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The time-dependent non-crossing approximation is used to study the transient current in a single electron transistor attached asymmetrically to two leads following a sudden change in the energy of the dot level. We show that for asymmetric…

Strongly Correlated Electrons · Physics 2015-05-13 A. Goker , B. A. Friedman , P. Nordlander

Acquiring quantitative information on charge transfer (CT) dynamics at the nanoscale remains an important scientific challenge. In particular, CT processes in single molecules at surfaces needs to be investigated to be properly controlled…

Mesoscale and Nanoscale Physics · Physics 2017-06-20 Hatem Labidi , Henry Pinto , Jerzy Leszczynski , Damien Riedel

Semiconductor nano-crystals, known as quantum dots (QDs), have attracted significant attention for their unique fluorescence properties. Under continuous excitation, QDs emit photons with intricate intensity fluctuation: the intensity of…

Applied Physics · Physics 2025-04-28 Xin Yang , Hawi Nyiera , Yonglei Sun , Jing Zhao , Kun Chen

A universal theoretical model is proposed that explains the observed shift of IR absorption and emission bands in the spectra of transition metal ions in solid solutions of semiconductor compounds. The model has been used for estimating the…

Materials Science · Physics 2022-01-05 S. V. Naydenov

The evolution of charge carriers in photoexcited room temperature ZnO nanoparticles in solution is investigated using ultrafast ultraviolet photoluminescence spectroscopy, ultrafast Zn K-edge absorption spectroscopy and ab-initio molecular…

Recent developments in high-power ultrafast optical technology and emerging theoretical frameworks in strong-field quantum electrodynamics (SF-QED) are unveiling nuanced differentiations between the semi-classical and full quantum…

We study theoretically the noise-assisted quantum exciton (electron) transfer (ET) in bio-complexes consisting of a single-level electron donor and an acceptor which has a complicated internal structure, and is modeled by many electron…

Biological Physics · Physics 2017-09-12 Shmuel Gurvitz , Alexander I. Nesterov , Gennady P. Berman

We develop a mathematical framework to analyze electrochemical impedance spectra in terms of a distribution of diffusion times (DDT) for a parallel array of random finite-length Warburg (diffusion) or Gerischer (reaction-diffusion) circuit…

Chemical Physics · Physics 2018-03-21 Juhyun Song , Martin Z. Bazant

We demonstrate electromagnetic interaction between distant quantum dots (QDs), as is observed from transient pump-probe differential reflectivity measurements. The QD-exciton lifetime is measured as a function of the probe photon energy and…

Other Condensed Matter · Physics 2009-11-11 E. W. Bogaart , J. E. M. Haverkort , R. Noetzel

A theory for the fluorescence resonance energy transfer (FRET) between a pair of semiconducting nanocrystal quantum dots is developed. Two types of donor-acceptor couplings for the FRET rate are described: dipole-dipole (d-d) and the…

Materials Science · Physics 2009-11-13 Roi Baer , Eran Rabani

We investigate the time an electronic excitation travels in a supermolecular setup using a measurement process in an open quantum-system framework. The approach is based on the stochastic Schr\"odinger equation and uses a Hamiltonian from…

Materials Science · Physics 2013-12-09 Dirk Hofmann , Heiko Appel , Massimiliano Di Ventra , Stephan Kümmel

Subwavelength ring-shaped structures of quantum emitters exhibit outstanding radiation properties and are useful for antennas, excitation transport, and storage. Taking inspiration from the oligomeric geometry of biological light-harvesting…

Interactions between nanoscale semiconductor structures form the basis for charge detectors in the solid state. Recent experimental advances have demonstrated the on-chip detection of single electron transport through a quantum dot (QD).…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Eugene V. Sukhorukov , Andrew N. Jordan , Simon Gustavsson , Renaud Leturcq , Thomas Ihn , Klaus Ensslin

We have observed strong photoluminescence from a single CdSe quantum dot embedded in a ZnSe nanowire. Exciton, biexciton and charged exciton lines have been identified unambiguously using photon correlation spectroscopy. This technique has…

We present a theoretical analysis of intraband optical transitions from the intermediate pseudo-band of confined states to the conduction band in a finite, inhomogeneous stack of self-assembled semiconductor quantum dots. The chain is…

Mesoscale and Nanoscale Physics · Physics 2015-03-20 Igor Bragar , Paweł Machnikowski

Colloidal quantum dots (cQDs) recently emerged as building blocks for semiconductor materials with tuneable properties. Electro-hydrodynamic printing can be used to obtain sub-micrometre patterns of cQDs without elaborate and aggressive…

We report fast, simultaneous charge sensing and transport measurements of gate-defined carbon nanotube quantum dots. Aluminum radio frequency single electron transistors (rf-SETs) capacitively coupled to the nanotube dot provide…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 M. J. Biercuk , D. J. Reilly , T. M. Buehler , V. C. Chan , J. M. Chow , R. G. Clark , C. M. Marcus

Semiconductor quantum dots are useful for controlling and observing quantum states and can also be used as sensors for reading out quantum bits and exploring local electronic states in nanostructures. However, challenges remain for the…

Mesoscale and Nanoscale Physics · Physics 2023-11-23 Yoshihiro Fujiwara , Motoya Shinozaki , Kazuma Matsumura , Kosuke Noro , Riku Tataka , Shoichi Sato , Takeshi Kumasaka , Tomohiro Otsuka

Through the development of new non-fullerene electron acceptor (NFA) materials, such as Y6 and its molecular derivatives, the power conversion efficiencies of organic photovoltaics (OPVs) have now exceeded 19%. However, despite this rapid…

The electronic structure of atomic quantum systems and their dynamical interaction with light is reflected in transition dipole matrix elements coupling the system's energy eigenstates. In this work, we measure phase shifts of the…