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We report low-temperature powder X-ray and neutron diffraction studies on breathing pyrochlore magnets Cu$M$Cr$_{4}$S$_{8}$ ($M$ = Al, Ga), which undergo a magnetic transition at $T_{\rm N} \approx$ 21 and 31 K for {$M$ = Al and Ga,…

Materials Science · Physics 2024-05-09 Masaki Gen , Taro Nakajima , Hiraku Saito , Yusuke Tokunaga , Taka-hisa Arima

Double perovskite-based magnets wherein frustration and competition between emergent degrees of freedom are at play can lead to novel electronic and magnetic phenomena. Herein, we report the electronic structure and magnetic properties of…

Er_2Ti_2O_7 has been suggested to be a realization of the frustrated < 111 > XY pyrochlore lattice antiferromagnet, for which theory predicts fluctuation-induced symmetry breaking in a highly degenerate ground state manifold. We present a…

Combining thermodynamic measurements with theoretical density functional and thermodynamic calculations we demonstrate that the honeycomb lattice iridates A2IrO3 (A = Na, Li) are magnetically ordered Mott insulators where the magnetism of…

Strongly Correlated Electrons · Physics 2012-03-26 Yogesh Singh , S. Manni , J. Reuther , T. Berlijn , R. Thomale , W. Ku , S. Trebst , P. Gegenwart

Transition-metal honeycomb compounds are capturing scientific attention due to their distinctive electronic configurations, underscored by the triangular-lattice spin-orbit coupling and competition between multiple interactions, paving the…

To study the relationship between the properties of low-dimensional spin systems with weakly coupled Cu-triangles and their crystal structure, single crystals of $Cs_3Cu_3Cl_8OH$ (1) and the new $Cs_3Cu_3Cl_{7.6}Br_{0.4}OH$ (2) were grown.…

The cobalt-based honeycomb magnet BaCo$_2$(AsO$_4$)$_2$ (BCAO) has recently emerged as a promising platform for frustrated magnetism beyond conventional paradigms. Neutron-scattering experiments and first-principles calculations have…

Strongly Correlated Electrons · Physics 2026-05-19 Arnaud Ralko , Jaime Merino

Single crystals of a honeycomb lattice antiferromagnet, Tb$_2$Ir$_3$Ga$_9$ were synthesized, and the physical properties have been studied. From magnetometry, a long-range antiferromagnetic ordering at $\approx$12.5 K with highly…

Mesoscale and Nanoscale Physics · Physics 2019-11-27 Mojammel A. Khan , Qiang Zhang , Jin-Ke Bao , Randy S. Fishman , Antia S. Botana , Y. Choi , G. Fabbris , D. Haskel , John Singleton , John F. Mitchell

The AR$_2$O$_4$ family (R = rare earth) have recently been attracting interest as a new series of frustrated magnets, with the magnetic R atoms forming zigzag chains running along the $c$-axis. We have investigated polycrystalline…

Strongly Correlated Electrons · Physics 2015-06-22 A. A. Aczel , L. Li , V. O. Garlea , J. -Q. Yan , F. Weickert , M. Jaime , B. Maiorov , R. Movshovich , L. Civale , V. Keppens , D. Mandrus

The magnetic properties of a pyrochlore iridate Dy$_2$Ir$_2$O$_7$ prepared by the CsCl flux method were investigated by means of specific heat and magnetization measurements. The low temperature behaviour was confirmed to be consistent with…

Strongly Correlated Electrons · Physics 2021-08-18 Kristina Vlaskova , Martin Divis , Milan Klicpera

Magnetization (M) and magnetoresistance (MR) measurements on polycrystalline R2Mn3Si5 (R = Tb, Dy and Ho) compounds (tetragonal, space group P4/mnc) have been carried out in the temperature range of 2 K-300 K, in various applied fields.…

Materials Science · Physics 2009-11-11 R. Nirmala , S. K. Malik , A. V. Morozkin , Y. Yamamoto , H. Hori

Our polycrystalline sample study on the Yb-based chalcogenide spinels $A$Yb$_2$$X_4$ ($A =$ Cd, Mg, $X =$ S, Se) has revealed frustrated magnetism due to the antiferromagnetically coupled Heisenberg spin on the pyrochlore lattice. Our…

Strongly Correlated Electrons · Physics 2017-06-07 Tomoya Higo , Kensuke Iritani , Mario Halim , Wataru Higemoto , Takashi U. Ito , Kentaro Kuga , Kenta Kimura , Satoru Nakatsuji

Superconductivity in LaRu$_3$Si$_2$ with the honeycomb structure of Ru atoms has been investigated. It is found that the normal state specific heat C/T exhibits a deviation from the Debye model down to the lowest temperature. A relation…

Superconductivity · Physics 2012-03-23 Sheng Li , Bin Zeng , Xiangang Wan , Fei Han , Jian Tao , Huan Yang , Zhihe Wang , Hai-Hu Wen

In this study, we performed powder neutron diffraction and inelastic scattering measurements of frustrated pyrochlore Nd$_2$Ir$_2$O$_7$, which exhibits a metal-insulator transition at a temperature $T_{\rm MI}$ of 33 K. The diffraction…

Strongly Correlated Electrons · Physics 2012-02-29 K. Tomiyasu , K. Matsuhira , K. Iwasa , M. Watahiki , S. Takagi , M. Wakeshima , Y. Hinatsu , M. Yokoyama , K. Ohoyama , K. Yamada

A detailed investigation of Ba$_2$MnGe$_2$O$_7$ was performed in its low-temperature magnetoelectric state combining neutron diffraction with magnetization measurements on single crystals. In the paramagnetic state at 10 K, polarized…

Strongly Correlated Electrons · Physics 2023-03-07 A. Sazonov , H. Thoma , R. Dutta , M. Meven , A. Gukasov , R. Fittipaldi , V. Granata , T. Masuda , B. Náfrádi , V. Hutanu

We report sample preparation, structure, electrical resistivity, magnetic susceptibility and heat capacity studies of a new compound Yb$_2$Ir$_3$Ge$_5$. We find that this compound crystallizes in an orthorhombic structure with a space group…

Strongly Correlated Electrons · Physics 2009-11-10 Yogesh Singh , S. Ramakrishnan

We employ the previously published neutron scattering experiments\cite{1,2,3} to suggest that Er$_2$Ti$_2$O$_7$ has a broken-symmetry multiple-{\bf q} state with tetragonal magnetic symmetry\cite{4}. The ordered moments do not appear to lie…

Strongly Correlated Electrons · Physics 2015-05-27 A. K. R. Briffa , R. J. Mason , M. W. Long

We find that the compounds for RE = Y, La-Dy, crystallize in the tetragonal Ibam (U$_2$Co$_3$Si$_5$ type) structure whereas the compounds for RE = Er-Lu, crystallize in a new orthorhombic structure with a space group Pmmn. Samples of…

Strongly Correlated Electrons · Physics 2009-11-10 Yogesh Singh

A pressure-induced collapse of magnetic ordering in $\beta$-Li$_2$IrO$_3$ at $P_m\sim1.5- 2$ GPa has previously been interpreted as evidence for possible emergence of spin liquid states in this hyperhoneycomb iridate, raising prospects for…

We have synthesized a new intermetallic compound with a distorted Heusler structure, YbRh$_{2}$Pb. We present a study of the magnetic, thermal, and transport properties. Heat capacity measurements revealed that YbRh$_{2}$Pb orders…

Strongly Correlated Electrons · Physics 2009-11-13 D. A. Sokolov , M. S. Kim , M. C. Aronson , C. Henderson , P. W. Stephens