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The nuclear spin, being much more isolated from the environment than its electronic counterpart, enables quantum experiments with prolonged coherence times and presents a gateway towards uncovering the intricate dynamics within an atom.…

Mesoscale and Nanoscale Physics · Physics 2023-09-08 Lukas M. Veldman , Evert W. Stolte , Mark P. Canavan , Rik Broekhoven , Philip Willke , Laëtitia Farinacci , Sander Otte

Transition-metal phthalocyanine molecules have attracted considerable interest in the context of spintronics device development due to their amenability to diverse bonding regimes and their intrinsic magnetism. The latter is highly…

Strongly Correlated Electrons · Physics 2024-12-19 Sumanta Bhandary , Emiliano Poli , Gilberto Teobaldi , David D. O'Regan

Triplet excitonic state in the organic molecule may arise from a singlet excitation and the following inter-system crossing. Especially for a spin-bearing molecule, an exchange interaction between the triplet exciton and the original spin…

Quantum Physics · Physics 2014-06-12 Wei Wu

A scanning tunneling microscope can probe the inelastic spin excitations of a single magnetic atom in a surface via spin-flip assisted tunneling in which transport electrons exchange spin and energy with the atomic spin. If the inelastic…

Mesoscale and Nanoscale Physics · Physics 2015-05-19 F. Delgado , J. Fernández-Rossier

Controlling the motion of macroscopic oscillators in the quantum regime has been the subject of intense research in recent decades. In this direction, opto-mechanical systems, where the motion of micro-objects is strongly coupled with laser…

Quantum Physics · Physics 2021-06-03 Maxime Perdriat , Clément Pellet-Mary , Paul Huillery , Loïc Rondin , Gabriel Hétet

We consider a system of two spins under a scanning tunneling microscope bias and derive its master equation. We find that the tunneling elements to the electronic contacts (tip and substrate) generate an exchange interaction between the…

Mesoscale and Nanoscale Physics · Physics 2021-08-25 Baruch Horovitz , Carsten Henkel

We investigate the effects of spin-momentum locking on the interference and diffraction patterns due to a double- or single-slit in an electronic \emph{Gedankenexperiment}. We show that the inclusion of the spin-degree-of-freedom, when…

Mesoscale and Nanoscale Physics · Physics 2020-10-15 D. Bercioux , T. van den Berg , D. Ferraro , J. Rech , T. Jonckheere , T. Martin

We review the problem of spin decoherence of magnetic atoms deposited on a surface. Recent breakthroughs in scanning tunnelling microscopy (STM) make it possible to probe the spin dynamics of individual atoms, either isolated or integrated…

Mesoscale and Nanoscale Physics · Physics 2017-02-14 F. Delgado , J. Fernández-Rossier

We investigate theoretically the long-range electrostatic interactions between a ground-state homonuclear alkali-metal dimer and an excited alkali-metal atom taking into account its fine-structure. The interaction involves the combination…

Chemical Physics · Physics 2017-09-13 Maxence Lepers , Olivier Dulieu

The interplay of exchange correlations and spin-orbit interaction (SOI) on the many-body spectrum of a copper phtalocyanine (CuPc) molecule and their signatures in transport are investigated. We first derive a minimal model Hamiltonian in a…

Mesoscale and Nanoscale Physics · Physics 2015-08-20 Benjamin Siegert , Andrea Donarini , Milena Grifoni

Light carries both spin and momentum. Spin-orbit interactions of light come into play at the subwavelength scale of nano-optics and nano-photonics, where they determine the behaviour of light. These phenomena, in which the spin affects and…

The origins of indirect spin exchange in crystalline thin films of Copper Octabutoxy Phthalocyanine (Cu-OBPc) are investigated using Magnetic Circular Dichroism (MCD) spectroscopy. These studies are made possible by a solution deposition…

Control over quantum systems is typically achieved by time-dependent electric or magnetic fields. Alternatively, electronic spins can be controlled by spin-polarized currents. Here we demonstrate coherent driving of a single spin by a…

Mesoscale and Nanoscale Physics · Physics 2024-06-26 Stepan Kovarik , Richard Schlitz , Aishwarya Vishwakarma , Dominic Ruckert , Pietro Gambardella , Sebastian Stepanow

Spin-orbit interaction couples electron spins to electric fields and allows electrical monitoring of electron spins and electrical detection of spin dynamics. Competing mechanisms of spin-orbit interaction are compared, and optimal…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Emmanuel I. Rashba

We investigate the coherence properties of individual nuclear spin quantum bits in diamond [Dutt et al., Science, 316, 1312 (2007)] when a proximal electronic spin associated with a nitrogen-vacancy (NV) center is being interrogated by…

We present a platform for the simulation of quantum magnetism with full control of interactions between pairs of spins at arbitrary distances in one- and two-dimensional lattices. In our scheme, two internal atomic states represent a…

Quantum Physics · Physics 2016-09-02 C. -L. Hung , A. González-Tudela , J. I. Cirac , H. J. Kimble

Solid-state electronic spins are extensively studied in quantum information science, as their large magnetic moments offer fast operations for computing and communication, and high sensitivity for sensing. However, electronic spins are more…

Using newly developed quantum-classical hybrid framework, we investigate interaction between spin-polarized conduction electrons and a single spin wave (SW) coherently excited within a metallic ferromagnetic nanowire. When the nanowire…

Mesoscale and Nanoscale Physics · Physics 2020-06-08 Abhin Suresh , Utkarsh Bajpai , Branislav K. Nikolic

We present a new model for the study of spin-orbit coupling in interacting quasi-one-dimensional systems and solve it exactly to find the spectral properties of such systems. We show that the combination of spin-orbit coupling and…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 A. V. Moroz , K. V. Samokhin , C. H. W. Barnes

Circulating orbital currents produced by the spin-orbit interaction for a single electron spin in a quantum dot are explicitly evaluated at zero magnetic field, along with their effect on the total magnetic moment (spin and orbital) of the…

Mesoscale and Nanoscale Physics · Physics 2014-07-24 J. van Bree , A. Yu. Silov , P. M. Koenraad , M. E. Flatté
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