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We theoretically investigate the orientation dependence of high-harmonic generation (HHG) in monolayer transition metal dichalcogenides (TMDCs). We find that, unlike conventional solid-state and atomic layered materials such as graphene,…

Materials Science · Physics 2017-06-05 Tomohiro Tamaya , Satoru Konabe , Shiro Kawabata

Application of transition metal dichalcogenides (TMDC) in photonic, optoelectronic or valleytronic devices requires the growth of continuous monolayers, heterostructures and alloys of different materials in a single process. We present a…

Two-dimensional (2D) lateral heterojunctions of transition metal dichalcogenides (TMDCs) have become a reality in recent years. Semiconducting TMDC layers in their common H -structure have a nonzero in-plane electric polarization, which is…

Materials Science · Physics 2020-08-18 Sridevi Krishnamurthi , Geert Brocks

Recent advances in time-resolved angle-resolved photoemission spectroscopy have enabled access to ultrafast electron states and their spin dynamics in solids. Atomically thin transition metal dichalcogenides are paradigmatic two-dimensional…

Mesoscale and Nanoscale Physics · Physics 2025-02-13 Alejandro S. Gómez , Yuriko Baba , Francisco Domínguez-Adame , Rafael A. Molina

Monolayer transition metal dichalcogenides (TMDCs) constitute the core group of materials in the emerging semiconductor technology of valleytronics. While the coupled spin-valley physics of pristine TMDC materials and their heterstructures…

Mesoscale and Nanoscale Physics · Physics 2023-11-14 Chumki Nayak , Suvadip Masanta , Sukanya Ghosh , Shubhadip Moulick , Atindra Nath Pal , Indrani Bose , Achintya Singha

Photon pairs, highly entangled in polarization have been generated under femtosecond laser pulse excitation by a type I crystal source, operating in a single arm interferometric scheme. The relevant effects of temporal walk-off existing in…

Quantum Physics · Physics 2009-11-13 M. Barbieri , C. Cinelli , F. De Martini , P. Mataloni

We theoretically introduce the fundamentally fastest induction of a significant population and valley polarization in a monolayer of a transition metal dichalcogenide (i.e., $\mathrm{MoS_2}$ and $\mathrm{WS_2}$). This may be extended to…

Mesoscale and Nanoscale Physics · Physics 2018-08-22 S. Azar Oliaei Motlagh , Jhih-Sheng Wu , Vadym Apalkov , Mark I. Stockman

We theoretically investigate detuning-dependent properties of high-order harmonic generation (HHG) in monolayer transition metal dichalcogenides (TMDCs). In contrast to HHG in conventional materials, TMDCs show both parallel and…

Materials Science · Physics 2018-04-18 Tomohiro Tamaya , Satoru Konabe , Shiro Kawabata

Transition metal dichalcogenides (TMDCs) exhibit high second harmonic (SH) generation in the visible due to their non-centrosymmetric crystal structure in odd-layered form and direct bandgap transition when thinned down to a monolayer. In…

We report that femtosecond surface plasmon polariton pulses can propagate along a metal-dielectric waveguide and that they can be modulated on the femtosecond timescale by direct ultrafast optical excitation of the metal, thereby offering…

Optics · Physics 2010-09-03 K. F. MacDonald , Z. L. Samson , M. I. Stockman , N. I. Zheludev

Atomically-thin transition metal dichalcogenide crystals (TMDCs) hold great promise for future semiconductor optoelectronics due to their unique electronic and optical properties. In particular, electron-hole pairs (excitons) in TMDCs are…

Mesoscale and Nanoscale Physics · Physics 2021-10-04 M. Wurdack , E. Estrecho , S. Todd , T. Yun , M. Pieczarka , S. K. Earl , J. A. Davis , C. Schneider , A. G. Truscott , E. A. Ostrovskaya

We study the collective electronic excitations in metallic single- and bilayer transition metal dichalcogenides (TMDCs) using time dependent density functional theory in the random phase approximation. For very small momentum transfers…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 Kirsten Andersen , Kristian S. Thygesen

In certain members of the transition metal dichalcogenide (TMDC) family, laser pulses of oppositely circularly polarized light excite electrons of opposite spin. Here we show that in the few cycle limit such pulses generate not only a spin…

Mesoscale and Nanoscale Physics · Physics 2025-09-24 Deepika Gill , Sangeeta Sharma , Sam Shallcross

Recent developments in the area of resonant dielectric nanostructures has created attractive opportunities for the concentrating and manipulating light at the nanoscale and the establishment of new exciting field of all-dielectric…

We theoretically investigate the interaction of an ultrastrong femtosecond-long linearly polarized optical pulse with AB-stacked bilayer graphene. The pulse excite electrons from the valence into the conduction band, resulting in finite…

Mesoscale and Nanoscale Physics · Physics 2021-08-11 Pardeep Kumar , Thakshila M. Herath , Vadym Apalkov , Mark I. Stockman

Monolayer transition metal dichalcogenides (TMDCs) are direct gap semiconductors with unique potential for ultrathin light emitters. Yet, their photoluminescence (PL) is not completely understood. We compute the radiative recombination rate…

Materials Science · Physics 2018-07-20 Hsiao-Yi Chen , Maurizia Palummo , Davide Sangalli , Marco Bernardi

We study theoretically the electron dynamics of transition metal dichalcogenide quantum dots in the field of an ultrashort and ultrafast circularly polarized optical pulse. The quantum dots have the shape of a disk and their electron…

Mesoscale and Nanoscale Physics · Physics 2023-09-01 Aranyo Mitra , Ahmal Jawad Zafar , Vadym Apalkov

Two-dimensional transition metal dichalcogenides (TMDC) have shown promise for various applications in optoelectronics and so-called valleytronics. Their operation and performance strongly depend on the stacking of individual layers. Here,…

Materials Science · Physics 2020-09-28 J. E. Zimmermann , B. Li , J. Hone , U. Höfer , G. Mette

To take advantage of the exceptional properties of atomically thin transition metal dichalcogenides (TMDC) for advanced devices and catalysts, integration with metallic surfaces is an efficacious approach for facilitating charge carrier…

Mesoscale and Nanoscale Physics · Physics 2024-08-27 Tao Yang , Zhipeng Huang , Stephan Sleziona , Eckart Hasselbrink , Peter Kratzer , Marika Schleberger , R. Kramer Campen , Yujin Tong

We present a significantly different reflection process from an optically thin flat metallic or dielectric layer and propose a strikingly simple method to form approximately unipolar half-cycle optical pulses via reflection of a…

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