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We present a novel method to measure transient photovoltage at nanointerfaces using ultrafast electron diffraction. In particular, we report our results on the photoinduced electronic excitations and their ensuing relaxations in a…

Materials Science · Physics 2009-11-13 Ryan A. Murdick , Ramani K. Raman , Yoshie Murooka , Chong-Yu Ruan

A model for photoassociation of ultracold atoms and molecules is presented, and applied to the case of $^{39}$K and $^{23}$Na$^{39}$K bosonic particles. The model relies on the assumption that photoaossociation is dominated by long-range…

Chemical Physics · Physics 2023-03-22 Baraa Shammout , Leon Karpa , Silke Ospelkaus , Eberhard Tiemann , Olivier Dulieu

The seamless transition between micro-scale photonics and nano-scale plasmonics requires the mitigation between different waveguiding mechanisms as well as between few orders of magnitude in the field lateral size, down to a small fraction…

Optics · Physics 2009-11-11 Pavel Ginzburg , David Arbel , Meir Orenstein

We present a method to control photodissociation by manipulating the bond softening mechanism occurring in strong shaped laser fields, by varying the chirp sign and magnitude of an ultra-short laser pulse. Manipulation of bond-softening is…

Following the lifespan of optical excitations from their creation to decay into photons is crucial in understanding materials optical properties. Macroscopically, techniques such as the photoluminescence excitation spectroscopy provide…

Strongly coupled plasmon-exciton systems offer promising applications in nanooptics. The classification of the coupling regime is currently debated both from experimental and theoretical perspectives. We present a method to unambiguously…

Mesoscale and Nanoscale Physics · Physics 2023-07-19 Felix Stete , Wouter Koopman , Matias Bargheer

We propose a system of highly efficient photoemitters comprising metal-dielectric (plasmonic-excitonic) multilayered structures. In the proposed structure, the absorption in the excitonic layer is greatly enhanced through quantum…

Mesoscale and Nanoscale Physics · Physics 2017-08-17 Takuya Matsuda , Hajime Ishihara

We explore the effects of photodissociation at the stages of post-asymptotic giant branch stars to find a mechanism able to produce multi-polar shapes. We perform two-dimensional gasdynamical simulations to model the effects of…

Solar and Stellar Astrophysics · Physics 2015-05-19 Guillermo Garcia-Segura

We investigate the formation of weakly bound, electronically excited, heteronuclear 6Li40K* molecules by single-photon photoassociation in a magneto-optical trap. We performed trap loss spectroscopy within a range of 325 GHz below the…

In coupled quantum systems pure dephasing mechanisms acting on one constituent of the hybrid system break symmetry and enable optical transitions which are forbidden in the non-coupled system, i.e., the pure dephasing bath opens a cascaded…

Quantum Physics · Physics 2022-07-26 Ruben Pompe , Matthias Hensen , Matthew Otten , Stephen K. Gray , Walter Pfeiffer

In organic photovoltaic systems, a photogenerated molecular exciton in the donor domain dissociates into a hole and an electron at the donor/acceptor heterojunction, and subsequently separate into free charge carriers that can be extracted…

Mesoscale and Nanoscale Physics · Physics 2018-07-18 Akihito Kato , Akihito Ishizaki

We develop a theory of cooperative emission of light by an ensemble of emitters, such as fluorescing molecules or semiconductor quantum dots, located near a metal nanostructure supporting surface plasmon. The primary mechanism of…

Mesoscale and Nanoscale Physics · Physics 2015-05-14 Vitaliy N. Pustovit , Tigran V. Shahbazyan

The number of eigenmodes in plasmonic nanostructures increases with complexity due to mode hybridization, raising the need for efficient mode characterization and selection. Here we experimentally demonstrate direct imaging and selective…

Physical systems with discrete energy levels are ubiquitous in nature and are fundamental building blocks of quantum technology. Realizing controllable artifcial atom- and molecule-like systems for light would allow for coherent and dynamic…

Watching the motion of electrons on their natural nanometre length- and femtosecond time scales is a fundamental goal and an open challenge of contemporary ultrafast science. Optical techniques and electron microscopy currently mostly…

Optics · Physics 2018-01-23 Jan Vogelsang , Germann Hergert , Dong Wang , Petra Groß , Christoph Lienau

Crystals of plasmonic metal nanoparticles have intriguing optical properties. They reach the regimes of ultrastrong and deep strong light-matter coupling, where the photonic states need to be included in the simulation of material…

In this paper we demonstrate the use of plasmonic focusing in conjunction with non-linear photoemisison to develop geometrically flat nanoscale electron sources with less than 40 pm-rad root mean squared (rms) normalized transverse…

We study the dislocation formation in 2D nanoscopic islands with two methods, the Molecular Static method and the Phase Field Crystal method. It is found that both methods indicate the same qualitative stages of the nucleation process. The…

Materials Science · Physics 2008-12-04 J. Jalkanen , O. Trushin , K. Elder , E. Granato , S. C. Ying , T. Ala-Nissila

Ultrafast nanophotonics is an emerging research field aimed at the development of nanodevices capable of light modulation with unprecedented speed. A promising approach exploits the optical nonlinearity of nanostructured materials (either…

Here we propose the efficient confinement of ultraviolet (UV) light into the plasmonic-photonic crystal hybrid, which can be practically developed by the self-assembly of dielectric colloidal nanosphere monolayer onto a flat aluminum (Al)…

Optics · Physics 2015-06-22 Seungwoo Lee , Juyoung Kim
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