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We examine the role of refractory organics as a major C carrier in the outer protosolar nebula and its implications for the compositions of large Kuiper belt objects (KBOs) and CI chondrites. By utilizing Rosetta measurements of refractory…
To understand the conditions under which dense, molecular gas is able to form within a galaxy, we post-process a series of three-dimensional galactic-disk-scale simulations with ray-tracing based radiative transfer and chemical network…
Complex organic molecules (COMs) have been observed in comets, hot cores and cold dense regions of the interstellar medium. It is generally accepted that these COMs form on icy dust grain through the recombination reaction of radicals…
Helioseismology has shown that the chemical composition of the Sun has changed over its lifetime. The surface abundance of helium and heavy elements is believed to have decreased by up to 10% relative to their initial values. However, this…
Context. While synthesis of organic molecules in molecular clouds or protoplanetary disks is complex, observations of interstellar grains, analyses of carbonaceous chondrites, and UV photochemistry experiments are rapidly developing and…
The presence of dust can strongly affect the chemical composition of the interstellar medium. We model the chemistry in photodissociation regions (PDRs) using both gas-phase and dust-phase chemical reactions. Our aim is to determine the…
(Exo-)planets inherit their budget of chemical elements from a protoplanetary disk. The disk temperature determines the phase of each chemical species, which sets the composition of solids and gas available for planet formation. We…
Molecular oxygen has been the subject of many observational searches as chemical models predicted it to be a reservoir of oxygen. Although it has been detected in two regions of the interstellar medium, its rarity is a challenge for…
This paper refines model predictions for the production of methane from UV-irradiated interplanetary dust particles (IDPs) now that the Rover Environmental Monitoring Station (REMS) instrument onboard the Mars Science Laboratory (MSL) Rover…
Sulfur is an abundant element in the cosmos and it is thus an important contributor to astrochemistry in the interstellar medium and in the Solar System. Astronomical observations of the gas and of the solid phases in the dense…
The chemical composition of a protoplanetary disk is determined not only by in situ chemical processes during the disk phase, but also by the history of the gas and dust before it accreted from the natal envelope. In order to understand the…
The composition of Solar System surfaces can be inferred through reflectance and emission spectroscopy, by comparing these observations to laboratory measurements and radiative transfer models. While several populations of objects appear to…
Solar and extrasolar planets are the subject of numerous studies aiming to determine their chemical composition and internal structure. In the case of extrasolar planets, the composition is important as it partly governs their potential…
Remote and in-situ observations of cometary gases have revealed the presence of a wealth of complex organic molecules, including carbon chains, alcohols, imines and the amino acid glycine. Such chemical complexity in cometary material…
We propose a chemical and dynamical process to explain the surface colors of the Kuiper belt. In our hypothesis, the initial bulk compositions of the bodies themselves can be quite diverse -- as is seen in comets -- but the early surface…
To explain the properties of dust in the interstellar medium (ISM), the presence of a refractory organic mantle is necessary. The outflows of AGB stars are among the main contributors of stellar dust to the ISM. We present the first study…
Complex organic molecules serve as indicators of molecular diversity. Their detection on comets, planets, and moons has prompted inquiries into their origins, particularly the conditions conducive to their formation. One hypothesis suggests…
In situ research on cometary chemistry began when measurements from the Giotto mission at comet 1P/Halley revealed the presence of complex organics in the coma. New telescopes and space missions have provided detailed remote and in situ…
Intending to solve the decade old problem of solar opacity, we report substantial photoabsorption uncertainty due to the effect of ion-ion correlations. By performing detailed opacity calculations of the solar mixture, we find that taking…
Because of their common origin, it was assumed that the composition of planet building blocks should, to a first order, correlate with stellar atmospheric composition, especially for refractory elements. In fact, information on the relative…