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We propose a fast and non-destructive spectroscopic method for single molecular ions that implements quantum logic schemes between an atomic ion and the molecular ion of interest. Our proposal relies on a hybrid coherent manipulation of the…

High-precision hydrogen spectroscopy is an active field which helps to determine the Rydberg constant and proton charge radius, tests bound-state QED, and can search for Beyond Standard Model (BSM) Physics. Additionally, with recent…

Atomic Physics · Physics 2022-06-15 S. F. Cooper , C. Rasor , R. G. Bullis , A. D. Brandt , D. C. Yost

We discuss techniques that allow for long coherence times in laser spectroscopy experiments with two trapped ions. We show that for this purpose not only entangled ions prepared in decoherence-free subspaces can be used but also a pair of…

Quantum Physics · Physics 2011-11-10 M. Chwalla , K. Kim , T. Monz , P. schindler , M. Riebe , C. F. Roos , R. Blatt

Highly charged ions (HCIs) combine compact electronic structure with strong relativistic effects, offering both robustness against external perturbations and enhanced sensitivity to variations of the fine-structure constant. Recent advances…

Atomic Physics · Physics 2026-02-17 S. G. Porsev , M. S. Safronova

Unique spectroscopic possibilities open up if a laser beam interacts with relativistic lithium-like ions stored in the heavy ion ring accelerator SIS300 at the future Facility for Antiproton and Ion Research FAIR in Darmstadt, Germany. At a…

Atomic Physics · Physics 2015-06-26 H. Backe

The tremendous progress in high-intensity laser technology and the establishment of dedicated high-field laboratories in recent years have paved the way towards a first observation of quantum vacuum nonlinearities at the high-intensity…

High Energy Physics - Phenomenology · Physics 2018-04-11 Holger Gies , Felix Karbstein , Christian Kohlfürst , Nico Seegert

Due to their rich level structure, molecules are well-suited for probing time variation of fundamental constants, precisely measuring parity violation and time-reversal non-invariance effects, studying quantum mechanical aspects of chemical…

Quantum Physics · Physics 2015-05-30 S. Ding , D. N. Matsukevich

Femtosecond interferometry combined with acousto-optical phase modulation is an effective approach to implement various types of coherent nonlinear and multidimensional spectroscopy schemes. The high sensitivity of this method has recently…

Atomic Physics · Physics 2025-02-24 Friedemann Landmesser , Nicolai Gölz , Ulrich Bangert , Tobias Sixt , Lukas Bruder

Quantum information science and intense laser matter interaction are two apparently unrelated fields. Here, we introduce the notion of quantum information theory to intense laser driven processes by providing the quantum mechanical…

Quantum Physics · Physics 2022-12-12 Philipp Stammer

Laser spectroscopy of cold and trapped molecular ions is a powerful tool for fundamental physics, including the determination of fundamental constants, the laboratory test for their possible variation, and the search for a possible electric…

Atomic Physics · Physics 2016-02-26 Fabian Wolf , Yong Wan , Jan C. Heip , Florian Gebert , Chunyan Shi , Piet O. Schmidt

The pioneering experiments of linear spectroscopy were performed using flames in the 1800s, but nonlinear optical measurements had to wait until lasers became available in the twentieth century. Because the nonlinear cross section of…

Quantum Physics · Physics 2016-07-13 Andreas Maser , Benjamin Gmeiner , Tobias Utikal , Stephan Götzinger , Vahid Sandoghdar

Super-resolution overcoming the standard quantum limit has been intensively studied for quantum sensing applications of precision target detection over the last decades. Not only higher-order entangled photons but also phase-controlled…

Quantum Physics · Physics 2023-12-07 Sangbae Kim , Byoung S. Ham

We consider transitions of electron holes (vacancies in otherwise filled shells of atomic systems) in multiply-charged ions that, due to level-crossing of the holes, have frequencies within the range of optical atomic clocks. Strong E1…

Atomic Physics · Physics 2011-07-21 J. C. Berengut , V. A. Dzuba , V. V. Flambaum , A. Ong

We propose here a few selective highly charged ions (HCIs), namely Ni$^{12+}$ and Cu$^{13+}$, Pd$^{12+}$ and Ag$^{13+}$, that not only promise to be very high accurate optical clocks below $10^{-19}$ uncertainties, but also offer quality…

Atomic Physics · Physics 2018-04-25 Yan-mei Yu , B. K. Sahoo

An optical atomic clock scheme is developed that utilizes two lasers to establish coherent coupling between the $5s^2 \phantom{}^1S_0$ ground state of $^{88}$Sr and the first excited state, $5s5p \phantom{}^3P_0$. The coupling is mediated…

Atomic Physics · Physics 2009-11-10 Robin Santra , Ennio Arimondo , Tetsuya Ido , Chris H. Greene , Jun Ye

Coherent two-dimensional spectroscopy in IR or visible region is very effective for studying correlations, energy relaxation/transfer pathways in complex multi-chromophore or multi-mode systems. However it is usually restricted up to…

Chemical Physics · Physics 2020-09-15 Darius Abramavicius

Nonlinear spectroscopy employs a series of laser pulses to interrogate dynamics in large interacting many-body systems, and has become a highly successful method for experiments in chemical physics. Current quantum optical experiments…

Quantum Physics · Physics 2016-10-19 Frank Schlawin , Manuel Gessner , Shaul Mukamel , Andreas Buchleitner

Spectroscopy has an illustrious history delivering serendipitous discoveries and providing a stringent testbed for new physical predictions, including applications from trace materials detection, to understanding the atmospheres of stars…

Atomic Physics · Physics 2015-01-05 Gar-Wing Truong , James D. Anstie , Eric F. May , Thomas M. Stace , Andre N. Luiten

Precision spectroscopy has long played a central role in testing the foundations of physics, from the early insights that led to the development of quantum mechanics to the validation of quantum electrodynamics and the determination of…

High Energy Physics - Phenomenology · Physics 2026-02-26 Cédric Delaunay , Jean-Philippe Karr , Yotam Soreq

Precision metrology and quantum measurement often demand matter be prepared in well defined quantum states for both internal and external degrees of freedom. Laser-cooled neutral atoms localized in a deeply confining optical potential…

Quantum Physics · Physics 2009-11-13 Jun Ye , H. J. Kimble , Hidetoshi Katori