Related papers: Electronic multipoles in second harmonic generatio…
Recently Second Harmonic Generation (SHG) for the yellow exciton series in cuprous oxide has been demonstrated [J. Mund et al., Phys. Rev. B 98, 085203 (2018)]. Assuming perfect $O_{\mathrm{h}}$ symmetry, SHG is forbidden along certain…
Optical coating, an integral part of many optical systems, is prone to damage from environmental exposure and laser irradiation. This underscores the need for reliable and sensitive coating diagnostics. We introduce second harmonic…
Second-harmonic generation (SHG) has emerged as a promising tool for detecting electronic and magnetic structures in noncentrosymmetric materials, but 100$\%$ spin-polarized SHG has not been reported. In this work, we demonstrate nearly…
Multipole expansion methods have been primarily used for analyzing the electromagnetic scattering from non-magnetic isotropic dielectric scatterers, and studies about the scattering from magnetic objects seem to be lacking. In this work, we…
Nonlinear optics is a rapidly growing field that has found a wide range of applications. A major limitation, however, is the demand of high power, especially for high-order nonlinearities. Here, by reconfiguring a multiple-scattering…
Second Harmonic Generation (SHG) from BiFeO3 nanocrystals is investigated for the first time to determine their potential as biomarkers for multiphoton imaging. Nanocrystals are produced by an auto-combustion method with TRIS as a fuel.…
Raman spectroscopy and Second Harmonic Generation (SHG) are complementary, non-destructive techniques that provide rich and distinct insights into the structural and electronic properties of materials. Raman spectroscopy offers detailed…
Topological properties in quantum materials are often governed by symmetry and tuned by crystal structure and external fields, and hence symmetry-sensitive nonlinear optical measurements in a magnetic field are a valuable probe. Here we…
The nonlinear frequency conversion of low-temporal-coherent light holds a variety of applications and has attracted considerable interest. However, its physical mechanism remains relatively unexplored, and the conversion efficiency and…
Achieving compact and efficient visible laser sources is crucial for a wide range of applications. However traditional semiconductor laser technology faces difficulties in producing high-brightness green light, leaving a green gap in…
Second harmonic generation (SHG) is forbidden in centrosymmetric molecular materials. However, a signal is frequently observed from interfaces where the symmetry is broken. Whereas the effect can be phenomenologically accommodated, an ab…
We present theoretical studies of high-order harmonic generation (HHG) driven by plasmonic fields in two-electron atomic systems. Comparing the two-active electron and single-active electron approximation models of the negative hydrogen ion…
We demonstrate supermode-based second harmonic generation in an integrated nonlinear interferometer made of linear and nonlinear directional couplers. We use a fully-fibered pump shaper to demonstrate second harmonic generation pumped by…
State-of-the-art experiments employ strong ultrafast optical fields to study the nonlinear response of electrons in solids on an attosecond time-scale. Notably, a recent experiment retrieved a 3rd order nonlinear susceptibility by comparing…
Here we employ the quasi-bound state in the continuum (quasi-BIC) resonance in all-dielectric metasurfaces for efficient nonlinear processes in consideration of the backward frequency conversion. We theoretically study the second-harmonic…
We study nonlinear response of a dimer composed of two identical Mie-resonant dielectric nanoparticles illuminated normally by a circularly polarized light. We develop a general theory describing hybridization of multipolar modes of the…
Strong-field methods in solids enable new strategies for ultrafast nonlinear spectroscopy and provide all-optical insights into the electronic properties of condensed matter in reciprocal and real space. Additionally, solid-state media…
We present a combined experimental and theoretical study of enhanced third-harmonic generation (THG) in silicon nitride metasurfaces. These structures exhibit strong resonant nonlinear responses, enabling up to two orders of magnitude…
Two-dimensional (2D) materials serve as exceptional platforms for controlled second harmonic generation (SHG), an important nonlinear optical phenomenon with diverse applications. Current approaches to SHG control often depend on…
The optical theorem relates the total scattering cross-section of a given structure with its forward scattering, but does not impose any restrictions on other directions. Strong backward-forward asymmetry in scattering could be achieved by…