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Colloidal semiconductor nanoplatelets, in which carriers are strongly confined only along one dimension, present fundamentally different excitonic properties than quantum dots, which support strong confinement in all three dimensions. In…

Mesoscale and Nanoscale Physics · Physics 2020-01-08 Daniel Amgar , Gaoling Yang , Ron Tenne , Dan Oron

Excitons in a semiconductor monolayer form a collective resonance that can reflect resonant light with extraordinarily high efficiency. Here, we investigate the nonlinear optical properties of such atomistically thin mirrors and show that…

Mesoscale and Nanoscale Physics · Physics 2022-03-02 Valentin Walther , Lida Zhang , Susanne F. Yelin , Thomas Pohl

We present a quantitative study of many-body effects including the three-particle level on second-harmonic generation in monolayer MoS$_2$. Our approach combines many-body perturbation theory with time-dependent current-density-functional…

Materials Science · Physics 2026-04-01 Peio Garcia-Goiricelaya , Julen Ibañez-Azpiroz

Excitonic semiconductors such as transition metal dichalcogenides (TMDCs) are attractive for next-generation photovoltaics (PVs) with low cost, light weight, and low material consumption. In WS2 and other TMDCs, the simultaneous large…

Optics · Physics 2024-10-22 Adam D. Alfieri , Tobia Ruth , Cheryl Lim , Jason Lynch , Deep Jariwala

We study a mechanism to induce superconductivity in atomically thin semiconductors where excitons mediate an effective attraction between electrons. Our model includes interaction effects beyond the paradigm of phonon-mediated…

Mesoscale and Nanoscale Physics · Physics 2024-11-28 Jonas von Milczewski , Xin Chen , Atac Imamoglu , Richard Schmidt

A microscopic theory is developed to analyze the dynamics of exciton formation out of incoherent carriers in semiconductor heterostructures. The carrier Coulomb and phonon interaction is included consistently. A cluster expansion method is…

Strongly Correlated Electrons · Physics 2009-11-07 W. Hoyer , M. Kira , S. W. Koch

Realizing strong nonlinear optical responses is a long-standing goal of both fundamental and technological importance. Recently significant efforts have focused on exploring excitons in solids as a pathway to achieving nonlinearities even…

Mesoscale and Nanoscale Physics · Physics 2023-06-21 Liuxin Gu , Lifu Zhang , Ruihao Ni , Ming Xie , Dominik S. Wild , Suji Park , Houk Jang , Takashi Taniguchi , Kenji Watanabe , Mohammad Hafezi , You Zhou

The dynamics of a mobile quantum impurity in a degenerate Fermi system is a fundamental problem in many-body physics. The interest in this field has been renewed due to recent ground-breaking experiments with ultra-cold Fermi gases. Optical…

Mesoscale and Nanoscale Physics · Physics 2017-04-05 Meinrad Sidler , Patrick Back , Ovidiu Cotlet , Ajit Srivastava , Thomas Fink , Martin Kroner , Eugene Demler , Atac Imamoglu

We investigate experimentally and theoretically few-particle effects in the optical spectra of single quantum dots (QDs). Photo-depletion of the QD together with the slow hopping transport of impurity-bound electrons back to the QD are…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Arno Hartmann , Yann Ducommun , Eli Kapon , Ulrich Hohenester , Elisa Molinari

Semiconducting transition metal dichalcogenides (TMDs), such as MoSe$_2$ and WSe$_2$, exhibit unique optical and electronic properties. Vertical stacking of layers of one or more TMDs, to create heterostructures, has expanded the fields of…

The rise of organic electronics calls for versatile modeling tools. In this context, we develop a semiclassical Boltzmann theory that describes transport and excitonic processes in crystalline organic semiconductors on equal footing. The…

Materials Science · Physics 2022-05-03 Charlotte Bäcker , Linus Thummel , Carsten Timm

Temperature influences the performance of two-dimensional materials in optoelectronic devices. Indeed, the optical characterization of these materials is usually realized at room temperature. Nevertheless most {\it ab-initio} studies are…

Mesoscale and Nanoscale Physics · Physics 2016-06-06 Alejandro Molina-Sánchez , Maurizia Palummo , Andrea Marini , Ludger Wirtz

We study the linear optical absorption of bulk semiconductors in the presence of a homogeneous constant (dc) electric field with an approach suitable for including excitonic effects while working with many-band models. The absorption…

Mesoscale and Nanoscale Physics · Physics 2015-06-19 Federico Duque-Gomez , J. E. Sipe

We develop a theoretical description of Coulomb interactions between trions (charged excitons) that define a nonlinear optical response in doped two-dimensional semiconductors. First, we formulate a microscopic theory of trion-trion…

Mesoscale and Nanoscale Physics · Physics 2022-07-07 Kok Wee Song , Salvatore Chiavazzo , Ivan A. Shelykh , Oleksandr Kyriienko

Excitonic band structure is critical for investigating exciton dynamics. Theoretically, quantum effects from exchange scattering between electron-hole pairs significantly modulate exciton dispersion. Here, we report the direct observation…

Strongly Correlated Electrons · Physics 2026-03-25 Zhibin Su , Junjian Mi , Shaohua Yan , Jiade Li , Siwei Xue , Zhiyu Tao , Enling Wang , Xiongfei Shi , Hechang Lei , Zhuan Xu , Jiandong Guo , Xuetao Zhu

To advance hierarchial equations of motion as a standard theory for quantum dissipative dynamics, we put forward a mixed Heisenberg--Schrodinger scheme with block-matrix implementation on efficient evaluation of nonlinear optical response…

Chemical Physics · Physics 2015-05-30 Jian Xu , Rui-Xue Xu , Darius Abramavicius , Houdao Zhang , YiJing Yan

In bilayers of semiconducting transition metal dichalcogenides, the twist angle between layers can be used to introduce a highly regular periodic potential modulation on a length scale that is large compared to the unit cell. In such…

Materials Science · Physics 2022-04-27 N. Götting , F. Lohof , C. Gies

Two-dimensional (2D) heterostructures (HS) formed by transition-metal dichalcogenide (TMDC) monolayers offer a unique platform for the study of intralayer and interlayer excitons as well as moir\'e-pattern-induced features. Particularly,…

Mesoscale and Nanoscale Physics · Physics 2021-11-15 Mohammed Adel Aly , Manan Shah , Lorenz Maximilian Schneider , Kyungnam Kang , Martin Koch , Eui-Hyeok Yang , Arash Rahimi-Iman

Semiconductor microresonators embedding quantum wells can host tightly confined and mutually interacting excitonic, optical and mechanical modes at once. We theoretically investigate the case where the system operates in the strong…

We study the stability of excitonic Mott phases in the presence of a periodic potential and a non-local exciton-exciton interaction. The non-local interaction is treated in a mean-field approximation, while the local repulsion of the…

Materials Science · Physics 2025-11-18 K. Ziegler , R. Ya. Kezerashvili