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We report the enhancement of the optical second harmonic signal in non-centrosymmetric semiconductor CdS quantum dots, when they are placed in close contact with isolated silver nanoparticles. The intensity enhancement is about 1000. We…

Mesoscale and Nanoscale Physics · Physics 2012-02-15 Pablo M. Jais , Catalina von Bilderling , Andrea V. Bragas

Nonlinear frequency conversion plays a crucial role in advancing the functionality of next-generation optical systems. Portable metrology references and quantum networks will demand highly efficient second-order nonlinear devices, and the…

The optimization of nonlinear optical processes at the nanoscale is a crucial step for the development of nanoscale photon sources for quantum-optical networks. The development of innovative plasmonic nanoantenna designs and hybrid…

The effect of slow light on second harmonic generation in a periodically poled $\chi^{(2)}$ nonlinear medium is investigated theoretically. A linear $\pi$ phase shifted grating is used to slow the group velocity of the fundamental frequency…

Optics · Physics 2022-02-02 Thomas E. Maybour , Devin H. Smith , Peter Horak

We demonstrate phase-matched second-harmonic generation (SHG) from three-dimensional metamaterials consisting of stacked metasurfaces. To achieve phase matching, we utilize a novel mechanism based on phase engineering of the metasurfaces at…

Spin waves are attractive information carriers owing to their gigahertz-to-terahertz frequencies, nanometric wavelengths, and negligible Joule heating. Yet the efficient excitation of short-wavelength, high-frequency spin waves and the…

Mesoscale and Nanoscale Physics · Physics 2025-09-10 Mathieu Moalic , Youenn Patat , Mateusz Zelent , Maciej Krawczyk

Nonlinear second harmonic optical activity of graphene covering a gold photon sieve was determined for different polarizations. The photon sieve consists of a subwavelength gold nanohole array placed on glass. It combines the benefits of…

Mesoscale and Nanoscale Physics · Physics 2016-01-14 Michael Lobet , Michael Sarrazin , Francesca Cecchet , Nicolas Reckinger , Alexandru Vlad , Jean-François Colomer , Dan Lis

We investigate the second-order non-linear interaction as a means to generate entanglement between fields of differing wavelengths. And show that perfect entanglement can, in principle, be produced between the fundamental and second…

Quantum Physics · Physics 2015-06-26 Nicolai B. Grosse , Warwick P. Bowen , Kirk McKenzie , Ping Koy Lam

Second and third harmonic signals have been usually generated by using nonlinear crystals, but that method suffers from the low efficiency in small thicknesses. Metamaterials can be used to generate harmonic signals in small thicknesses.…

Optics · Physics 2016-07-28 Iman Sajedian , Inki Kim , Abdolnasser Zakery , Junsuk Rho

In a previous study, we have discovered that nonlinear processes can be enhanced several orders of magnitude due to the path interference effects which are introduced by Fano resonances. Emergence of this phenomenon has been demonstrated…

Quantum Physics · Physics 2014-04-16 Mehmet Emre Tasgin

Colloidal quantum dots (QDs) are an attractive medium for nonlinear optics and deterministic heterogeneous integration with photonic devices. Their intrinsic nonlinearities can be strengthened further by coupling QDs to low mode-volume…

Second-harmonic generation (SHG) is a second-order nonlinear optical process that is not allowed in media with inversion sym-metry. However, due to the broken symmetry at the surface, surface SHG still occurs, but is generally small. We…

Dielectric metasurfaces provide a unique platform for efficient harmonic generation and optical wavefront manipulation at the nanoscale. Tailoring phase and amplitude of a nonlinearly generated wave with a high emission efficiency using…

Optics · Physics 2022-10-03 David Hähnel , Jens Förstner , Viktor Myroshnychenko

Second-harmonic generation microscopy is a powerful technique capable of probing local crystal symmetries and electric fields at interfaces. However, it often suffers from weak signal strength and is difficult to understand in multilayer…

We introduce a versatile numerical method for modeling light diffraction in periodically patterned photonic structures containing quadratically nonlinear non-centrosymmetric optical materials. Our approach extends the generalized source…

Optics · Physics 2015-06-23 Martin Weismann , Dominic F. G. Gallagher , Nicolae C. Panoiu

Second-order nonlinearity gives rise to many distinctive physical phenomena, e.g., second-harmonic generation, which plays an important role in fundamental science and various applications. Lithium niobate, one of the most widely used…

Polaritons can provide strong optical field enhancement allowing to boost light-matter interaction. Here, we experimentally observe enhancement of mid-infrared second-harmonic generation (SHG) using grating-coupled surface phonon polaritons…

The interface between two different semiconductors is crucial in determining the electronic properties at the heterojunction, therefore novel techniques that can probe these regions are of particular interest. Recently it has been shown…

Mesoscale and Nanoscale Physics · Physics 2021-09-01 Frederico B. Sousa , Lucas Lafeta , Alisson R. Cadore , Prasana K. Sahoo , Leandro M. Malard

Recent years have witnessed significant developments in the study of nonlinear properties of various optical materials at the nanoscale. However, in most cases experimental results on harmonic generation from nanostructured materials are…

Plasmons facilitate a strong confinement and enhancement of near-field light, offering exciting opportunities to enhance nonlinear optical responses at the nanoscale. However, despite significant advancements, the electrically tunable range…