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This paper presents a new explanation of the width of gamma-ray spectra based on Rahm's electronegativity scale. This quantitatively proves, for the first time, that positrophilic electrons in the positron-electron annihilation process are…

Atomic and Molecular Clusters · Physics 2021-04-28 Yu Wu , Xiaoguang Ma , Fang Yuan , Jipeng Sui , Meishan Wang , Chuanlu Yang

The positron-electron annihilation gamma-ray spectra of linear alkanes CnH2n+2 (n=1-12) have been studied systematically. A profile quality (PQ) parameter, is introduced to assess the agreement between the obtained theoretical profiles and…

Chemical Physics · Physics 2014-01-22 X. G. Ma , F. Wang

In the article by Ma~\emph{et al.}~[Phys.~Rev.~A {\bf 94}, 052709 (2016)], $\gamma$-ray spectra for positron annihilation on molecules were calculated in the independent-particle approximation with the positron wavefunction set to unity.…

Atomic Physics · Physics 2017-03-22 D. G. Green , G. F. Gribakin

In this study, a fully self-consistent method was developed to obtain the wave functions of the positron and electrons in molecules simultaneously. The wave function of a positron at room temperature , with a characteristic energy of…

Atomic and Molecular Clusters · Physics 2020-06-24 Lin Tang , Xiaoguang Ma , Jipeng Sui , Meishan Wang , Chuanlu Yang

Calculations of gamma spectra for positron annihilation on a selection of molecules, including methane and its fluoro-substitutes, ethane, propane, butane and benzene are presented. The annihilation gamma spectra characterise the momentum…

Atomic Physics · Physics 2012-04-18 D. G. Green , S. Saha , F. Wang , G. F. Gribakin , C. M. Surko

Here we describe an advanced multi functional, variable-energy positron beam system capable of measuring the energies of multiple positron-induced electrons in coincidence with the Doppler-shifted gamma photon resulting from the…

We present measurements and theoretical modeling demonstrating the capability of Doppler Broadened annihilation gamma Spectroscopy (DBS) to provide element-specific information from the topmost atomic layer of surfaces that are either clean…

$\gamma$-ray spectra for positron annihilation with the core and valence electrons of the noble gas atoms Ar, Kr and Xe is calculated within the framework of diagrammatic many-body theory. The effect of positron-atom and short-range…

Atomic Physics · Physics 2015-03-06 D. G. Green , G. F. Gribakin

Bound electron contribution to the Doppler-shift of gamma-ray spectra in the positron-electron annihilation process of molecular methane has been studied in gas phase. Two accurate ab initio quantum mechanical schemes, i.e. the delocalized…

Atomic Physics · Physics 2013-04-01 Xiaoguang Ma , Feng Wang

Theoretical gamma-ray spectra of molecule hexane have been calculated and compared with the experimental results in both gas (Surko et al, 1997) and liquid (Kerr et al, 1965) phases. The present study reveals that in gas phase not all…

Atomic Physics · Physics 2015-03-13 Xiaoguang Ma , Feng Wang

Precise measurements of spectra of cosmic ray electrons and positrons can effectively probe the nature of dark matter (DM) particles. In a class of models where DM particles initially annihilate into a pair of intermediate particles which…

High Energy Physics - Phenomenology · Physics 2018-09-26 Lei Zu , Cun Zhang , Lei Feng , Qiang Yuan , Yi-Zhong Fan

Tracing ultrafast processes induced by interaction of light with matter is often very challenging. In molecular systems, the initially created electronic coherence becomes damped by the slow nuclear rearrangement on a femtosecond timescale…

Chemical Physics · Physics 2021-09-20 Nikolay V. Golubev , Jiří Vaníček , Alexander I. Kuleff

Measuring the Doppler broadening of the positron annihilation radiation or the angular correlation between the two annihilation gamma quanta reflects the momentum distribution of electrons seen by positrons in the material.Vacancy-type…

Materials Science · Physics 2007-05-23 I. Makkonen , M. Hakala , M. J. Puska

We present a novel method for the analysis of the Doppler broadened spectrum of gamma photons emitted following the annihilation of surface trapped positrons with the electrons of bilayer graphene supported on polycrystalline Cu substrate.…

Materials Science · Physics 2021-05-06 R. W. Gladen , V. A. Chirayath , P. A. Sterne , A. J. Fairchild , A. R. Koymen , A. H. Weiss

We present first-principles approaches based on density functional theory for calculating positron states and annihilation characteristics in condensed matter. The treatment of the electron-positron correlation effects (the enhancement of…

Materials Science · Physics 2007-05-23 B. Barbiellini , M. Hakala , R. M. Nieminen , M. J. Puska

Electron-positron momentum distributions measured by the coincidence Doppler broadening method can be used in the chemical analysis of the annihilation environment, typically a vacancy-impurity complex in a solid. In the present work, we…

Materials Science · Physics 2007-05-23 P. Folegati , I. Makkonen , R. Ferragut , M. J. Puska

We use recently released data on the positron-to-electron ratio in cosmic rays from the AMS-02 experiment to constrain dark matter annihilation in the Milky Way. Due to the yet unexplained positron excess, limits are generally weaker than…

High Energy Physics - Phenomenology · Physics 2013-10-31 Joachim Kopp

The aim of this work is to identify the mechanisms responsible for very large rates and other peculiarities observed in low-energy positron annihilation on molecules. The two mechanisms considered are: (i) Direct annihilation of the…

Atomic Physics · Physics 2009-10-31 G. F. Gribakin

Preliminary results are presented from a new positron beam system currently under development at the University of Texas at Arlington for the coincident energy measurement of Doppler-shifted annihilation quanta and positron-induced Auger…

Instrumentation and Detectors · Physics 2019-07-25 R W Gladen , V A Chirayath , A J Fairchild , N K Byrnes , A R Koymen , A H Weiss

We present the results of lifetime positron annihilation spectroscopy (PALS) for the alloys Fe21Ga and Fe22.4Ga, whose defect structure is connected with annealing from 20 to 1000C along the phase diagram of Fe21Ga and Fe22.4Ga, at the…

Materials Science · Physics 2015-09-08 L. V. El'nikova , Yu. V. Funtikov
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