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Spin-crossover (SCO) molecules are versatile magnetic switches with applications in molecular electronics and spintronics. Downscaling devices to the single-molecule level remains, however, a challenging task since the switching mechanism…

The interplay of electric charge, spin, and orbital polarizations, coherently driven by picosecond long oscillations of light fields in spin-orbit coupled systems, is the foundation of emerging terahertz spintronics and orbitronics. The…

Utilizing an atomistic computational model which handles both translational and spin degrees of freedom, combined molecular and spin dynamics simulations have been performed to investigate the effect of vacancy defects on spin wave…

Computational Physics · Physics 2018-03-08 Mark Mudrick , Markus Eisenbach , Dilina Perera , David P. Landau

The inelastic scanning tunneling microscopy (STM) has been shown recently (Loth et al. Science 329, 1628 (2010)) to be extendable as to access the nanosecond, spin-resolved dynamics of magnetic adatoms and molecules. Here we analyze…

Atomic and Molecular Clusters · Physics 2015-06-04 Michael Schüler , Yaroslav Pavlyukh , Jamal Berakdar

In terms of the exact quantum master equation solution for open electronic systems, the coherent dynamics of two charge states described by two parallel quantum dots with one fully polarized electron on either dot is investigated in the…

Mesoscale and Nanoscale Physics · Physics 2013-08-20 Jinshuang Jin , Wei-Min Zhang , Matisse Wei-Yuan Tu , Nien-En Wang

Joint influence of two effects, namely, nonequilibrium spin injection by current, and current induced surface torque, on spin-valve type ferromagnetic metallic junctions is considered theoretically. The CPP configuration is assumed. The…

Materials Science · Physics 2007-05-23 R. J. Elliott , E. M. Epshtein , Yu. V. Gulyaev , P. E. Zilberman

The study of how spin interacts with lattice vibrations and relaxes to equilibrium provides unique insights on its chemical environment and the relation between electronic structure and molecular composition. Despite its importance for…

Materials Science · Physics 2022-08-23 Sourav Mondal , Alessandro Lunghi

Lack of inversion symmetry at a metallic surface can lead to an observable spin-orbit interaction. For certain metal surfaces, such as the Au(111) surface, the experimentally observed spin-orbit coupling results in spin rotation lengths on…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 Jamie D. Walls , Eric J. Heller

We study the triangular antiferromagnet Cu$_3$ in external electric fields, using symmetry group arguments and a Hubbard model approach. We identify a spin-electric coupling caused by an interplay between spin exchange, spin-orbit…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Mircea Trif , Filippo Troiani , Dimitrije Stepanenko , Daniel Loss

Among the possible types of magnetic dipole interactions in molecular systems, couplings between nuclear motion and the nuclear spin have probably received the least attention in molecular spectroscopy. Although very small in comparison to…

Chemical Physics · Physics 2026-04-22 Matthias Diez , Johannes K. Krondorfer , Albert Hirtenfelder , Andreas W. Hauser

We explore the influence of contact interactions on a synthetically spin-orbit coupled system of two ultracold trapped atoms. Even though the system we consider is bosonic, we show that a regime exists in which the competition between the…

Quantum Gases · Physics 2020-02-03 Ayaka Usui , Thomás Fogarty , Steve Campbell , Simon A. Gardiner , Thomas Busch

Single molecular magnets (SMMs) and Metal-Organic Frameworks (MOFs) attract significant interest due to their potential in quantum information processing, scalable quantum computing, and extended lifetimes and coherence times. The limiting…

Quantum Physics · Physics 2024-07-12 Nosheen Younas , Yu Zhang , Andrei Piryatinski , Eric R Bittner

We derive the spin-atomic vibration interaction $V_{\rm SA}$ and the spin-flip Hamiltonian $V_{\rm SF}$ of a single atomic spin in a crystal field. We here apply the perturbation theory to a model with the spin-orbit interaction and the…

Mesoscale and Nanoscale Physics · Physics 2010-11-11 Satoshi Kokado , Kikuo Harigaya , Akimasa Sakuma

The time-dependent Schrodinger equation of a many particle spin system consisting of an electron in a quantum dot interacting with the spins of the nuclei (N) in the dot due to hyperfine interaction is solved exactly for a given arbitrary…

Quantum Physics · Physics 2007-05-23 A. K. Rajagopal

Laser cooled and quantum degenerate atoms are widely being pursued as quantum simulators that may explain the behavior of strongly correlated material systems, and as the basis of today's most precise sensors. A key challenge towards these…

We investigate the spectral evolution in different metal phthalocyanine molecules on NbSe$_2$ surface using scanning tunnelling microscopy (STM) as a function of the coupling with the substrate. For manganese phthalocyanine (MnPc), we…

Mesoscale and Nanoscale Physics · Physics 2019-07-15 Shawulienu Kezilebieke , Rok Žitko , Marc Dvorak , Teemu Ojanen , Peter Liljeroth

Artificial molecules containing just one or two electrons provide a powerful platform for studies of orbital and spin quantum dynamics in nanoscale devices. A well-known example of these dynamics is tunneling of electrons between two…

The rates of a hindered molecular rotation induced by tunneling electrons are evaluated using scattering theory within the sudden approximation. Our approach explains the excitation of copper phthalocyanine molecules (CuPc) on Cu(111) as…

Materials Science · Physics 2013-12-30 J. Schaffert , M. C. Cottin , A. Sonntag , C. A. Bobisch , R. Moeller , J. -P. Gauyacq , N. Lorente

The spin-orbit coupling in the absence of spatial inversion symmetry plays an important role in realizing intriguing electronic states in solids, such as topological insulators and unconventional superconductivity. Usually, the inversion…

Strongly Correlated Electrons · Physics 2016-08-24 Satoru Hayami , Hiroaki Kusunose , Yukitoshi Motome

Spin-orbit coupling in solids is typically a single-body effect arising from relativity. In this work, we propose a spontaneous generation of spin-orbit coupling from symmetry breaking. A spin-dependent electron-phonon coupling model is…

Strongly Correlated Electrons · Physics 2024-10-23 Xiangyu Zhang , Da Wang , Congjun Wu