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Multi-dimensional coherent spectroscopy (MDCS)1,2 is a powerful method for optical spectroscopy that has become an important tool for studying ultrafast dynamics in a wide range of systems. It is an optical analog of multidimensional…
Diffuse correlation spectroscopy (DCS) is a powerful tool for assessing microvascular hemodynamic in deep tissues. Recent advances in sensors, lasers, and deep learning have further boosted the development of new DCS methods. However,…
Dual-comb spectroscopy (DCS) utilizes a pair of broadband mutually coherent laser frequency combs to enable high-resolution, high-accuracy spectroscopic measurements with atomic-clock-level frequency referencing, and rapid, multiplexed…
In the current study, a quantum-cascade-laser-based dual-comb spectrometer (DCS) was used to paint a detailed picture of a 1.0 ms high-temperature reaction between propyne and oxygen. The DCS interfaced with a shock tube to provide…
We present an optical-optical double-resonance (OODR) spectrometer based on a 3.3 ${\mu}$m continuous wave pump and two cavity-enhanced probes: a frequency comb tunable in the 1.64 - 1.8 ${\mu}$m range, and a comb-referenced continuous wave…
We present the development and performance of an optically detected magnetic resonance (ODMR) spectrometer. The spectrometer represents advances over similar instruments in three areas: i) the exciting light is a tunable laser source which…
Ultrabroadband electro-optic sampling with few-cycle optical pulses is known to be an extremely sensitive technique to detect electric field amplitudes. By combining this method with dual-comb spectroscopy and with a new class of ultrafast…
High dynamic range (HDR) imaging is one of the biggest achievements in modern photography. Traditional solutions to HDR imaging are designed for and applied to CMOS image sensors (CIS). However, the mainstream one-micron CIS cameras today…
On-chip spectroscopy that could realize real-time fingerprinting with label-free and high-throughput detection of trace molecules is one of the 'holy grails" of sensing. Such miniaturized spectrometers would greatly enable applications in…
The transition to chaos is ubiquitous in nonlinear systems ranging from fluid dynamics and superconducting circuits to biological organisms. Optical systems driven out of equilibrium such as lasers and supercontinuum generation exhibit…
Vibrational sum- and difference-frequency generation (SFG and DFG) spectroscopy probes the nonlinear response of interfaces at mid-infrared (MIR) wavelengths while detecting upconverted signals in the visible. Recent work has moved from…
Coherent diffraction imaging (CDI) is high-resolution lensless microscopy that has been applied to image a wide range of specimens using synchrotron radiation, X-ray free electron lasers, high harmonic generation, soft X-ray laser and…
Dual-comb spectroscopy (DCS) is a powerful Fourier-transform spectroscopic technique that provides high-speed, high-resolution, and broadband measurements without moving parts. However, the high peak power of mode-locked pulses limits the…
Optical frequency division (OFD) via optical frequency combs (OFC) has enabled a leap in microwave metrology leading to noise performance never explored before. Extending the method to millimeter-wave (mmW) and terahertz (THz)-wave domain…
Optical spectroscopy of molecular radicals is an important tool in physical chemistry, and is a prerequisite for many experiments which use molecules for quantum science and precision measurement. However, even the simplest molecules have…
This paper studies different signaling techniques on the continuous spectrum (CS) of nonlinear optical fiber defined by nonlinear Fourier transform. Three different signaling techniques are proposed and analyzed based on the statistics of…
High order modulation formats constitute the most prominent way for increasing spectral efficiency in transmission systems. Coherent transceivers that support such higher order formats require heavy digital signal processing (DSP), which…
Satellite-based greenhouse gases (GHG) sensing technologies play a critical role in the study of global carbon emissions and climate change. However, none of the existing satellite-based GHG sensing technologies can achieve the measurement…
Measuring low light absorption with combined uncertainty < 1 permille is crucial in a wide range of applications. Popular cavity ring-down spectroscopy can provide ultra-high precision, below 0.01 permille, but its accuracy is strongly…
We present the design of a continuous-wave, highly sensitive optical spectrometer for millimeter-wave frequencies between 50 and 1000 GHz. The spectrometer uses photomixing of near-infrared light to generate radiation in a wide frequency…