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The detailed nature of spatially heterogeneous dynamics of glycerol-silica nanocomposites is unraveled by combining dielectric spectroscopy with atomistic simulation and statistical mechanical theory. Analysis of the spatial mobility…

Confinement can modify the dynamics, the thermodynamics and the structural properties of liquid water, the prototypical anomalous liquid. By considering a general anomalous liquid, suitable for globular proteins, colloids or liquid metals,…

Soft Condensed Matter · Physics 2015-06-19 Fabio Leoni , Giancarlo Franzese

In this paper we derive relations between the local resistivities inside the interfacial region and the overall resistances of the surface between two phases for a mixture. These resistivities are the coefficients in the force-flux…

Soft Condensed Matter · Physics 2009-07-28 K. Glavatskiy , D. Bedeaux

Reactions at solid-water interfaces play a foundational role in water treatment systems, catalysis, chemical separations, and in predicting chemical fate and transport in the environment. Over the last century, experimental measurements and…

Chemical Physics · Physics 2022-12-14 Anastasia G. Ilgen , Kevin Leung , Louise J. Criscenti , Jeffery A. Greathouse

For an accurate description of nanofluidic systems, it is crucial to account for the transport properties of liquids at surfaces on sub-nanometer scales, where classical hydrodynamics fails due to the finite range of surface-liquid…

Soft Condensed Matter · Physics 2025-10-07 Shane R. Carlson , Roland R. Netz

Coarse grained molecular dynamics simulations are presented in which the sensitivity of the ice nucleation rate to the hydrophilicity of a graphene nanoflake is investigated. We find that an optimal interaction strength for promoting ice…

Materials Science · Physics 2015-06-01 Stephen J. Cox , Shawn M. Kathmann , Ben Slater , Angelos Michaelides

Improving interfacial thermal transport is crucial for heat dissipation in systems. Here, we design a strategy by utilizing the water adsorption-desorption process in porous metal-organic frameworks (MOFs) to tune the interfacial heat…

Materials Science · Physics 2023-02-24 Guang Wang , Hongzhao Fan , Jiawang Li , Zhigang Li , Yanguang Zhou

The motion of three-phase contact lines is one of the most relevant research topics of micro- and nano-fluidics. According to many hydrodynamic and molecular models, the dynamics of contact lines is assumed overdamped and dominated by…

Fluid Dynamics · Physics 2022-09-29 Michele Pellegrino , Berk Hess

The use of CO2 as a natural refrigerant in data center cooling, oil recovery and in CO2 capture and storage which is gaining traction in recent years involves heat transfer between CO2 and the base fluid. A need arises to improve the…

Applied Physics · Physics 2017-09-04 Zeeshan Ahmed , Ajinkya Sarode , Pratik Basarkar , Atul Bhargav , Debjyoti Banerjee

Direct Numerical Simulations of two superposed fluids in a channel with a textured surface on the lower wall have been carried out. A parametric study varying the viscosity ratio between the two fluids has been performed to mimic both {\bf…

Fluid Dynamics · Physics 2019-05-22 I. Arenas , E. Garcia , M. K. Fu , P. Orlandi , M. Hultmark , S. Leonardi

The structural characterization of microgels at interfaces is fundamental to understand both their 2D phase behavior and their role as stabilizers that enable emulsions to be broken on demand. However, this characterization is usually…

This work describes the behaviour of water molecules in 1-butyl-3-methylimidazolium tetrafluoroborate ionic liquid under nanoconfinement between graphene sheets. By means of molecular dynamics simulations, an adsorption of water molecules…

Confinement breaks the translational symmetry of materials. Such symmetry breaking can be used to obtain configurations that are not otherwise accessible in the bulk. Here, we explore the effect of substrate-liquid interactions on the…

Statistical Mechanics · Physics 2015-12-03 Amir Haji-Akbari , Pablo G. Debenedetti

The molecular mechanism of slip at the interface between polymer melts and weakly attractive smooth surfaces is investigated using molecular dynamics simulations. In agreement with our previous studies on slip flow of shear-thinning fluids,…

Soft Condensed Matter · Physics 2010-11-11 Nikolai V. Priezjev

Efficient thermal transport across solid-liquid interfaces is essential for optimizing heat dissipation in modern technological applications. This study employs molecular dynamics (MD) simulations to investigate the impact of surface…

Atomic and Molecular Clusters · Physics 2025-11-27 Viktor Mandrolko , Konstantinos Termentzidis , David Lacroix , Mykola Isaiev

Recently, a logarithmic decrease of conductivity has been observed in topological insulators at low temperatures, implying a tendency of localization of surface electrons. Here, we report quantum transport experiments on the topological…

Mesoscale and Nanoscale Physics · Physics 2014-10-09 Hong-Chao Liu , Hai-Zhou Lu , Hong-Tao He , Baikui Li , Shi-Guang Liu , Qing Lin He , Gan Wang , Iam Keong Sou , Shun-Qing Shen , Jiannong Wang

The interfacial resistance to evaporation, in particular for the case of water, is a longstanding issue. The previous data on its main characterizing parameter, the accommodation coefficient, manifest a dispersion over three orders of…

We study the relaxation of a thermal grating in multilayer materials with interface thermal resistances. The analytical development allows for the nu- merical determination of this thermal property in Approach to Equilibrium Molecular…

Materials Science · Physics 2018-05-31 Pier Luca Palla , Sonia Zampa , Evelyne Lampin , Fabrizio Cleri

Although ubiquitous in nature and industrial processes, transport processes at the interface during evaporation and condensation are still poorly understood. Experiments have shown temperature discontinuities at the interface during…

Soft Condensed Matter · Physics 2023-08-01 Gang Chen

Understanding heat transfer characteristics of phase change and enhancing thermal energy transport in nanoscale are of great interest in both theoretical and practical applications. In the present study, we investigated the nanoscale…

Computational Physics · Physics 2016-04-11 Li Li , Pengfei Ji , Yuwen Zhang