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Strongly out-of-equilibrium regimes in magnetic nanostructures exhibit novel properties, linked to the nonlinear nature of magnetization dynamics, which are of great fundamental and practical interest. Here, we demonstrate that field-driven…

Spatial structuring of materials at subwavelength scales underlies the concept of metamaterials possessing exotic properties beyond those of the constituent media. Temporal modulation of material parameters enables further functionalities.…

Nanoscale miniaturization has revolutionized the field of spintronics by enabling exponential growth in areal bit density. A similar leap is also expected in device speeds through successfully harnessing femtosecond magnetization dynamics.…

Dynamic reconfiguration is crucial for nanoplasmonic structures to achieve diversified functions and optimize performances; however, the dynamic reconfiguration of spatial arrangements remains a formidable technological challenge. Here, we…

Ultrafast optical pumping of spatially nonuniform magnetic textures is known to induce far-from-equilibrium spin transport effects. Here, we use ultrafast x-ray diffraction with unprecedented dynamic range to study the laser-induced…

We demonstrate the use of the magnetic-field-dependence of highly spatially confined, GHz-frequency ferromagnetic resonances in a ferromagnetic nanostructure for the detection of adsorbed magnetic nanoparticles. This is achieved in a large…

Ultrashort optical pulses can trigger a variety of non-equilibrium processes in magnetic thin films affecting electrons and spins on femtosecond timescales. In order to probe the charge and magnetic degrees of freedom simultaneously, we…

A novel polarization-modulation transient method has been developed for studying fast anisotropic relaxation in electronic excited states of polyatomic and biologically relevant molecules under excitation with femtosecond laser pulses. The…

Chemical Physics · Physics 2020-05-12 Ioanna Gorbunova , Nikolay Bezverkhnii , Maxim Sasin , Idris Gagzhiev , Oleg Vasyutinskii

Ultrafast chiro-optical spectroscopy provides unique access to the structural dynamics of molecules, spin-valley relaxation in semiconductors, and the non-equilibrium optical response of chiral nanophotonic systems. Yet, because chiral…

Atomic-scale disorder shapes the potential energy landscape traversed by photoexcited charge carriers, while the carriers themselves also dynamically reshape this landscape. However, resolving ultrafast photocarrier motion at atomic length…

Mesoscale and Nanoscale Physics · Physics 2026-04-29 Vedran Jelic , Kaedon Cleland-Host , Stefanie Adams , Mohamed Hassan , Austin Hayes , Tyler L. Cocker

Circularly-polarized extreme UV and X-ray radiation provides valuable access to the structural, electronic and magnetic properties of materials. To date, this capability was available only at large-scale X-ray facilities such as…

Optically induced demagnetization of 3d metallic ferromagnets proceeds as fast as ~100 fs and is a crucial prerequisite for spintronic applications, such as ultrafast magnetization switching and spin transport. On the 100 fs time scale, the…

Ultrafast Electron Microscopy (UEM) has been demonstrated to be an effective table-top technique for imaging the temporally-evolving dynamics of matter with subparticle spatial resolution on the time scale of atomic motion. However, imaging…

Optics · Physics 2017-08-02 M. Th. Hassan , J. S. Baskin , B. Liao , A. H. Zewail

The requirement of high space-time resolution and brightness is a great challenge for imaging atomic motion and making molecular movies. Important breakthroughs in ultrabright tabletop laser, x-ray and electron sources have enabled the…

Atomic Physics · Physics 2022-02-10 Ming Zhang , Zhenning Guo , Xiaoyu Mi , Zheng Li , Yunquan Liu

We report a novel scheme to generate laser-induced, ultrafast, intense (Tesla scale), spatially isolated, magnetic fields. Three-dimensional particle-in-cell simulations show that a femtosecond azimuthally-polarized infrared vector beam,…

Exotic magnetic textures emerging from the subtle interplay between thermodynamic and topological fluctuation have attracted intense interest due to their potential applications in spintronic devices. Recent advances in electron microscopy…

X-ray magnetic circular dichroism spectroscopy using an X-ray free electron laser is demonstrated with spectra over the Fe L$_{3,2}$-edges. This new ultrafast time-resolved capability is then applied to a fluence-dependent study of…

Spin polarized atomic ensembles can be used for the precise measurement of magnetic field. Conventional atomic magnetometers have demonstrated high sensitivities, albeit at low detection bandwidth, fundamentally limited by the Larmor…

We theoretically consider magnetization dynamics in a ferromagnetic slab induced by the magnetic field of a strong femtosecond laser pulse. The longitudinal geometry, in which the initial magnetization lies in both the plane of incidence…

Mesoscale and Nanoscale Physics · Physics 2025-04-01 Evgeny A. Karashtin , Tatiana V. Murzina

Irradiating a ferromagnetic material with an ultrashort laser pulse leads to demagnetization on a femtosecond timescale. We implement Elliott-Yafet type spin-flip scattering, mediated by electron-electron and electron-phonon collisions,…

Materials Science · Physics 2011-08-29 Benedikt Y. Mueller , T. Roth , M. Cinchetti , M. Aeschlimann , B. Rethfeld