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We present quantum mechanical explanations for unresolved phenomena observed in field-free molecular alignment by a femtosecond laser pulse. Quantum phase analysis of molecular rotational states reveals the physical origin of the following…

Optics · Physics 2015-04-09 Sang Jae Yun , Chul Min Kim , Jongmin Lee , Chang Hee Nam

In ultrafast experiments with gas phase molecules, the alignment of the molecular axis relative to the polarization of the interacting laser pulses plays a crucial role in determining the dynamics following this light-matter interaction.…

Chemical Physics · Physics 2025-04-14 Shashank Kumar , Eric Liu , Liang Z. Tan , Varun Makhija , Niranjan Shivaram

High-order harmonic generation by a bicircular field, which consists of two coplanar counter-rotating circularly polarized fields of frequency $r\omega$ and $s\omega$ ($r$ and $s$ are integers), is investigated for a polyatomic molecule.…

Atomic Physics · Physics 2016-10-05 Senad Odžak , Elvedin Hasović , Dejan B. Milošević

High spin magnetic molecules are promising candidates for quantum information processing because they intrinsically have multiple sublevels for information storage and computational operations. However, due to their susceptibility to the…

Quantum Physics · Physics 2021-02-11 Ye-Xin Wang , Zheng Liu , Yu-Hui Fang , Shen Zhou , Shang-Da Jiang , Song Gao

Advances in the distribution of quantum information will likely require entanglement shared across a hybrid quantum network. Many entanglement protocols require the generation of indistinguishable photons between the various nodes of the…

Based upon our previous works (Eur.Phys.J.D 6, 319(1999); Chin.Phys.Lett. 18, 236(2001)), we develop a classical approach to calculate the high-order harmonic generation of the laser driven atoms and molecules. The Coulomb singularities in…

Atomic Physics · Physics 2007-05-23 Chaohong Lee , Yiwu Duan , Wing-Ki Liu , Jian-Min Yuan , Lei Shi , Xiwen Zhu , Kelin Gao

Strong field photoemission and electron recollision provide a viable route to extract electronic and nuclear dynamics from molecular targets with attosecond temporal resolution. However, since an {\em ab-initio} treatment of even the…

Atomic Physics · Physics 2016-11-02 N. Suárez , A. Chacón , M. F. Ciappina , B. Wolter , J. Biegert , M. Lewenstein

The quantum interference between a coherent state and a single photon is an important tool in continuous variable optical quantum technologies to characterize and engineer non-Gaussian quantum states. Semiconductor quantum dots, which have…

We study quantum interference effects due to electron motion on a three-dimensional cubic lattice in a continuously-tunable magnetic field of arbitrary orientation and magnitude. These effects arise from the interference between magnetic…

Mesoscale and Nanoscale Physics · Physics 2009-10-28 Yeong-Lieh Lin , Franco Nori

Genuine quantum interference between independent nonlinear processes of different order provides a route to coherent control that cannot be reduced to a classical field interference. Here we present an all-optical analogue of coherent…

Optics · Physics 2026-01-27 Alessia Stefano , Samuel E. Fontaine , J. E. Sipe , Marco Liscidini

High-order harmonic generation (HHG) from aligned acetylene molecules interacting with mid infra-red (IR), linearly polarized laser pulses is studied theoretically using a mixed quantum-classical approach in which the electrons are…

Atomic Physics · Physics 2018-05-18 Peter Mulholland , Daniel Dundas

We observe quantum, Hong-Ou-Mandel, interference of fields produced by two remote atomic memories. High-visibility interference is obtained by utilizing the finite atomic memory time in four-photon delayed coincidence measurements.…

Quantum Physics · Physics 2015-06-26 T. Chaneliere , D. N. Matsukevich , S. D. Jenkins , S. -Y. Lan , R. Zhao , T. A. B. Kennedy , A. Kuzmich

We survey the inclusion of interferometric elements in nonlinear spectroscopy performed with quantum light. Controlled interference of electromagnetic fields coupled to matter can induce constructive or destructive contributions of…

Quantum Physics · Physics 2021-06-16 Shahaf Asban , Konstantin E. Dorfman , Shaul Mukamel

We study the quantum interference between the excitation pathways in a three-level $\Lambda$-type atom interacting with two short laser pulse trains under the conditions of electromagnetically induced transparency. The probability amplitude…

Atomic Physics · Physics 2023-06-16 Gabriela Buica

A strong inhomogeneous static electric field is used to spatially disperse a supersonic beam of polar molecules, according to their quantum state. We show that the molecules residing in the lowest-lying rotational states can be selected and…

We calculate angle-resolved above-threshold ionization spectra for diatomic molecules in linearly polarized laser fields, employing the strong-field approximation. The interference structure resulting from the individual contributions of…

Atomic Physics · Physics 2009-11-13 H. Hetzheim , C. Figueira de Morisson Faria , W. Becker

High-order harmonic generation (HHG) with relativistically strong laser pulses is considered employing electron ionization-recollisions from multiply charged ions in counterpropagating, linearly polarized attosecond pulse trains. The…

Atomic Physics · Physics 2015-05-19 Markus C. Kohler , Michael Klaiber , Karen Z. Hatsagortsyan , Christoph H. Keitel

Isotropic gases irradiated by long pulses of intense IR light can generate very high harmonics of the incident field. It is generally accepted that, due to the symmetry of the generating medium, be it an atomic or an isotropic molecular…

Atomic Physics · Physics 2016-09-28 R. E. F. Silva , P. Rivière , F. Morales , O. Smirnova , M. Ivanov , F. Martín

The double-slit experiment is the most direct demonstration of interference between individual quantum objects. Since similar experiments with single particles and more slits produce interference fringes reducible to a combination of…

Quantum Physics · Physics 2021-05-11 Lee A. Rozema , Zhao Zhuo , Tomasz Paterek , Borivoje Dakić

This paper focuses on investigating high-order harmonic generation (HHG) in graphene quantum dots (GQDs) under intense near-infrared laser fields. To model the GQD and its interaction with the laser field, we utilize a mean-field approach.…

Mesoscale and Nanoscale Physics · Physics 2023-09-15 H. K. Avetissian , A. G. Ghazaryan , Kh. V. Sedrakian , G. F. Mkrtchian