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We study a novel regime of the Rydberg excitation blockade using highly Stark-shifted, yet long-living, states of Rb atoms subject to electric fields above the classical ionization limit. Such states allow tuning the dipole-dipole…

A possible route to extract electronic and nuclear dynamics from molecular targets with attosecond temporal and nanometer spatial resolution is to employ recolliding electrons as `probes'. The recollision process in molecules is, however,…

We study a model for frustrated tunneling ionization using ultrashort laser pulses. The model is based on the strong field approximation and it employs the saddle point approximation to predict quasiclassical trajectories that are captured…

Quantum Physics · Physics 2021-09-22 Edvin Olofsson , Stefanos Carlström , Jan Marcus Dahlström

We study strong-field double ionization in a three-electron atom by applying a simplified, reduced-dimensionality model with three active electrons. The influence of the spin-induced symmetry of the spatial part of the wavefunction on the…

The classical dynamics of two electrons in the Coulomb potential of an attractive nucleus is chaotic in large parts of the high-dimensional phase space. Quantum spectra of two-electron atoms, however, exhibit structures which clearly hint…

Chaotic Dynamics · Physics 2009-11-10 Min-Ho Lee , Gregor Tanner , Nark Nyul Choi

Trapped ions are among the leading candidates for quantum computing technologies. Interfacing ion qubits in separate traps and interfacing ion qubits with superconducting qubits are two of the many challenges to scale up quantum computers.…

Quantum Physics · Physics 2021-06-01 Noah Van Horne , Manas Mukherjee

We theoretically study frustrated double ionization (FDI) of atoms subjected to intense circularly polarized laser pulses using a three-dimensional classical model. We find a novel "knee" structure of FDI probability as a function of…

Atomic Physics · Physics 2021-05-26 HuiPeng Kang , Shi Chen , Jing Chen , Gerhard G. Paulus

Highly excited Rydberg states are usually extremely polarizable and exceedingly sensitive to electric fields. Because of this Rydberg ions confined in electric fields have state-dependent trapping potentials. We engineer a Rydberg state…

Atomic Physics · Physics 2020-05-27 Fabian Pokorny , Chi Zhang , Gerard Higgins , Markus Hennrich

For conventional ion traps, the trapping potential is close to independent of the electronic state, providing confinement for ions dependent primarily on their charge-to-mass ratio $Q/m$. In contrast, storing ions within an optical dipole…

We use an independent electron model with semi-classical approximation to electron dynamics to investigate differential cross sections for electron emission in fast collisions of protons with ammonia molecules. An effective potential model…

Atomic Physics · Physics 2023-09-29 Alba Jorge , Marko Horbatsch , Tom Kirchner

We present a theoretical and experimental investigation of homonuclear ionizing collisions of laser-cooled metastable helium atoms, considering both the fermionic He-3 and bosonic He-4 isotope. The theoretical description combines quantum…

Other Condensed Matter · Physics 2007-05-23 R. J. W. Stas , J. M. McNamara , W. Hogervorst , W. Vassen

Strong field processes in the non-relativistic regime are insensitive to the electron spin, i.e. the observables appear to be independent of this electron property. This does not have to be the case for several active electrons where Pauli…

Femtosecond laser pulses are utilized to drive multiple ionization in gas-phase formic acid dimers and ions are studied using time-of-flight mass spectrometry. The interaction of formic acid dimer with 200 fs linearly polarized laser pulses…

Atomic and Molecular Clusters · Physics 2022-10-12 Shaun F. Sutton , Dane M. Miller , Lenin M. Quiroz , Ananya Sen , Pilarisetty Tarakeshwar , Scott G. Sayres

We observe "trilobite-like" states of ultracold 85Rb2 molecules, in which a ground-state atom is bound by the electronic wavefunction of its Rydberg-atom partner. We populate these states through the ultraviolet excitation of weakly-bound…

Atomic Physics · Physics 2015-06-15 M. A. Bellos , R. Carollo , J. Banerjee , E. E. Eyler , P. L. Gould , W. C. Stwalley

Solving the full classical four-body Coulomb problem numerically using a Wigner initial distribution we formulate a classical-quantum hybrid approach to study triple ionization by single photon absorption from the Li ground state in the…

Atomic Physics · Physics 2007-05-23 Agapi Emmanouilidou , Jan M. Rost

We show that the high energy limit for the amplitude of the double electron capture to the bound state of the Coulomb field of a nucleus with emission of a single photon is determined by behavior of the wave function in the vicinity of the…

Quantum Physics · Physics 2009-11-13 E. G. Drukarev , A. I. Mikhailov , I. A. Mikhailov , W. Scheid

We report on the fragmentation dynamics of triply charged, diatomic, molecular ions of NO and CO. Dissociative fragmentation after multiple ionization of NO and CO is studied under the impact of 200 keV proton beam using recoil-ion momentum…

Atomic Physics · Physics 2022-09-23 Avijit Duley , Narendra Nath Dutta , C. Bagdia , L. C. Tribedi , C. P. Safvan , A. H. Kelkar

Aluminum monofluoride (AlF) is a suitable molecule for laser cooling and trapping. Such experiments require an extensive spectroscopic characterization of the electronic structure. Two of the theoretically predicted higher lying triplet…

Chemical Physics · Physics 2024-03-05 N. Walter , M. Doppelbauer , S. Schaller , X. Liu , R. Thomas , S. Wright , B. G. Sartakov , G. Meijer

We investigate the dynamics of electron-electron recollisions in the double ionization of atoms in strong laser fields. The statistics of recollisions can be reformulated in terms of an area-preserving map from the observation that the…

Atomic Physics · Physics 2010-06-30 Francois Mauger , Cristel Chandre , Turgay Uzer

We show that the recently observed class of long-range ion-Rydberg molecules can be divided into two families of states, which are characterised by their unique electronic structures resulting from the ion-induced admixture of quantum…

Atomic Physics · Physics 2023-02-14 Daniel J. Bosworth , Frederic Hummel , Peter Schmelcher