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A$_{2}$BX$_{6}$ vacancy-ordered double perovskites (VODPs) have captured substantial research interest in the scientific community as they offer environmentally friendly and stable alternatives to lead halide perovskites. In this study, we…

Materials Science · Physics 2024-11-11 Surajit Adhikari , Priya Johari

Monte Carlo simulations based on a first-principles-derived Hamiltonian are conducted to study the properties of PZT alloys compositionally modulated along the [100] pseudocubic direction near the morphotropic phase boundary (MPB). It is…

Materials Science · Physics 2009-11-10 Ningdong Huang , Zhirong Liu , Zhongqing Wu , Jian Wu , Wenhui Duan , Binglin Gu , Xiaowen Zhang

Structural phase transformations in (001)-oriented (1-x)Pb(Mg1/3Nb2/3O3)-32%PbTiO3 (PMN-x%PT) crystals have been investigated by x-ray diffraction. A C->T->MC sequence was observed in both the field-cooled (FC) and zero-field-cooled (ZFC)…

Materials Science · Physics 2009-11-10 Hu Cao , Feiming Bai , Jiefang Li , D. Viehland , Guangyong Xu , H. Hiraka , G. Shirane

The domain structure of (1-x)Pb(Mg1/3Nb2/3)O3- xPbTiO3 single crystals with composition x ~ 0.33 in the range of the morphotropic phase boundary (MPB) was studied. Based on the analysis of spontaneous strain compatibility and charge of…

Materials Science · Physics 2009-11-10 A. A. Bokov , Z. -G. Ye

The dielectric and structural order-disorder properties of as-sintered complex perovskite (x)Pb(In1/2Nb1/2)O3:(1-x)Pb(Mg1/3Nb2/3)O3 ceramics are highly influenced by the quantity of Pb(In1/2Nb1/2)O3 (PIN). High PIN quantity causes the…

Materials Science · Physics 2011-03-31 C. W. Tai , K. Z. Baba-Kishi

Using the Hubbard Hamiltonian for transition metal-3d and oxygen-2p states with perovskite geometry, we propose a new scaling procedure for a nontrivial extension of these systems to large spatial dimensions $D$. The scaling procedure is…

Condensed Matter · Physics 2009-10-28 J. Schmalian , P. Lombardo , M. Avignon , K. - H. Bennemann

In this work, we compare existing non-polarizable force fields developed to study the solid or solution phases of hybrid organic-inorganic halide perovskites with the AMOEBA polarizable force field. The aim is to test whether more…

Materials Science · Physics 2024-03-14 P. V. G. M. Rathnayake , Stefano Bernardi , Asaph Widmer-Cooper

The morphotropic phase boundary (MPB) in the magnetoelectric multiferroic BiFeO3-PbTiO3 is shown to be uniquely dependent on crystallite size. The system exhibits the phenomenon of abnormal grain growth (AGG) during sintering with abrupt…

Materials Science · Physics 2015-07-21 Bastola Narayan , V. Kothai , Rajeev Ranjan

Perovskite solid solutions PbHfO3-PbSnO3 offer valuable opportunities for studying the formation mechsnisms of incommensurate phases, owing to the presence of an intermediate (between cubic and incommensurate) phase, which is stabilized in…

Halide perovskites are a promising class of materials for optoelectronic applications, due to their excellent optoelectronic performance. However, they suffer several dynamical degradation problems, the characterization of which is…

Materials Science · Physics 2021-11-01 Sander Raaijmakers , Mike Pols , José Manuel Vicent-Luna , Shuxia Tao

The novel strain-driven morphotropic phase boundary (MPB) in highly-strained BiFeO3 thin film is featured by ordered mixed phase nanodomains (MPNs). Through scanning probe microscopy and synchrotron X-ray diffraction, eight structural…

Materials Science · Physics 2012-03-01 Lu You , Zuhuang Chen , Xi Zou , Hui Ding , Weigang Chen , Lang Chen , Guoliang Yuan , Junling Wang

The average structure of the solid solution LaMn$_{1-x}$Ga$_x$O$_3$ (LMGO) has been investigated from a symmetry-motivated approach utilizing synchrotron x-ray and neutron powder diffraction techniques. We show experimentally that a…

Strongly Correlated Electrons · Physics 2025-04-16 Ben R. M. Tragheim , Elodie A. Harbourne , Clemens Ritter , Andrew L. Goodwin , Mark S. Senn

A new lead-free (1-x)Li0.12Na0.88NbO3-xBaTiO3 (0 to x to 40) piezoelectric ceramics have been prepared using conventional ceramics processing route. Structural analysis revealed an existence of morphotropic phase boundary (MPB), separating…

Materials Science · Physics 2014-12-24 Supratim Mitra , Ajit R. Kulkarni

For decades it has been a well-known fact that among the few ferroelectric compounds in the perovskite family namely BaTiO3, KNbO3, PbTiO3 Na1/2Bi1/2TiO3 the dielectric and piezoelectric properties of BaTiO3 is considerably higher than the…

We propose experimental verification and theoretical explanation of magnetic anomalies in the complex Fe-contained double perovskite multiferroics like PbFe$_{1/2}$Nb$_{1/2}$O$_3$. The theoretical part is based on our model of coexistence…

Materials Science · Physics 2016-04-20 V. A. Stephanovich , V. V. Laguta

We report neutron inelastic scattering on single crystal 0.68Pb(Mg1/3Nb2/3O3)-0.32PbTiO3 (PMN-0.32PT), a relaxor ferroelectric material that lies within the compositional range of the morphotropic phase boundary (MPB). Data were obtained…

Materials Science · Physics 2009-11-13 Hu Cao , Chris Stock , Guangyong Xu , Peter M. Gehring , Jiefang Li , Dwight Viehland

The forging of strong correlations on decreasing temperature can take place without the arousal of conventional order. If this happens, as in some geometrically frustrated magnets, disorder can be a phenomenon more interesting than order…

Statistical Mechanics · Physics 2019-07-31 D. Slobinsky , L. Pili , R. A. Borzi

We present a theoretical study of the phase diagram of a frustrated Ising model with nearest-neighbor ferromagnetic interactions and long-range (Coulombic) antiferromagnetic interactions. For nonzero frustration, long-range ferromagnetic…

Statistical Mechanics · Physics 2022-08-30 M. Grousson , G. Tarjus , P. Viot

Structural disorder is common in metal-halide perovskites and important for understanding the functional properties of these materials. First-principles methods can address structure variation on the atomistic scale, but they are often…

Focused ion beam (FIB) techniques have been frequently used to section metal-halide perovskites for microstructural investigations. However, the ion beams directly irradiated to the sample surface may alter the properties far different from…

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