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Excitons dominate the optical response of two-dimensional (2D) semiconductors. Strong interactions produce peculiar excitonic complexes, which provide a testing ground for exciton and quantum many-body theories. Here, we report a hitherto…

Three-dimensional (3D) excitonic complexes influence the optoelectronic properties of bulk semiconductors. More generally, correlated few-particle molecules and ions, held together by pairwise Coulomb potentials, play a fundamental role in…

Materials Science · Physics 2022-12-26 F Marsusi , E. Mostaani , N. D. Drummond

The additional layer degree of freedom in trilayer moir\'e superlattices of transition metal dichalcogenides enables the emergence of novel excitonic species, such as quadrupolar excitons, which exhibit unique excitonic interactions and…

Excitons, composite electron-hole quasiparticles, are known to play an important role in optoelectronic phenomena in many semiconducting materials. Recent experiments and theory indicate that the band-gap optics of the newly discovered…

Mesoscale and Nanoscale Physics · Physics 2015-09-02 Yuri N. Gartstein , Xiao Li , Chuanwei Zhang

As the bound state of two oppositely charged particles, excitons emerge from optically excited semiconductors as the electronic analogue of a hydrogen atom. In the two-dimensional (2D) case, realized either in quantum well systems or truly…

Optics · Physics 2022-05-13 Tobias Graß , Utso Bhattacharya , Julia Sell , Mohammad Hafezi

In this work we provide an exact and efficient numerical approach to simulate multi-time correlation functions in the Mahan-Nozi\`{e}res-De Dominicis model, which crudely mimics the spectral properties of doped two-dimensional…

Mesoscale and Nanoscale Physics · Physics 2022-06-07 Lachlan P Lindoy , Yao-Wen Chang , David R Reichman

When electron-hole pairs are excited in a semiconductor, it is a priori not clear if they form a fermionic plasma of unbound particles or a bosonic exciton gas. Usually, the exciton phase is associated with low temperatures. In atomically…

Quantum interference between one- and two-photon absorption pathways allows coherent control of interband transitions in unbiased bulk semiconductors; carrier population, carrier spin polarization, photocurrent injection, and spin current…

Other Condensed Matter · Physics 2007-05-23 R. D. R. Bhat , J. E. Sipe

2D magnetic semiconductors, which intrinsically couple a rich landscape of magnetic orders with tightly bound electron-hole pairs (excitons), present an exciting platform to investigate the interplay between optical and magnetic phenomena…

Because of the reduced dielectric screening and enhanced Coulomb interactions, two-dimensional (2D) materials like phosphorene and transition metal dichalcogenides (TMDs) exhibit strong excitonic effects, resulting in fascinating…

Materials Science · Physics 2019-11-04 Xiaoyang Zheng , Xian Zhang

We theoretically analyze a quasi-two-dimensional system of fermionic polar molecules in a harmonic transverse confining potential. The renormalized energy bands are calculated by solving the Hartree-Fock equation numerically for various…

Quantum Gases · Physics 2012-02-06 Mehrtash Babadi , Eugene Demler

We theoretically investigate exciton-polaritons in a two-dimensional (2D) semiconductor heterostructure, where a static magnetic field is applied perpendicular to the plane. To explore the interplay between magnetic field and a strong…

Mesoscale and Nanoscale Physics · Physics 2024-12-12 Emma Laird , Francesca M. Marchetti , Dmitry K. Efimkin , Meera M. Parish , Jesper Levinsen

It is well-known that exciton effects are determinant to understand the optical absorption spectrum of low-dimensional materials. However, the role of excitons in nonlinear optical responses has been much less investigated at an…

Mesoscale and Nanoscale Physics · Physics 2024-06-21 J. J. Esteve-Paredes , M. A. García-Blázquez , A. J. Uría-Álvarez , M. Camarasa-Gómez , J. J. Palacios

Understanding the nature of molecular excitons in low-dimensional molecular solids is of paramount importance in fundamental photophysics and various applications such as energy harvesting, switching electronics and display devices. Despite…

Materials Science · Physics 2023-05-18 Dogyeong Kim , Sol Lee , Jiwon Park , Jinho Lee , Hee Cheul Choi , Kwanpyo Kim , Sunmin Ryu

Interaction of excitons with resident charge carriers in semiconductors gives rise to bound three-particle complexes, trions, whose optical response is conveniently described in the framework of many-body correlated Fermi polaron states.…

Mesoscale and Nanoscale Physics · Physics 2024-06-05 Z. A. Iakovlev , M. M. Glazov

Techniques for coherent multidimensional optical spectroscopy have been developed and utilised to understand many different processes, including energy transfer in photosynthesis and many-body effects in semiconductor nanostructures.…

Optics · Physics 2017-01-24 Jonathan Tollerud , Jeffrey Davis

The equilibrium and non-equilibrium optical properties of single-layer transition metal dichalcogenides (TMDs) are determined by strongly bound excitons. Exciton relaxation dynamics in TMDs have been extensively studied by time-domain…

Excitonic effects in the linear optical response of semiconductors are well-known and the subject of countless experimental and theoretical studies. For the technologically important second order nonlinear response, however, description of…

Strongly Correlated Electrons · Physics 2007-05-23 Thomas G. Pedersen , Horia D. Cornean

In previous work we have argued that the optical properties of moderately doped two-dimensional semiconductors can be described in terms of excitons dressed by their interactions with a degenerate Fermi sea of additional charge carriers.…

Mesoscale and Nanoscale Physics · Physics 2018-06-27 Dmitry K. Efimkin , Allan H. MacDonald

The momentum-space signatures of excitons can be experimentally accessed through time-resolved (pump-probe) photoelectron spectroscopy. In this work, we develop a computational framework for exciton photoemission orbital tomography (exPOT)…