamental point of view and for emerging applications in quantum engineering. However, the…

Quantum Physics · Physics 2015-05-30 Y. L. A. Rezus , S. G. Walt , R. Lettow , A. Renn , G. Zumofen , S. Goetzinger , V. Sandoghdar

Ultra-fast and multi-dimensional spectroscopy gives a powerful looking glass into the dynamics of molecular systems. In particular two-dimensional electronic spectroscopy (2DES) provides a probe of coherence and the flow of energy within…

Quantum Physics · Physics 2021-03-31 André Anda , Jared H. Cole

The transport of CO2 across the air-water interface is central to physical oceanography and carbon sequestration. A comprehensive understanding of this process requires high-resolution diagnostics of diffusion, absorption, and reaction…

Fluid Dynamics · Physics 2025-09-23 Dongfang Zhao , Yumin Shi , Shengkai Wang

Two-dimensional electronic spectroscopy provides information on coupling and energy transfer between excited states on ultrafast timescales. Only recently, incoherent fluorescence detection has made it possible to combine this method with…

Optics · Physics 2025-05-14 Sanchayeeta Jana , Simon Durst , Lucas Ludwig , Markus Lippitz

Multispectral imaging plays an important role in many applications from astronomical imaging, earth observation to biomedical imaging. However, the current technologies are complex with multiple alignment-sensitive components, predetermined…

Optics · Physics 2021-09-17 Sujit Kumar Sahoo , Dongliang Tang , Cuong Dang

The spectrogram is a classical DSP tool used to view signals in both time and frequency. Unfortunately, the Heisenberg Uncertainty Principal limits our ability to use them for detecting and measuring narrowband signal modulation in wideband…

Information Theory · Computer Science 2014-01-22 Ray Maleh , Frank A. Boyle

Nonlinear spectroscopy with quantum entangled photons is an emerging field of research that holds the promise to achieve a superior signal-to-noise ratio and effectively isolate many-body interactions. Photon sources used for this purpose…

We demonstrate spectroscopy of incoherent light with sub-diffraction resolution. In a proof-of-principle experiment we analyze the spectrum of a pair of incoherent point-like sources whose separation is below the diffraction limit. The two…

Hyperspectroscopy is a new method of surface image taking, providing simultaneously high position and spectral resolutions which allow one to make some conclusions about chemical compositions of the surfaces. We are now studying…

Instrumentation and Detectors · Physics 2016-11-18 I. Rodionov , J-M. Bidault , I. Crotty , P. Fonte , F. Galy , V. Peskov , O. Zanette

Time-resolved spectroscopic temperature measurements of a sealed carbon dioxide sample cell were realized with an optical frequency comb combined with a two-dimensional dispersive spectrometer. A supercontinuum laser source based on an…

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