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Dynamical control of the nonlinear optical properties of solids -- with light itself -- will be essential for future ultrafast photonic technologies. Previously, methods to modulate nonlinear processes including second-harmonic generation…

Second harmonic generation (SHG) is a non-linear optical process, where two photons coherently combine into one photon of twice their energy. Efficient SHG occurs for crystals with broken inversion symmetry, such as transition metal…

Recent experiments and calculations in topological semimetals have observed anomalously strong second-order optical nonlinearity, but yet whether the enhancement also occurs at surfaces of topological semimetals in general remains an open…

We predict frequency multiplication of surface acoustic waves in dielectric substrates via the ferromagnetic resonance of adjacent magnetic transducers when driven by microwaves. We find pure second harmonic generation (SHG) without any…

Mesoscale and Nanoscale Physics · Physics 2023-03-29 Chengyuan Cai , Xi-Han Zhou , Weichao Yu , Tao Yu

Electrical tuning of second-order nonlinearity in optical materials is attractive to strengthen and expand the functionalities of nonlinear optical technologies, though its implementation remains elusive. Here, we report the electrically…

We have studied on optical second harmonic generations (SHGs) from atomically thin MoTe2 flakes with 2H and 1T' phases. From 2H-MoTe2 samples with odd (even) numbers of layers, strong (negligible) SHGs are observed due to the…

Optics · Physics 2018-05-25 Yu Song , Ruijuan Tian , Jiulong Yang , Rui Yin , Jianlin Zhao , Xuetao Gan

The origin of the second harmonic generation (SHG) from plasmonic structures remains a subject of debate. Here, we investigate SHG from gold plasmonic nanostructures by scanning nanostructures at the single-particle level to acquire…

Since the first observation of second harmonic generation (SHG), there have been extensive studies on this nonlinear phenomenon not only to clarify its physical origin but also to realize unconventional functionalities. Nonetheless, a…

We study second harmonic generation in nonlinear, GaAs gratings. We find large enhancement of conversion efficiency when the pump field excites the guided mode resonances of the grating. Under these circumstances the spectrum near the pump…

Optics · Physics 2015-05-20 D. de Ceglia , G. D'Aguanno , N. Mattiucci , M. A. Vincenti , M. Scalora

We present a theoretical study of the characteristics of the nonlinear spin-orbital angular momentum coupling induced by second-harmonic generation in plasmonic and dielectric nanostructures made of centrosymmetric materials. In particular,…

As one of the two types of backward second-harmonic generation (SHG), symmetric SHG exhibits some physical characteristics and application prospects that are distinct from those of forward SHG. It is generally realized through quasi-phase…

Optics · Physics 2025-09-25 Ming-Yuan Gao , Zhi-Yuan Zhou , Bao-Sen Shi

We study the effect of degenerate parametric down-conversion (DPDC) in an ensemble of two-level quantum emitters (QEs) coupled via near-field interactions to a single surface plasmon (SP) mode of a nonlinear plasmonic cavity. For this…

Optics · Physics 2023-02-15 Andrei Piryatinski , Maxim Sukharev

Nano-resonator integrated with two-dimensional materials (e.g. transition metal dichalcogenides) have recently emerged as a promising nano-optoelectronic platform. Here we demonstrate resonatorenhanced second-harmonic generation (SHG) in…

Second and third harmonic generation in the opaque region of a GaAs wafer is experimentally observed both in transmission and reflection. These harmonic components can propagate through an opaque material as long as the pump is tuned to a…

Optics · Physics 2019-05-13 L. Rodriguez , J. Trull , M. Scalora , R. Vilaseca , C. Cojocaru

Second-harmonic generation microscopy is a powerful technique capable of probing local crystal symmetries and electric fields at interfaces. However, it often suffers from weak signal strength and is difficult to understand in multilayer…

We have developed a numerical method for calculating the second harmonic generation (SHG) generated by an anisotropic material whose optical properties present an arbitrary modulation in one dimension. The method is based on the Berreman…

Optics · Physics 2023-05-31 J. Ortega , C. L. Folcia , J. Etxebarria

Second harmonic generation (SHG) is a powerful optical tool for identifying non-centrosymmetric crystalline structures. Here, we analyze SHG in multilayer graphenes (MLG), with a focus on its dependence on the stacking order, encapsulation…

Mesoscale and Nanoscale Physics · Physics 2026-03-25 Patrick Johansen Sarsfield , Takaaki V. Joya , Takuto Kawakami , Mikito Koshino , Vladimir Fal'ko

Symmetry governs the selection rules of light-matter interactions in crystalline materials, making symmetry manipulation a powerful tool for tuning their optical properties. Here, we demonstrate that the hot-electron injection from a…

Optics · Physics 2025-04-02 Zhizi Guan , Zhiwei Peng , David J. Srolovitz , Jacob Khurgin , Dangyuan Lei

Non-perturbative high-harmonic generation (HHG) has recently been observed in the liquid phase, where it was demonstrated to have a different physical mechanism compared to gas and solid phases of matter. The currently best physical picture…

We present theoretical studies of high-order harmonic generation (HHG) produced by non-homogeneous fields as resulting from the illumination of plasmonic nanostructures with a short laser pulse. We show that both the inhomogeneity of the…

Atomic Physics · Physics 2012-04-27 M. F. Ciappina , J. Biegert , R. Quidant , M. Lewenstein