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Moir\'e superlattices formed by transition metal dichalcogenide (TMD) heterobilayers provide a versatile platform for studying strongly correlated electronic, excitonic, and topological phenomena in solids. In particular, angle-aligned…

The $k\cdot p$ effective mass approximation (EMA) predicts large, nearly size-independent exciton oscillator strengths in quantum confined semiconductors. Yet, experimental reports have concluded that the total oscillator strength of the…

Mesoscale and Nanoscale Physics · Physics 2017-03-06 Yanhao Tang , Mersedeh Saniepay , Chenjia Mi , Rémi Beaulac , John A. McGuire

We report the direct observation of intervalley exciton between the Q conduction valley and $\Gamma$ valence valley in bilayer WSe$_2$ by photoluminescence. The Q$\Gamma$ exciton lies at ~18 meV below the QK exciton and dominates the…

Coupling degrees of freedom of distinct nature plays a critical role in numerous physical phenomena. The recent emergence of layered materials provides a laboratory for studying the interplay between internal quantum degrees of freedom of…

Mesoscale and Nanoscale Physics · Physics 2014-01-07 Aaron M. Jones , Hongyi Yu , Jason S. Ross , Philip Klement , Nirmal J. Ghimire , Jiaqiang Yan , David G. Mandrus , Wang Yao , Xiaodong Xu

The strong excitonic effect in monolayer transition metal dichalcogenide (TMD) semiconductors has enabled many fascinating light-matter interaction phenomena. Examples include strongly coupled exciton-polaritons and nearly perfect atomic…

Mesoscale and Nanoscale Physics · Physics 2021-04-13 Hongchao Xie , Shengwei Jiang , Daniel A. Rhodes , James C. Hone , Jie Shan , Kin Fai Mak

We report that an external electric field applied normal to bilayers of transition-metal dichalcogenides TX2, M = Mo, W, X = S, Se, creates significant spin-orbit splittings and reduces the electronic band gap linearly with the field…

Materials Science · Physics 2015-06-22 Nourdine Zibouche , Pier Philipsen , Agnieszka Kuc , Thomas Heine

Bilayer van der Waals (vdW) heterostructures such as MoS2/WS2 and MoSe2/WSe2 have attracted much attention recently, particularly because of their type II band alignments and the formation of interlayer exciton as the lowest-energy…

Mesoscale and Nanoscale Physics · Physics 2017-12-14 Shiyuan Gao , Li Yang , Catalin D. Spataru

Monolayer transition metal dichalcogenide semiconductors host strongly bound two-dimensional excitonic complexes, and form an excellent platform for probing many-body physics through manipulation of Coulomb interaction. Quantum confined…

Mesoscale and Nanoscale Physics · Physics 2021-02-24 Nithin Abraham , Kenji Watanabe , Takashi Taniguchi , Kausik Majumdar

The twist angle in transition metal dichalcogenide (TMD) heterobilayers is a compelling degree of freedom that determines electron correlations and the period of lateral confinement of moir\'e excitons. Here we perform polarization-resolved…

Monolayer transition metal dichalcogenides, known for exhibiting strong excitonic resonances, constitute a very interesting and versatile platform for investigation of light-matter interactions. In this work we report on a strong coupling…

Mesoscale and Nanoscale Physics · Physics 2019-05-20 M. Król , K. Lekenta , R. Mirek , K. Łempicka , D. Stephan , K. Nogajewski , M. R. Molas , A. Babiński , M. Potemski , J. Szczytko , B. Piętka

Advent of new materials such as van der Waals heterostructures, propels new research directions in condensed matter physics and enables development of novel devices with unique functionalities. Here, we show experimentally that a monolayer…

Mesoscale and Nanoscale Physics · Physics 2018-01-24 Patrick Back , Aroosa Ijaz , Sina Zeytinoglu , Martin Kroner , Atac Imamoglu

A single monolayer of the layered semimetal WTe2 behaves as a two-dimensional topological insulator, with helical conducting edge modes surrounding a bulk state that becomes insulating at low temperatures. Here we present evidence that the…

We report on large exciton tuning in WSe$_2$ monolayers via substrate induced non-degenerate doping. We observe a redshift of $\sim$62 meV for the $A$ exciton together with a 1-2 orders of magnitude photoluminescence (PL) quenching when the…

Optoelectronic devices which allow rerouting, modulation and detection of the optical signals would be extremely beneficial for telecommunication technology. One of the most promising platforms for such devices are excitonic devices, as…

Applied Physics · Physics 2019-11-28 Yuanda Liu , Kostya S. Novoselov , Weibo Gao

We present optical spectroscopy (photoluminescence and reflectance) studies of thin layers of the transition metal dichalcogenide WSe2, with thickness ranging from mono- to tetra-layer and in the bulk limit. The investigated spectra show…

Mesoscale and Nanoscale Physics · Physics 2015-03-06 Ashish Arora , Maciej Koperski , Karol Nogajewski , Jacques Marcus , Clement Faugeras , Marek Potemski

Excitons in monolayer semiconductors have large optical transition dipole for strong coupling with light field. Interlayer excitons in heterobilayers, with layer separation of electron and hole components, feature large electric dipole that…

Mesoscale and Nanoscale Physics · Physics 2019-03-07 Wei-Ting Hsu , Bo-Han Lin , Li-Syuan Lu , Ming-Hao Lee , Ming-Wen Chu , Lain-Jong Li , Wang Yao , Wen-Hao Chang , Chih-Kang Shih

We employ ab-initio electronic structure calculations to investigate the charge-density waves and periodic lattice distortions in bilayer 2H-NbSe$_2$. We demonstrate that the vertical stacking can give rise to a variety of patterns that may…

Strongly Correlated Electrons · Physics 2024-11-08 Fabrizio Cossu , Dhani Nafday , Krisztian Palotás , Mehdi Biderang , Heung-Sik Kim , Alireza Akbari , Igor Di Marco

Two-dimensional (2D) materials serve as exceptional platforms for controlled second harmonic generation (SHG), an important nonlinear optical phenomenon with diverse applications. Current approaches to SHG control often depend on…

Mesoscale and Nanoscale Physics · Physics 2024-07-03 Soonyoung Cha , Tianyi Ouyang , Takashi Taniguchi , Kenji Watanabe , Nathaniel M. Gabor , Chun Hung Lui

Long-lived interlayer excitons with distinct spin-valley physics in van der Waals heterostructures based on transition metal dichalcogenides make them promising for information processing in next-generation devices. While the emission…

Mesoscale and Nanoscale Physics · Physics 2021-10-18 Alberto Ciarrocchi , Dmitrii Unuchek , Ahmet Avsar , Kenji Watanabe , Takashi Taniguchi , Andras Kis

Band-inverted electron-hole bilayers support quantum spin Hall insulator and exciton condensate phases. We investigate such a bilayer in an external magnetic field. We show that the interlayer correlations lead to formation of a helical…

Mesoscale and Nanoscale Physics · Physics 2016-02-09 D. I. Pikulin , P. G. Silvestrov , T. Hyart