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Room-temperature (RT) two-dimensional (2D) van der Waals (vdW) ferromagnets hold immense promise for next-generation spintronic devices for information storage and processing. To achieve high-density energy-efficient spintronic devices, it…

Layered antiferromagnetism is the spatial arrangement of ferromagnetic layers with antiferromagnetic interlayer coupling. Recently, the van der Waals magnet, chromium triiodide (CrI3), emerged as the first layered antiferromagnetic…

Motivated by manipulating the magnetic order of bilayer CrI$_3$, we carry out microscopic calculations to find the magnetic order and various magnetic domains of the system in the presence of an electric field. Making use of density…

Materials Science · Physics 2022-06-17 Sahar Izadi Vishkay , Reza Asgari

CeTe$_3$ is a van der Waals antiferromagnet composed of magnetic [CeTe]$^+$ layers coupled to highly conducting Te$^{0.5-}$ square nets. Its simple quasi-two-dimensional electronic structure and cleavable nature make it an appealing…

Strongly Correlated Electrons · Physics 2026-04-29 Ryutaro Okuma , Yuita Fujisawa , Natsumi Maekawa , Akiko Nakao , Yoshihisa Ishikawa , Riki Kobayashi , Yoshinori Okada , Daichi Ueta

We study the microscopical origin of anisotropic ferromagnetism in the van der Waals magnet CrI3. We conclude that the nearest neighbors exchange is well described by the Heisenberg-Kitaev-Gamma (HKGamma) model, and we also found a nonzero…

Mesoscale and Nanoscale Physics · Physics 2021-05-19 Rodrigo Jaeschke-Ubiergo , Eric Suarez Morell , Alvaro Sebastian Nunez

Chromium triiodide is an intrinsically magnetic van der Waals material down to the single-layer limit. Here, we provide a first-principles description of finite-temperature magnetic and spectral properties of monolayer (ML) CrI$_3$ based on…

Strongly Correlated Electrons · Physics 2022-05-24 Yaroslav O. Kvashnin , Alexander N. Rudenko , Patrik Thunström , Malte Rösner , Mikhail I. Katsnelson

Graphene-based heterostructures are a promising material system for designing the topologically nontrivial Chern insulating devices. Recently, a two-dimensional (2D) monolayer ferromagnetic insulator CrI$_{3}$ was successfully synthesized…

Materials Science · Physics 2018-02-07 Jiayong Zhang , Bao Zhao , Tong Zhou , Yang Xue , Chunlan Ma , Zhongqin Yang

Magneto-optical effect refers to a rotation of polarization plane, which has been widely studied in traditional ferromagnetic metal and insulator films and scarcely in two-dimensional layered materials. Here we uncover a new nonreciprocal…

The crystallographic, magnetic, and transport properties of the van der Waals bonded, layered compound CrTe3 have been investigated on single crystal and polycrystalline materials. The crystal structure contains layers made up of lozenge…

Strongly Correlated Electrons · Physics 2017-04-19 Michael A. McGuire , V. Ovidiu Garlea , Santosh KC , Valentino R. Cooper , Jiaqiang Yan , Huibo Cao , Brian C. Sales

Merons are nontrivial topological spin textures highly relevant for many phenomena in solid state physics. Despite their importance, direct observation of such vortex quasiparticles is scarce and has been limited to a few complex materials.…

Mesoscale and Nanoscale Physics · Physics 2021-01-28 Mathias Augustin , Sarah Jenkins , Richard F. L. Evans , Kostya S. Novoselov , Elton J. G. Santos

Stacking order can significantly influence the physical properties of two-dimensional (2D) van der Waals materials. The recent isolation of atomically thin magnetic materials opens the door for control and design of magnetism via stacking…

Diverse interlayer tunability of physical properties of two-dimensional layers mostly lies in the covalent-like quasi-bonding that is significant in electronic structures but rather weak for energetics. Such characteristics result in…

Materials Science · Physics 2019-04-03 Peiheng Jiang , Cong Wang , Dachuan Chen , Zhicheng Zhong , Zhe Yuan , Zhong-Yi Lu , Wei Ji

Layered van der Waals (vdW) magnetic materials have attracted significant research interest to date. In this work, we employ the first-principles many-body perturbation theory to calculate excited-state properties of a prototype vdW magnet,…

Materials Science · Physics 2020-07-01 Linghan Zhu , Li Yang

Two dimensional van der Waals ferromagnets with honeycomb structures are expected to host the bosonic version of Dirac particles in their magnon excitation spectra. Using inelastic neutron scattering, we study spin wave excitations in…

Strongly Correlated Electrons · Physics 2021-10-29 Lebing Chen , Matthew B. Stone , Alexander I. Kolesnikov , Barry Winn , Wonhyuk Shon , Pengcheng Dai , Jae-Ho Chung

The recent discovery of magnetism in atomically thin layers of van der Waals crystals has created great opportunities for exploring light-matter interactions and magneto-optical phenomena in the two-dimensional limit. Optical and…

Materials Science · Physics 2019-06-19 Meng Wu , Zhenglu Li , Ting Cao , Steven G. Louie

Hybrid structures consisting of two-dimensional (2D) magnets and semiconductors have exhibited extensive functionalities in spintronics and opto-spintronics. In this work, we have fabricated WSe$_2$/Fe$_3$GeTe$_2$ van der Waals (vdW)…

The magnetic properties of the two isostructural molecule-based magnets, Ni(NCS)$_{2}$(thiourea)$_{2}$, $S$ = 1, [thiourea = SC(NH$_2$)$_2$] and Co(NCS)$_{2}$(thiourea)$_{2}$, $S$ = 3/2, are characterised using several techniques in order…

Magnetic proximity interactions (MPIs) between atomically-thin semiconductors and two-dimensional magnets provide a means to manipulate spin and valley degrees of freedom in nonmagnetic monolayers, without the use of applied magnetic…

Mesoscale and Nanoscale Physics · Physics 2023-04-11 Junho Choi , Christopher Lane , Jian-Xin Zhu , Scott A. Crooker

Insulating Nb$_3$Cl$_8$ is a layered chloride consisting of two-dimensional triangular layers of $S_{eff}$ = 1/2 Nb$_3$Cl$_{13}$ clusters at room temperature. Magnetic susceptibility measurement show a sharp, hysteretic drop to a…

Strongly Correlated Electrons · Physics 2017-01-20 J. P. Sheckelton , K. W. Plumb , B. A. Trump , C. L. Broholm , T. M. McQueen

The recent discovery of two-dimensional magnetic order in van-der Waals materials has stimulated a renaissance in the field of atomically-thin magnets. This has led to promising demonstrations of spintronic functionality such as tunneling…

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